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Hierarchical material nanostructuring is considered to be a very promising direction for high performance thermoelectric materials. In this work we investigate thermal transport in hierarchically nanostructured silicon. We consider the…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Dhritiman Chakraborty , Samuel Foster , Neophytos Neophytou

Introducing hierarchical disorder from multiple defects into materials through nanostructuring is one of the most promising directions to achieve extremely low thermal conductivities and thus improve thermoelectric performance. The success…

Materials Science · Physics 2019-09-16 Laura de Sousa Oliveira , Vassilios Vargiamidis , Neophytos Neophytou

Prevailing nanostructuring strategies focus on increasing phonon scattering and reducing the mean-free-path of phonons across the spectrum. In nanoporous Si materials, for example, boundary scattering reduces thermal conductivity…

Mesoscale and Nanoscale Physics · Physics 2020-12-02 Laura de Sousa Oliveira , S. Aria Hosseini , Alex Greaney , Neophytos Neophytou

In nanostructures phonon transport behaviour is distinctly different to transport in bulk materials such that materials with ultra low thermal conductivities and enhanced thermoelectric performance can be realized. Low thermal…

Materials Science · Physics 2019-03-01 Dhritiman Chakraborty , Samuel Foster , Neophytos Neophytou

Thermal phonon transport in square- and triangular-lattice Si phononic crystal (PnC) nanostructures with a period of 300 nm was investigated by measuring the thermal conductivity using micrometer-scale time-domain thermoreflectance. The…

Mesoscale and Nanoscale Physics · Physics 2015-05-22 Junki Nakagawa , Yuta Kage , Takuma Hori , Junichiro Shiomi , Masahiro Nomura

Nanostructured materials exhibit low thermal conductivity because of the additional scattering due to phonon-boundary interactions. As these interactions are highly sensitive to the mean free path (MFP) of a given phonon mode, MFP…

Materials Science · Physics 2016-01-13 Giuseppe Romano , Keivan Esfarjani , David A. Strubbe , David Broido , Alexie M. Kolpak

Boundary-engineering in nanostructures has the potential to dramatically impact the development of materials for high-efficiency conversion of thermal energy directly into electricity. In particular, nanostructuring of semiconductors can…

Materials Science · Physics 2016-10-04 Giuseppe Romano , Alexie M. Kolpak

Because of high surface-to-volume ratio, the most prominent size effect limiting thermal transport originates from phonon-surface scattering in nanostructures. Herein we propose the mechanism of phonon scattering by the bond strength…

Mesoscale and Nanoscale Physics · Physics 2019-01-16 Guofeng Xie , Gang Zhang

Understanding the impact of lattice imperfections on nanoscale thermal transport is crucial for diverse applications ranging from thermal management to energy conversion. Grain boundaries (GBs) are ubiquitous defects in polycrystalline…

Tailoring thermal properties with nanostructured materials can be of vital importance for many applications. Generally classical phonon size effects are employed to reduce the thermal conductivity, where strong phonon scattering by…

Applied Physics · Physics 2019-10-14 Yue Xiao , Qiyu Chen , Dengke Ma , Nuo Yang , Qing Hao

Prior experimental studies showed that nanowires are promising structures for improving the thermoelectric performance of practical thermoelectric materials due to the strongly induced phonon-boundary scattering. However, few studies…

Mesoscale and Nanoscale Physics · Physics 2017-09-13 Lei Ma , Riguo Mei , Mengmeng Liu , Xuxin Zhao , Qixing Wu , Hongyuan Sun

A comprehensive rational thermal material design paradigm requires the ability to reduce and enhance the thermal conductivities of nanomaterials. In contrast to the existing ability to reduce the thermal conductivity, methods that allow to…

Mesoscale and Nanoscale Physics · Physics 2017-10-09 Abhinav Malhotra , Kartik Kothari , Martin Maldovan

Recent advances in our understanding of thermal transport in nanocrystalline systems are responsible for the integration of new technologies into advanced energy systems, including thermoelectric refrigeration systems and renewable energy…

Mesoscale and Nanoscale Physics · Physics 2019-08-12 Brian F. Donovan , Ronald J. Warzoha , R. Bharath Venkatesh , Nicholas T. Vu , Jay Wallen , Daeyeon Lee

Understanding thermal transport in silicon nanostructures is crucial for effective thermal management in semiconductor devices. In such nanostructures, boundary scattering can significantly reduce thermal conductivity. Diffusive boundary…

Materials Science · Physics 2025-10-28 Michimasa Morita , Junichiro Shiomi

Thermoelectric material provides a high hope for converting harmful and useless heat into useful energy, electricity. It can also be used as solid state Peltier coolers in integrated circuits, an outstanding challenge for electronic…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Lina Yang , Nuo Yang , Baowen Li

Nanocrystalline silicon and silicon-germanium alloys are promising thermoelectric materials that have achieved substantially improved figure of merits compared to their bulk counterparts. This enhancement is typically attributed to a…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Chengyun Hua , Austin J. Minnich

Phonon surface scattering has been at the core of heat transport engineering in nanoscale structures and devices. Herein, we demonstrate that this phonon pathway can be the sole mechanism only below a characteristic, size-dependent…

Nanostructured silicon is a promising material for thermoelectric conversion, because the thermal conductivity in silicon nanostructures can be strongly reduced with respect to that of bulk materials. We present thermal conductivity…

Mesoscale and Nanoscale Physics · Physics 2018-07-04 Giovanni Pennelli , Elisabetta Dimaggio , Massimo Macucci

Phonon properties of small Si nanowires in [110] direction have been analyzed using density functional perturbation theory. Several samples with varying diameters ranging from 0.38 to 1.5 nm have been calculated. It is found that the…

Materials Science · Physics 2022-07-06 Konstanze R. Hahn , Claudio Melis , Fabio Bernardini , Lorenzo Paulatto , Luciano Colombo

The thermal conductivity of nanostructures needs to be as small as possible so that it will have a greater efficiency for solid-state electricity generation/refrigeration by thermoelectrics. We studied how the period length and the mass…

Mesoscale and Nanoscale Physics · Physics 2013-01-14 Lina Yang , Nuo Yang , Baowen Li
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