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The creation of light-matter hybrid states, polaritons, in a cavity offers new intriguing opportunities to manipulate the electronic structure and electron dynamics of atoms and molecules. Here, we investigate the effect of electronic…

Quantum Physics · Physics 2025-07-30 Paul A. Albrecht , Eric W. Fischer , Tillmann Klamroth , Peter Saalfrank

We investigate the spatial characteristics of high-order harmonic radiation generated in argon, and observe cross-like patterns in the far field. An analytical model describing harmonics from an astigmatic driving beam reveals that these…

High-harmonic generation - the emission of high-frequency radiation by the ionization and subsequent recombination of an atomic electron driven by a strong laser field - is widely understood using a quasiclassical trajectory formalism,…

Quantum Physics · Physics 2020-07-29 Emilio Pisanty , Marcelo F. Ciappina , Maciej Lewenstein

In most proposals for the generation of entanglement in large ensembles of atoms via projective measurements, the interaction with the vacuum is responsible for both the generation of the signal that is detected and the spin depolarization…

Quantum Physics · Physics 2009-11-13 C. Genes , P. R. Berman

We demonstrate a simple method to improve the Lewenstein model for the description of high-order harmonic generation (HHG). It is shown that HHG spectra can be expressed as the product of a returning electron wave packet and the…

Atomic Physics · Physics 2007-07-31 Anh-Thu Le , Toru Morishita , C. D. Lin

The coherent radiation spectrum of two-level polar molecules with UV transition is studied at the multiphoton resonant excitation by a moderately strong laser field. The spectrum corresponding to harmonic generation and low-frequency…

Atomic Physics · Physics 2011-06-14 H. K. Avetissian , B. R. Avchyan , G. F. Mkrtchian

We introduce and demonstrate a new approach to measuring coherent electron wave packets using high-harmonic spectroscopy. By preparing a molecule in a coherent superposition of electronic states, we show that electronic coherence opens…

Chemical Physics · Physics 2014-07-09 P. M. Kraus , S. B. Zhang , A. Gijsbertsen , R. R. Lucchese , N. Rohringer , H. J. Wörner

We calculate the ground--state energy and other physical properties of the hydrogen atom inside a spherical box with an impenetrable wall. We apply the variational method and perturbation theory and compare both approximate results. We show…

Quantum Physics · Physics 2015-05-19 Francisco M. Fernández , N. Aquino , A. Flores-Riveros

We present ab initio calculations using the $R$-matrix with time dependence (RMT) method for high-order harmonic generation (HHG) in argon in a short, intense pulse regime. The calculations employ a $6$-cycle $\sin^2$ pulse at $850$ nm with…

Atomic Physics · Physics 2026-04-23 Aaron T. Bondy , Klaus Bartschat

High harmonic generation (HHG) from crystals in strong laser fields has been understood by the band theory of solid, which is based on the periodic boundary condition (PBC) of translational invariant. For systems having PBC of rotational…

Optics · Physics 2022-01-25 Yigeng Peng , Tong Wu , Guanglu Yuan , Lihan Chi , Chao Yu , Ruifeng Lu

High-order harmonic generation (HHG) in simultaneous intense near-infrared (NIR) laser light and brilliant x rays above an inner-shell absorption edge is examined. A tightly bound inner-shell electron is transferred into the continuum.…

We analyze the dynamics of two atoms with a short-ranged pair interaction in a one-dimensional harmonic trap with time-dependent frequency. Our analysis is focused on two representative cases: (i) a sudden change of the trapping frequency…

Quantum Gases · Physics 2019-07-15 M. Ebert , A. Volosniev , H. -W. Hammer

High-order harmonic generation in polyatomic molecules generally involves multiple channels, each associated with a different orbital. Their unambiguous assignment remains a major challenge for high-harmonic spectroscopy. Here we present a…

We develop a dynamic theory of output coupling, for fermionic atoms initially confined in a magnetic trap. We consider an exactly soluble one-dimensional model, with a spatially localized delta-type coupling between the atoms in the trap…

Quantum Physics · Physics 2009-11-10 P. A. S. Pires Filho , C. L. Cesar , L. Davidovich

We present a classical model for high harmonic generation during the propagation of an intense laser pulse through an atomic gas. Numerical simulations of the model show excellent quantitative agreement with the corresponding quantum model…

Atomic Physics · Physics 2018-07-04 S. A. Berman , J. Dubois , C. Chandre , M. Perin , T. Uzer

High-harmonic generation (HHG) is a typical high-order nonlinear optical phenomenon and can be used to probe electronic structures of solids. Here, we investigate the temperature dependence of HHG from Pr_{0.6}Ca_{0.4}MnO_{3} in the range…

Strongly Correlated Electrons · Physics 2025-01-27 A. Nakano , K. Uchida , Y. Tomioka , M. Takaya , Y. Okimoto , K. Tanaka

In the present paper, we investigate the high-order harmonic generation (HHG) from diatomic molecules with large internuclear distance using a strong field approximation (SFA) model. We find that the hump and dip structure emerges in the…

Atomic Physics · Physics 2009-11-13 Y. J. Chen , J. Liu

We analytically and numerically investigate the emission of high-harmonic radiation from model solids by intense few-cycle mid-infrared laser pulses. In single-active-electron approximation, we expand the active electron's wavefunction in a…

Other Condensed Matter · Physics 2019-07-26 Francisco Navarrete , Marcelo F. Ciappina , Uwe Thumm

We present a theoretical demonstration on the generation of entangled coherent states and of coherent state superpositions, with photon numbers and frequencies orders of magnitude higher than those provided by the current technology. This…

Recent years have witnessed significant developments in the study of nonlinear properties of various optical materials at the nanoscale. However, in most cases experimental results on harmonic generation from nanostructured materials are…