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In this work we study the interplay between the crystal structure and magnetism of the pyroarsenate \alpha-Cu_2As_2O_7 by means of magnetization, heat capacity, electron spin resonance and nuclear magnetic resonance measurements as well as…

The single-molecule magnets {Mn$_{70}$} and {Mn$_{84}$} are characterized by a 14-site unit cell with $S=2$ spin sites arranged in a circular geometry. Experimentally, these systems exhibit a magnetic ground state with a notably low total…

Strongly Correlated Electrons · Physics 2025-02-21 R. Rausch , C. Karrasch

The layered triangular lattice owing to $1:2$ order of $B$ and $B'$ sites in the triple perovskite $A_3 B B'_2$O$_9$ family provides an enticing domain for exploring the complex phenomena of quantum spin liquids (QSLs). We report a…

Strongly Correlated Electrons · Physics 2024-08-07 K. Bhattacharya , S. Mohanty , A. D. Hillier , M. T. F. Telling , R. Nath , M. Majumder

By using the tensor-network state algorithm, we study a spin-orbital model with SU(2)$\times$SU(2)$\times$U(1) symmetry on the triangular lattice. This model was proposed to describe some triangular $d^1$ materials and was argued to host a…

Strongly Correlated Electrons · Physics 2024-06-19 Yang Liu , Z. Y. Xie , Hong-Gang Luo , Jize Zhao

The magnetization processes of the spin-3/2 antiferromagnet LiInCr4O8 comprising a "breathing" pyrochlore lattice, which is an alternating array of small and large tetrahedra, are studied under ultrahigh magnetic fields of up to 130 T using…

Alkali superoxides differ from conventional transition metal magnets, exhibit magnetism from partially occupied oxygen molecular $\pi^*$-orbitals. Among them, CsO$_2$ stands out for its potential to exhibit novel quantum collective…

Strongly Correlated Electrons · Physics 2024-11-12 Ryota Ono , Ravi Kaushik , Sergey Artyukhin , Martin Jansen , Igor Solovyev , Russell A. Ewings

Motivated by the rich interplay among electronic correlation, spin-orbit coupling (SOC), crystal-field splitting, and geometric frustrations in the honeycomb-like lattice, we systematically investigated the electronic and magnetic…

Strongly Correlated Electrons · Physics 2013-05-01 Yongkang Luo , Chao Cao , Bingqi Si , Yuke Li , Jinke Bao , Hanjie Guo , Xiaojun Yang , Chenyi Shen , Chunmu Feng , Jianhui Dai , Guanghan Cao , Zhu-an Xu

Susceptibility, high-field magnetization and submillimeter wave electron spin resonance measurements of layered quasi-stoichiometric Li1-xNi1+xO2 are reported and compared to isomorphic NaNiO2. A new mechanism of magnetic frustration…

Strongly Correlated Electrons · Physics 2009-11-07 E. Chappel , M. D. Nunez-Regueiro , S. de Brion , G. Chouteau , V. Bianchi , D. Caurant , N. Baffier

We study effect of inhomogeneities of the lattice in the S=1/2 bond-alternating chain by using a quantum Monte Carlo method and an exact diagonalization method. We adopt a defect in the alternating order as the inhomogeneity and we call it…

Materials Science · Physics 2012-01-09 M. Nishino , H. Onishi , K. Yamaguchi , S. Miyashita

Quantum spin liquids (QSLs) are an exotic state of matter that is subject to extensive research. However, the relationship between the ubiquitous disorder and the QSL behaviors is still unclear. Here, by performing comparative experimental…

Antiferromagnetic insulators on the diamond lattice are candidate materials to host exotic magnetic phenomena ranging from spin-orbital entanglement to degenerate spiral ground-states and topological paramagnetism. Compared to other…

Strongly Correlated Electrons · Physics 2017-08-16 L. Ge , J. Flynn , J. A. M. Paddison , M. B. Stone , S. Calder , M. A. Subramanian , A. P. Ramirez , M. Mourigal

We investigate the ground-state magnetic structure of the spin-$1/2$ XXZ antiferromagnet on the triangular lattice in the easy-axis regime using the density-matrix renormalization group. By applying spiral boundary conditions, we exactly…

Strongly Correlated Electrons · Physics 2026-04-17 Masahiro Kadosawa , Masaaki Nakamura , Yukinori Ohta , Satoshi Nishimoto

We have carried out detailed bulk and local probe studies on the hexagonal oxides Ba3MIr2O9 (M=Sc,Y) where Ir is expected to have a fractional oxidation state of +4.5. In the structure, Ir-Ir dimers are arranged in an edge shared triangular…

Strongly Correlated Electrons · Physics 2014-05-06 Tusharkanti Dey , R. Kumar , A. V. Mahajan , S. D. Kaushik , V. Siruguri

TmZn2GaO5 is a newly synthesized triangular lattice magnet that exhibits a unique quantum phase characterized by strong Ising anisotropy, a pseudo-doublet crystal electric field ground state, and a low-energy gapped excitation at the K…

We derive a spin-orbital Hamiltonian for a triangular lattice of e_g orbital degenerate (Ni^{3+}) transition metal ions interacting via 90 degree superexchange involving (O^{2-}) anions, taking into account the on-site Coulomb interactions…

Strongly Correlated Electrons · Physics 2009-11-11 Albert J. W. Reitsma , Louis F. Feiner , Andrzej M. Oles'

Polycrystalline samples of NaYbO$_2$ are investigated by bulk magnetization and specific-heat measurements, as well as by nuclear magnetic resonance (NMR) and electron spin resonance (ESR) as local probes. No signatures of long-range…

Strongly Correlated Electrons · Physics 2019-05-08 K. M. Ranjith , D. Dmytriieva , S. Khim , J. Sichelschmidt , S. Luther , D. Ehlers , H. Yasuoka , J. Wosnitza , A. A. Tsirlin , H. Kühne , M. Baenitz

The peculiar field-dependent magnetism of Na0.82CoO2 has been investigated through an analysis of its DC and AC spin susceptibilities. To account for the easily activated narrow b2g-a1g gap of the crystal field for Co in the cobalt oxide…

Strongly Correlated Electrons · Physics 2016-10-04 G. J. Shu , F. C. Chou

The magnetic ground state of the hyper-kagome lattice in Na4Ir3O8 is explored via combined bulk magnetization, muon spin relaxation, and neutron scattering measurements. A short-range, frozen, state comprised of quasi-static moments…

Recently, the mixed transition metal oxides of the form Li(Ni1-y-zCoyMnz)O2, have become the center of attention as promising candidates for novel battery material. These materials have also revealed very interesting magnetic properties due…

Strongly Correlated Electrons · Physics 2013-07-30 J. Magnus Wikberg , Martin Mansson , Mohammed Dahbi , Kazuya Kamazawa , Jun Sugiyama

A large body of knowledge about magnetism is attained from models of interacting spins, which usually reside on magnetic ions. Proposals beyond the ionic picture are uncommon and seldom verified by direct observations in conjunction with…