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We study intraband high-order harmonic generation arising from a band-gap material driven by a linearly polarized laser field. We factorize the intraband high-order harmonic-generation signal into intracycle and intercycle terms. The…

We find that, for sufficiently strong mid-IR fields, transitions between different conduction bands play an important role in the generation of high-order harmonics in a dielectric. The transitions make a significant contribution to the…

Other Condensed Matter · Physics 2015-06-22 Peter G. Hawkins , Misha Yu. Ivanov , Vladislav S. Yakovlev

High harmonic generation in solids is becoming an important method for strong field solid state physics research. The power scale relationship between high harmonics and the driving laser is investigated both experimentally and…

Optics · Physics 2022-08-23 Shuai Wang , Xinkui He , Yueying Liang , Yabei Su , Shaobo Fang , Zhiyi Wei

An interesting property of high harmonic generation in solids is its laser polarization dependent nature which in turn provides information about the crystal and band structure of the generation medium. Here we report on the linear…

The strong ellipticity dependence of high-harmonic generation in gases enables numerous experimental techniques that are nowadays routinely used, for instance, to create isolated attosecond pulses. Extending such techniques to high-harmonic…

High-harmonic generation by a laser-driven solid slab is simulated using time-dependent density functional theory. Multiple harmonic plateaus up to very high harmonic orders are observed already at surprisingly low field strengths. The full…

Atomic Physics · Physics 2017-11-29 Kenneth K. Hansen , Tobias Deffge , Dieter Bauer

The generation of high harmonics is a strongly nonlinear effect that allows to probe properties of the target and to study electron dynamics in matter. It has been investigated in many different kinds of targets, including molecular gases,…

Quantum Physics · Physics 2026-05-06 Lina Bielke , Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer

We theoretically investigate the orientation dependence of high-harmonic generation (HHG) in monolayer transition metal dichalcogenides (TMDCs). We find that, unlike conventional solid-state and atomic layered materials such as graphene,…

Materials Science · Physics 2017-06-05 Tomohiro Tamaya , Satoru Konabe , Shiro Kawabata

Second-order phase transitions appear as a divergence in one of the linear response functions. For a system of correlated electrons, the relevant divergent response can and does involve many-particle observables, most famously the double…

Strongly Correlated Electrons · Physics 2024-06-17 Erik G. C. P. van Loon

We show that interlayer charge transfer in 2D materials can be driven by an in-plane electric field, giving rise to electrical multipole generation in linear and second order of in-plane field. The linear and nonlinear effects have quantum…

Mesoscale and Nanoscale Physics · Physics 2024-09-05 Huiyuan Zheng , Dawei Zhai , Cong Xiao , Wang Yao

We present analytically and numerically the spectrum of high harmonic emission generated by twisted electrons in the presence of linearly polarized light. Ensuing transitions from electronic continuum states with orbital angular momentum to…

Atomic Physics · Physics 2019-10-23 Sebastian Gemsheim , Jan-Michael Rost

We theoretically and experimentally investigate orientation-dependent high-harmonic generation (HHG) in zinc oxide subjected to intense femtosecond mid-infrared (MIR) laser pulses. In agreement with past measurements from literature, we…

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas

We investigate the multielectron effects on high-harmonic generation from solid-state materials using the time-dependent Hartree-Fock theory. We find qualitative change in harmonic spectra, in particular, multiple-plateau formation at…

Kerr-type nonlinearities form the basis for our physical understanding of nonlinear optical phenomena in condensed matter, such as self-focusing, solitary waves, and wave mixing. In strong fields, they are complemented by higher-order…

High harmonic generation (HHG) in solids has recently emerged as a powerful all-optical approach for probing material properties and ultrafast electron dynamics in quantum systems. It has been widely applied for studying two-dimensional and…

Optics · Physics 2026-04-28 Eyal Uzner , Ofer Neufeld

We perform a detailed analysis of high-order harmonic generation in diatomic molecules within the strong-field approximation, with emphasis on quantum-interference effects. Specifically, we investigate how the different types of electron…

Atomic Physics · Physics 2011-11-10 C. Figueira de Morisson Faria

We report on calculations of harmonic generation by neon in a mixed (800-nm + time-delayed 400-nm) laser pulse scheme. In contrast with previous studies we employ a short (few-cycle) 400-nm pulse, finding that this affords control of the…

Atomic Physics · Physics 2017-01-20 K. R. Hamilton , H. W. van der Hart , A. C. Brown

We consider a quantum mechanical model for the high-order harmonic generation in bulk solids. The bandgap is assumed to be considerably larger than the exciting photon energy. Using dipole approximation, the dynamical equations for…

Quantum Physics · Physics 2017-11-09 Viktor Szaszkó-Bogár , Katalin Varjú , Péter Földi

The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…

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