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Here we report on a novel High Harmonic Generation (HHG) light source designed for space charge free ultrafast photoelectron spectroscopy (PES) on solids. The ultimate overall energy resolution achieved on a polycrystalline Au sample is ~22…

Angle-resolved photoemission spectroscopy (ARPES), an experimental technique based on the photoelectric effect, is arguably the most powerful method for probing the electronic structure of solids. The past decade has witnessed notable…

Materials Science · Physics 2021-06-21 Baiqing Lv , Tian Qian , Hong Ding

We use time- and angle-resolved photoemission spectroscopy (tr-ARPES) in the Extreme Ultraviolet (EUV) to measure the time- and momentum-dependent electronic structure of photo-excited K0.3MoO3. Prompt depletion of the Charge Density Wave…

The significant progress in angle-resolved photoemission spectroscopy (ARPES) in last three decades has elevated it from a traditional band mapping tool to a precise probe of many-body interactions and dynamics of quasiparticles in complex…

Superconductivity · Physics 2018-04-13 Xingjiang Zhou , Shaolong He , Guodong Liu , Lin Zhao , Li Yu , Wentao Zhang

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

Ultrafast spectroscopies have become an important tool for elucidating the microscopic description and dynamical properties of quantum materials. In particular, by tracking the dynamics of non-thermal electrons, a material's dominant…

Angle-resolved photoelectron spectroscopy (ARPES) is the main experimental tool to explore electronic structure of solids resolved in the electron momentum k . Soft-X-ray ARPES (SX-ARPES), operating in a photon energy range around 1 keV,…

The high-order harmonic generation (HHG), if phase matched, opens a unique way to produce coherent ultrafast extreme-UV (XUV) or soft x-ray light sources. Here we describe a robust and tunable method for scaling and narrowing the bandwidth…

Optics · Physics 2017-10-03 L. Mashhadi , G. Shayeganrad

Time-resolved photoelectron spectroscopy (trPES) can directly detect transient electronic structure, thus bringing out its promising potential to clarify nonequilibrium processes arising in condensed matters. Here we report the result of…

Strongly Correlated Electrons · Physics 2015-05-20 K. Ishizaka , T. Kiss , T. Yamamoto , Y. Ishida , T. Saitoh , M. Matsunami , R. Eguchi , T. Ohtsuki , A. Kosuge , T. Kanai , M. Nohara , H. Takagi , S. Watanabe , S. Shin

Angle-resolved photoemission spectroscopy (ARPES) is a technique used to map the occupied electronic structure of solids. Recent progress in X-ray focusing optics has led to the development of ARPES into a microscopic tool, permitting the…

Time- and angle-resolved photoemission spectroscopy (trARPES) is a powerful spectroscopic method to measure the ultrafast electron dynamics directly in momentum-space. However, band gap materials with exceptional strong Coulomb interaction…

Mesoscale and Nanoscale Physics · Physics 2019-12-09 Dominik Christiansen , Malte Selig , Ermin Malic , Ralph Ernstorfer , Andreas Knorr

A versatile method for angle-resolved photoemission spectra (ARPES) calculations is reported within the one-step model of photoemission. The initial states are obtained from a repeated-slab calculation using the projector-augmented wave…

Materials Science · Physics 2024-02-28 Misa Nozaki , Peter Krüger

We describe a setup for time- and angle-resolved photoemission spectroscopy with wavelength-tunable excitation and extreme ultraviolet probe. It is enabled by using the 10 kHz twin Ti:sapphire amplifiers seeded by the common Ti:sapphire…

Materials Science · Physics 2025-02-11 Takeshi Suzuki , Yigui Zhong , Kecheng Liu , Teruto Kanai , Jiro Itatani , Kozo Okazaki

The paper describes a time-resolved photoemission (TRPES) apparatus equipped with a Yb-doped fiber laser system delivering 1.2-eV pump and 5.9-eV probe pulses at the repetition rate of 95 MHz. Time and energy resolutions are 11.3 meV and…

Instrumentation and Detectors · Physics 2016-12-13 Y. Ishida , T. Otsu , A. Ozawa , K. Yaji , S. Tani , S. Shin , Y. Kobayashi

Time- and Angle-resolved photoelectron spectroscopy from surfaces can be used to record the dynamics of electrons and holes in condensed matter on ultrafast time scales. However, ultrafast photoemission experiments using extreme-ultraviolet…

The ongoing development of intense high-harmonic generation (HHG) sources has recently enabled highly nonlinear ionization of atoms by the absorption of at least 10 extreme-ultraviolet (XUV) photons within a single atom [Senfftleben…

Soft X-ray angle resolved photoemission spectroscopy (SX-ARPES) is one of the most powerful spectroscopic techniques to visualize the three-dimensional bulk electronic structure in reciprocal lattice space. Compared with ARPES employing…

Strongly Correlated Electrons · Physics 2026-03-05 Kohei Yamagami , Yuichi Yokoyama , Yuta Sumiya , Hayaru Shouno , Tetsuro Nakamura , Masaichiro Mizumaki

The lack of available table-top extreme ultraviolet (XUV) sources with high enough fluxes and coherence properties have limited the availability of nonlinear XUV and x-ray spectroscopies to free electron lasers (FEL). Here, we demonstrate…

In this article we review our angle- and time-resolved photoemission studies (ARPES and trARPES) on various ferropnictides.

Angle-resolved photoemission spectroscopy (ARPES) is one of the most direct methods of studying the electronic structure of solids. By measuring the kinetic energy and angular distribution of the electrons photoemitted from a sample…

Strongly Correlated Electrons · Physics 2009-11-10 Andrea Damascelli