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We study ionic liquids interacting with electrified interfaces. The ionic fluid is modeled as a Coulomb lattice gas. We compare the ionic density profiles calculated using a popular modified Poisson-Boltzmann equation with the explicit…

Soft Condensed Matter · Physics 2017-12-21 Matheus Girotto , Thiago Colla , Alexandre P. dos Santos , Yan Levin

Confinement can significantly alter fluid properties, offering potential for specific technological applications. However, achieving precise control over the structural complexity of confined fluids and soft matter remains challenging, as…

Soft Condensed Matter · Physics 2024-11-20 Fabio Leoni , Erdal C. Oğuz , Giancarlo Franzese

A model of mobile, charged ion channels in a fluid membrane is studied. The channels may switch between an open and a closed state according to a simple two-state kinetics with constant rates. The effective electrophoretic charge and the…

Soft Condensed Matter · Physics 2009-11-07 Stephan C. Kramer , Reiner Kree

The sliding motion of aqueous droplets on hydrohobic surfaces leads to charge separation at the trailing edge, with implications from triple-line friction to hydrovoltaic energy generation. Charges deposited on the solid surface have been…

Soft Condensed Matter · Physics 2025-09-12 Zouhir Benrahla , Tristan Saide , Louis Burnaz , Emilie Verneuil , Simon Gravelle , Jean Comtet

Highly energetic ions traversing a two-dimensional material such as graphene produce strong electronic excitations. Electrons excited to energy states above the work function can give rise to secondary electron emission, reducing the amount…

We present a theoretical model and experimental demonstration of thin liquid film deformations due to a dielectric force distribution established by surface electrodes. We model the spatial electric field produced by a pair of parallel…

Soft Condensed Matter · Physics 2023-06-22 Israel Gabay , Federico Paratore , Evgeniy Boyko , Antonio Ramos , Amir D. Gat , Moran Bercovici

Transmembrane ion flow through channel proteins undergoing density fluctuations may cause lateral gradients of the electrical potential across the membrane giving rise to electrophoresis of charged channels. A model for the dynamics of the…

Pattern Formation and Solitons · Physics 2009-11-11 Markus Hilt , Walter Zimmermann

There is a long-standing question about the molecular configuration of interfacial water molecules in the proximity of solid surfaces, particularly carbon atoms which play a crucial role in electrochemistry and biology. In this study, the…

Statistical Mechanics · Physics 2021-03-03 Iman Ahmadabadi , Ali Esfandiar , Ali Hassanali , Mohammad Reza Ejtehadi

Inhomogeneity of ion correlation widely exists in many physicochemical, soft matter, and biological systems. Here, we apply the modified Gaussian renormalized fluctuation theory to study the classic example of the vapor-liquid interface of…

Soft Condensed Matter · Physics 2022-11-22 Nikhil R. Agrawal , Rui Wang

Liquid-based bio-applications of graphene require a quantitative understanding of the graphene-liquid interface, with the surface charge density of adsorbed ions, the interfacial charge transfer resistance, and the interfacial charge noise…

Mesoscale and Nanoscale Physics · Physics 2017-08-31 Jinglei Ping , A. T. Charlie Johnson

Water mediates electrostatic interactions via the orientation of its dipoles around ions, molecules, and interfaces. This induced water polarization consequently influences multiple phenomena. In particular, water polarization modulated by…

We investigate electrode geometries required to produce periodic 2-dimensional ion-trap arrays with the ions placed between two planes of electrodes. We present a generalization of previous methods for traps containing a single electrode…

Quantum Physics · Physics 2015-09-29 F. N. Krauth , J. Alonso , J. P. Home

Strain-inducing deformations in graphene alter charge distributions and provide a new method to design specific features in the band structure and transport properties. Novel approaches implement engineered substrates to induce specifically…

Mesoscale and Nanoscale Physics · Physics 2021-01-04 Md Tareq Mahmud , Nancy Sandler

Using molecular dynamics simulations with recently developed importance sampling methods, we show that the differential capacitance of a model ionic liquid based double-layer capacitor exhibits an anomalous dependence on the applied…

It is known that ion-irradiation can lead surfaces to spontaneously develop patterns with characteristic length scales on the order of only a few nanometers. Pattern formation typically occurs only for irradiation angles beyond a critical…

Materials Science · Physics 2025-05-13 Tyler P. Evans , Scott A. Norris

Crystallographic defects play a key role in determining the properties of crystalline materials. The new class of two-dimensional materials, foremost graphene, have enabled atomically resolved studies of defects, such as vacancies, grain…

Materials Science · Physics 2015-06-22 Ossi Lehtinen , Nilesh Vats , Gerardo Algara-Siller , Pia Knyrim , Ute Kaiser

The confinement of an ionic liquid between charged solid surfaces is treated using an exactly solvable 1D Coulomb gas model. The theory highlights the importance of two dimensionless parameters: the fugacity of the ionic liquid, and the…

Soft Condensed Matter · Physics 2014-09-08 Alpha A Lee , Dominic Vella , Susan Perkin , Alain Goriely

Graphite is a ubiquitous electrode material with particular promise for use in e.g., energy storage and desalination devices, but very little is known about the properties of the graphite-electrolyte double layer at technologically relevant…

Materials Science · Physics 2021-09-03 Aaron R. Finney , Ian J. McPherson , Patrick R. Unwin , Matteo Salvalaglio

Understanding the interactions of ambient molecules with graphene and adjacent dielectrics is of fundamental importance for a range of graphene-based devices, particularly sensors, where such interactions could influence the operation of…

Mesoscale and Nanoscale Physics · Physics 2015-11-30 Eric J. Olson , Rui Ma , Tao Sun , Mona A. Ebrish , Nazila Haratipour , Kyoungmin Min , Narayana R. Aluru , Steven J. Koester

The recent discovery of graphene has sparked significant interest, which has so far been focused on the peculiar electronic structure of this material, in which charge carriers mimic massless relativistic particle. However, the structure of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Jannik C. Meyer , A. K. Geim , M. I. Katsnelson , K. S. Novoselov , T. J. Booth , S. Roth