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Higher-order optical harmonics entered the realm of nanostructured solids being observed recently in optical gratings and metasurfaces with a subwavelength thickness. Structuring materials at the subwavelength scale allows for resonant…

We study intraband high-harmonic generation (HHG) in a crystal driven by quantum light. Previous theoretical studies have developed a framework based on coherent state expansions in terms of P distributions to consider nonclassical driving…

Quantum Physics · Physics 2026-05-08 Rasmus Vesterager Gothelf , Christian Saugbjerg Lange , Lars Bojer Madsen

The ongoing development of intense high-harmonic generation (HHG) sources has recently enabled highly nonlinear ionization of atoms by the absorption of at least 10 extreme-ultraviolet (XUV) photons within a single atom [Senfftleben…

The majority of sources of coherent optical radiation rely on laser oscillators driven by population inversion. Despite their technological importance in communications, medicine, industry, and other fields, it remains a challenge to access…

Optics · Physics 2021-10-22 Lamia Ateshian , Hyeongrak Choi , Mikkel Heuck , Dirk Englund

Plasmonic metasurfaces have emerged as a promising platform for enhancing a range of nonlinear optical processes, offering compact geometry and flexibility in light manipulation. Second order nonlinear processes, like second harmonic…

High harmonic generation traditionally combines ~100 near-infrared laser photons, to generate bright, phase matched, extreme ultraviolet beams when the emission from many atoms adds constructively. Here we show that by guiding a…

An analytic description of high harmonic generation (HHG) in solids induced by intense low-frequency pulses is presented within an adiabatic approach, which treats laser-matter interactions nonperturbatively. We derive the analytical…

Optics · Physics 2026-01-01 A. V. Flegel , Liang-Wen Pi , M. V. Frolov

Attosecond metrology sensitive to sub-optical-cycle electronic and structural dynamics is opening up new avenues for ultrafast spectroscopy of condensed matter. Using intense lightwaves to precisely control the extremely fast carrier…

We report strong third-harmonic generation (THG) in monolayer graphene grown by chemical vapor deposition (CVD) and transferred to an amorphous silica (glass) substrate; the photon energy is in three-photon resonance with the…

Mesoscale and Nanoscale Physics · Physics 2013-06-12 Sung-Young Hong , Jerry I. Dadap , Nicholas Petrone , Po-Chun Yeh , James Hone , Richard M. Osgood

High-order harmonic generation (HHG) arising from the non-perturbative interaction of intense light fields with matter constitutes a well-established tabletop source of coherent extreme-ultraviolet and soft X-ray radiation, which is…

Second harmonic generation (SHG), as one of the most significant \c{hi}(2) nonlinear optical processes, plays crucial roles in a broad variety of optical and photonic applications. Designing various delicate schemes to achieve highly…

Optics · Physics 2021-09-01 Lei Wang , XiuQuan Zhang , Feng Chen

Attosecond pulse trains (APTs) are indispensable for probing electron dynamics at their intrinsic timescales. High harmonic generation (HHG) has long been a successful and widely used technique in producing extreme ultraviolet APTs. While…

Accelerator Physics · Physics 2025-10-16 Lanpeng Ni , Junhao Liu , Zheng Qi , Chao Feng

Harmonic generation in the limit of ultra-steep density gradients is studied experimentally. Observations demonstrate that while the efficient generation of high order harmonics from relativistic surfaces requires steep plasma density…

We report on continuous high-harmonic generation at 1 kHz repetition rate from a liquid-sheet plasma mirror driven by relativistic-intensity near-single-cycle light transients. Through precise control of both the surface plasma density…

We theoretically investigate high-harmonic generation (HHG) in honeycomb-lattice graphene models when subjected to a DC electric field. By integrating the quantum master equation with the Boltzmann equation, we develop a numerical method to…

Mesoscale and Nanoscale Physics · Physics 2024-07-16 Minoru Kanega , Masahiro Sato

The ability to perform attosecond-pump attosecond-probe spectroscopy (APAPS) is a longstanding goal in ultrafast science. While first pioneering experiments demonstrated the feasibility of APAPS, the low repetition rates (10-120 Hz) and the…

A three step model for high harmonic generation from impurities in solids is developed. The process is found to be similar to high harmonic generation in atomic and molecular gases with the main difference coming from the non-parabolic…

Atomic Physics · Physics 2018-10-31 S. Almalki , A. Parks , G. Bart , P. B. Corkum , T. Brabec , C. R. McDonald

Thermotropic liquid crystals are versatile optical materials that exhibit a state of matter intermediate between liquids and solids. Their properties can change significantly with temperature, pressure, or other external factors, leading to…

Bright squeezed light from parametric down-conversion in the infrared (IR) frequency range has triggered the emergence of attosecond quantum optics -- a new research field at the interface of quantum optics, strong-field physics, and…

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

Atomic Physics · Physics 2015-10-15 Christian Buth
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