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Accurate \textit{ab initio} calculations on the rotation-vibration spectrum of methyl fluoride (\ce{CH3F}) are reported. A new nine-dimensional potential energy surface (PES) and dipole moment surface (DMS) have been generated using…

Chemical Physics · Physics 2018-08-16 Alec Owens , Andrey Yachmenev , Jochen Küpper , Sergei N. Yurchenko , Walter Thiel

Accurate potential energy surfaces (PESs) have been determined for the $^3$A$'$ and $^3$A$''$ states of N$_2$O using electronic structure calculations at the multireference configuration interaction level with Davidson correction (MRCI+Q)…

Chemical Physics · Physics 2020-11-06 Debasish Koner , Juan Carlos San Vicente Veliz , Raymond J. Bemish , Markus Meuwly

Optimal set of 1050 rovibronic energy levels for 35 triplet electronic states of $D_2$ has been obtained by means of a statistical analysis of all available wavenumbers of triplet-triplet rovibronic transitions studied in emission,…

Optics · Physics 2009-11-13 B. P. Lavrov , I. S. Umrikhin

Collisional (de-)excitation of H$_{2}$ by helium plays an important role in the thermal balance and chemistry of various astrophysical environments, making accurate rate coefficients essential for the interpretation of observations of the…

Astrophysics of Galaxies · Physics 2024-05-15 Hubert Jóźwiak , Franck Thibault , Alexandra Viel , Piotr Wcisło , François Lique

The interaction potential energy surface (PES) of He-H2 is of great importance for quantum chemistry, as the simplest test case for interactions between a molecule and a closed-shell atom. It is also required for a detailed understanding of…

Astrophysics · Physics 2009-11-07 Arnold I. Boothroyd , Peter G. Martin , Michael R. Peterson

Accurate rotational-vibrational line lists for $^{31}$P$^{14}$N and $^{31}$P$^{15}$N in their ground electronic states are computed. The line lists are produced using an empirical potential energy curve obtained by fitting to the…

Astrophysics of Galaxies · Physics 2015-04-14 Leo Yorke , Sergei N. Yurchenko , Lorenzo Lodi , Jonathan Tennyson

An optimal set of 1050 rovibronic energy levels for 35 triplet electronic states of $D_2$ has been obtained by means of a statistical analysis of all available wavenumbers of triplet-triplet rovibronic transitions studied in emission,…

Optics · Physics 2008-02-08 B. P. Lavrov , I. S. Umrikhin

A rovibronic line list for the ground ($X$ $^3\Sigma^-$) and first excited ($a$ $^1\Delta$) states of phosphinidene, $^{31}$PH, is computed. The line list is designed for studies of exoplanetary and cool stellar atmospheres with…

Earth and Planetary Astrophysics · Physics 2019-07-17 Jonathan Langleben , Jonathan Tennyson , Sergei N. Yurchenko , Peter Bernath

An analysis of the measured rovibrational transitions is carried out for the 12C32S2 isotopologue of carbon disulfide. Data from 21 sources is extracted and validated using a consistent set of standard linear molecule quantum numbers. A…

Atomic Physics · Physics 2025-02-28 Tanvi Sattiraju , Jonathan Tennyson

Calculation of the rotation-vibration spectrum of H3+, as well as of its deuterated isotopologues, with near-spectroscopic accuracy requires the development of sophisticated theoretical models, methods, and codes. The present paper reviews…

A new line list for H$_2$$^{16}$O is presented. This line list, which is called POKAZATEL, includes transitions between rotation-vibrational energy levels up to 41000 cm$^{-1}$ in energy and is the most complete to date. The potential…

Earth and Planetary Astrophysics · Physics 2018-08-21 Oleg L. Polyansky , Aleksandra A. Kyuberis , Nikolai F. Zobov , Jonathan Tennyson , Sergei N. Yurchenko , Lorenzo Lodi

We present 'BYTe', a comprehensive 'hot' line list for the ro-vibrational transitions of ammonia, 14NH3, in its ground electronic state. This line list has been computed variationally using the program suite TROVE, a new…

Earth and Planetary Astrophysics · Physics 2017-07-03 S. N. Yurchenko , R. J. Barber , J. Tennyson

A module of the ATLAS electromagnetic barrel liquid argon calorimeter was exposed to the CERN electron test-beam at the H8 beam line upgraded for precision momentum measurement. The available energies of the electron beam ranged from 10 to…

Instrumentation and Detectors · Physics 2008-11-26 M. Aharrouche , ATLAS Electromagnetic Barrel Calorimeter Collaboration

New ab initio potential energy surfaces for the doublet pi ground electronic state of the Ar-SH complex are presented, calculated at the RCCSD(T)/aug-cc-pV5Z level. Weakly bound rotation-vibration levels are calculated using coupled-channel…

Chemical Physics · Physics 2007-05-23 Richard J. Doyle , David M. Hirst , Jeremy M. Hutson

A potential energy curve (PEC) accurate to a fraction of 1 ppm ($1:10^6$) is computed for the $^3\Sigma_\mathrm{u}^+$ state of He$_2$ endowed with relativistic and QED corrections. The nuclear Schr\"odinger equation is solved on this PEC…

Chemical Physics · Physics 2026-02-25 Ádám Margócsy , Balázs Rácsai , Péter Jeszenszki , Edit Mátyus

Energies and lifetimes are reported for the lowest 136 levels of Fe XIV, belonging to the (1s$^2$2s$^2$2p$^6$) 3s$^2$3p, 3s3p$^2$, 3s$^2$3d, 3p$^3$, 3s3p3d, 3p$^2$3d, 3s3d$^2$, 3p3d$^2$ and 3s$^24\ell$ configurations. Additionally,…

Solar and Stellar Astrophysics · Physics 2015-06-22 K M Aggarwal , F P Keenan

We show that chemically-accurate potential energy surfaces (PESs) can be generated from quantum computers by measuring only the density along an adiabatic transition between different molecular geometries. In lieu of using phase estimation,…

Quantum Physics · Physics 2024-10-08 James Brown

We report a set of adiabatic potential energy surfaces (PESs) for diiodomethane, including the ground electronic state and all excited states accessible via single-photon absorption near 260 nm. Although constrained to four dimensions,…

Chemical Physics · Physics 2026-02-26 Yijue Ding

Energies for the lowest 56 levels, belonging to the 3s$^2$3p, 3s3p$^2$, 3p$^3$, 3s$^2$3d, 3s3p3d, 3s$^2$4$\ell$ and 3s$^2$5$\ell$ configurations of Si II, are calculated using the {\sc grasp} (General-purpose Relativistic Atomic Structure…

Instrumentation and Methods for Astrophysics · Physics 2015-06-19 KM Aggarwal , FP Keenan

Constructing accurate, high dimensional molecular potential energy surfaces (PESs) for polyatomic molecules is challenging. Reproducing Kernel Hilbert space (RKHS) interpolation is an efficient way to construct such PESs. However, the…

Chemical Physics · Physics 2020-11-06 Debasish Koner , Markus Meuwly