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X-ray Thomson scattering (XRTS) has emerged as a widely used diagnostics for extreme states of matter in a great variety of situations, and over a broad range of parameters. The standard approach for the interpretation of XRTS measurements…

Plasma Physics · Physics 2026-04-29 Thomas Gawne , Jan Vorberger , Zhandos Moldabekov , Hannah Bellenbaum , Tobias Dornheim

Quasi-one-dimensional systems exhibit many-body effects elusive in higher dimensions. A prime example is spin-orbital separation, which has been measured by resonant inelastic X-ray scattering (RIXS) in Sr$_2$CuO$_3$. Here, we theoretically…

Strongly Correlated Electrons · Physics 2022-10-03 Aaron Müller , Francesco Grandi , Martin Eckstein

The paper describes a new concept of visible pump/X-ray probe/slow detector experiments that could be performed at third-generation synchrotron light sources. We propose a technique that would allow time resolution up to femtosecond…

Instrumentation and Detectors · Physics 2009-11-07 E. L. Saldin , E. A. Schneidmiller , M. V. Yurkov

Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…

Instrumentation and Detectors · Physics 2020-05-06 Yanwen Sun , Mike Dunne , Paul Fuoss , Taito Osaka , Aymeric Robert , Mark Sutton , Makina Yabashi , Diling Zhu

We present two different theories for Raman scattering and Resonant Inelastic X-ray Scattering (RIXS) in the low temperature ferromagnetic phase of YTiO$_3$ and compare this to the available experimental data. For description of the orbital…

Strongly Correlated Electrons · Physics 2010-03-30 L. J. P. Ament , G. Khaliullin

We examine x-ray scattering from an isolated organic molecule from the linear to nonlinear absorptiveregime. In the nonlinear regime, we explore the importance of both the elastic and inelastic channelsand observe the onset of nonlinear…

Chemical Physics · Physics 2021-06-09 Phay J. Ho , Adam E. A. Fouda , Kai Li , Gilles Doumy , Linda Young

Motivated by recent experimental progress we revisit the theory of pump-probe time- and angle-resolved photoemission spectroscopy (trARPES), which is one of the most powerful techniques to trace transient pump-driven modifications of the…

Mesoscale and Nanoscale Physics · Physics 2022-01-14 Michael Schüler , Michael A. Sentef

Ultrafast time-resolved x-ray scattering is an emerging approach to image the dynamical evolution of the electronic charge distribution during complex chemical and biological processes in real-space and real-time. Recently, the differences…

Atomic Physics · Physics 2015-06-15 Gopal Dixit , Robin Santra

We develop a phenomenological theory to predict the characteristic features of the momentum-dependent scattering amplitude in resonant inelastic x-ray scattering (RIXS) at the energy scale of the superconducting gap in iron-based…

Superconductivity · Physics 2016-05-10 Pasquale Marra , Jeroen van den Brink , Steffen Sykora

The real-space multiple-scattering (RSMS) approach is applied to model non-resonant inelastic scattering from deep core electron levels over a broad energy spectrum. This approach is applicable to aperiodic or periodic systems alike and…

Other Condensed Matter · Physics 2009-11-11 J. A. Soininen , A. L. Ankudinov , J. J. Rehr

Resonant inelastic x-ray scattering (RIXS) has become a powerful tool in the study of the electronic structure of condensed matter. Although the linewidths of many RIXS features are narrow, the experimental broadening can often hamper the…

Strongly Correlated Electrons · Physics 2012-02-13 J. Laverock , A. R. H. Preston , D. Newby , K. E. Smith , S. B. Dugdale

We describe how improvements in methodology and instrumentation for meV-resolved inelastic x-ray scattering (IXS), coupled with a fresh examination of older theory, allow identification of interaction between the quasi-elastic and acoustic…

Soft Condensed Matter · Physics 2022-05-18 Alfred Q. R. Baron , Daisuke Ishikawa

Coherent excitation of materials via ultrafast laser pulses can have interesting, observable dynamics in time-resolved photoemission measurements. The broad spectral width of ultrafast pump pulses can coherently excite multiple exciton…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Avinash Rustagi , Alexander F. Kemper

Time-resolved X-ray scattering patterns from photoexcited molecules in solution are in many cases anisotropic at the ultrafast time scales accessible at X-ray Free Electron Lasers (XFELs). This anisotropy arises from the interaction of a…

We present a theoretical investigation of the origin of Raman-like and fluorescencelike (FL) features of resonant inelastic x-ray scattering (RIXS) spectra. Using a combination of local-density approximation + dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2018-09-26 Atsushi Hariki , Mathias Winder , Jan Kuneš

We describe here an experimental technique based on the acoustic scattering phenomenon allowing the direct probing of the vorticity field in a turbulent flow. Using time-frequency distributions, recently introduced in signal analysis…

chao-dyn · Physics 2009-10-31 Christophe Baudet , Olivier Michel , William J. Williams

We present a theoretical study of temporal, spectral, and spatial reshaping of intense, ultrafast x-ray pulses propagating through a resonant medium. Our calculations are based on the solution of a 3D time-dependent Schr\"odinger-Maxwell…

Atomic Physics · Physics 2020-12-30 Kai Li , Marie Labeye , Phay J. Ho , Mette B. Gaarde , Linda Young

Resonant inelastic X-ray scattering (RIXS) spectra of model copper- and nickel-based transition metal oxides are measured over a wide range of energies near the M-edge (h$\nu$=60-80eV) to better understand the properties of resonant…

Strongly Correlated Electrons · Physics 2012-11-20 L. Andrew Wray , Wanli Yang , Hiroshi Eisaki , Zahid Hussain , Yi-De Chuang

We use Time Resolved Correlation (TRC), a recently introduced light scattering method, to study the dynamics of a variety of jammed, or glassy, soft materials. The output of a TRC experiment is cI(t,tau), the time series of the degree of…

Soft Condensed Matter · Physics 2009-11-10 Agnes Duri , Pierre Ballesta , Luca Cipelletti , Hugo Bissig , Veronique Trappe

Understanding the excitations of quantum materials is essential for unraveling how their microscopic constituents interact. Among these, particle-hole excitations form a particularly important class, as they govern fundamental processes…

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