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We present a general model study of surface-enhanced resonant Raman scattering and fluorescence, focusing on the interplay between electromagnetic (EM) effects and the molecular dynamics as treated by a density matrix calculation. The model…

Other Condensed Matter · Physics 2007-05-23 Peter Johansson , Hongxing Xu , Mikael Käll , ;

Stimulated Raman scattering, employing a pump and a Stokes beam, exhibits itself through both the Raman loss observed in the pump beam and the Raman gain in the Stokes beam. This phenomenon finds application in spectroscopy for chemical…

Optics · Physics 2024-08-13 Minhaeng Cho

We theoretically propose a method to enhance Raman scattering by injecting a seeded light field which is correlated with the initially prepared atomic spin wave. Such a light-atom correlation leads to an interference in the Raman…

Quantum Physics · Physics 2013-05-29 Chun-Hua Yuan , L. Q. Chen , Z. Y. Ou , Weiping Zhang

We theoretically analyze and experimentally demonstrate the possibility of amplifying optical signals in an unrepeatered mode-division multiplexed tranmsmission system, through inter-modal stimulated Raman scattering process between signal…

In a recent report sum-frequency excitation of a Raman-active phonon was experimentally demonstrated for the first time. This mechanism is the sibling of impulsive stimulated Raman scattering, in which difference-frequency components of a…

Materials Science · Physics 2018-05-23 Dominik M. Juraschek , Sebastian F. Maehrlein

Stimulated Raman scattering of a laser pump pulse seeded by a Stokes pulse generically leaves a two-level medium initially at rest in an excited state constituted of static solitons and radiation. The soliton birth manifests as sudden very…

solv-int · Physics 2016-09-08 J. Leon , A. V. Mikhailov

We study Raman scattering in active media placed in proximity of different types of metal nanostructures, at wavelengths that display either Fabry-Perot or plasmonic resonances, or a combination of both. We use a semi-classical approach to…

Optics · Physics 2015-06-05 M. Scalora , M. A. Vincenti , D. de Ceglia , M. Grande , J. W. Haus

We report the observations of spontaneous Raman scattering in silicon photonic crystal waveguides. Continuous-wave measurements of Stokes emission for both wavelength and power dependence is reported in single line-defect waveguides in…

Optics · Physics 2009-11-13 J. F. McMillan , M. Yu , D. L. Kwong , C. W. Wong

Frequency up-conversion, enabled by molecular optomechanical coupling, has recently emerged as a promising approach for converting infrared signals into the visible range through quantum coherent conversion of signals. However, detecting…

Quantum Physics · Physics 2024-04-17 Fen Zou , Lei Du , Yong Li , Hui Dong

Stimulated Raman scattering (SRS) represents a powerful tool for accessing the vibrational properties of molecular compounds or solid state systems. From a spectroscopic perspective, SRS is able to capture Raman spectra free from incoherent…

We investigate for the first time the enhancement of the stimulated Raman scattering in slow-light Silicon-on-Insulator (SOI) photonic crystal line defect waveguides. By applying the Bloch-Floquet formalism to the guided modes in a planar…

Optics · Physics 2010-04-12 J. F. McMillan , X. Yang , N. C. Panoiu , R. M. Osgood , C. W. Wong

The physical processes associated with propagation of a high-power (power > critical power for self-focusing) laser beam in water include nonlinear focusing, stimulated Raman scattering (SRS), optical breakdown and plasma formation. The…

We propose an optical method for increasing the number of atoms in a pair of dilute gas Bose-Einstein condensates. The method uses laser-driven Raman transitions which scatter atoms between the condensate and non-condensate atom fractions.…

Statistical Mechanics · Physics 2011-07-04 C. M. Savage , Janne Ruostekoski , Dan F. Walls

We present a general model study of surface-enhanced resonant Raman scattering and fluorescence focusing on the interplay between electromagnetic effects and the molecular dynamics. Our model molecule is placed close to two Ag…

Other Condensed Matter · Physics 2007-05-23 Hongxing Xu , Xue-Hua Wang , Martin P. Persson , H. Q. Xu , Mikael Kall , Peter Johansson

An internal field induced resonant intensity enhancement of Raman scattering of phonon excitations in InAs nanowires is reported. The experimental observation is in good agreement with the simulated results for the scattering of light under…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Jaya Kumar Panda , Anushree Roy , Achintya Singha , Mauro Gemmi , Daniele Ercolani , Vittorio Pellegrini , Lucia Sorba

Enhancement of optical response with high-index dielectric nanoparticles is attributed to the excitation of their Mie-type magnetic and electric resonances. Here we study Raman scattering from crystalline silicon nanoparticles and reveal…

High-gain resonant nonlinear Raman scattering on trapped cold atoms within a high-fineness ring optical cavity is simply explained under a nonlinear opto-mechanical mechanism, and a proposal using it to detect frequency of micro-trap on…

Atomic Physics · Physics 2014-03-24 Lin Zhang

We present a method for deriving limits on Raman scattering in structured media and exploit it to constrain the maximum Raman signal resulting from a planewave incident on either a single Raman molecule in the vicinity of a structured…

We present a quantum-mechanical model that describes fiber-based frequency conversion by four-wave-mixing Bragg scattering in the presence of Raman interactions. In the case of continuous-wave pumps we find closed-form expressions for the…

Quantum Physics · Physics 2024-06-06 Mathias Linde Holst Korsgaard , Jacob Gade Koefoed , Karsten Rottwitt

We present a self-consistent quantum optics approach to calculating the surface enhanced Raman spectrum of molecules coupled to arbitrarily shaped plasmonic systems. Our treatment is intuitive to use and provides fresh analytical insight…

Optics · Physics 2017-06-26 Mohsen Kamandar Dezfouli , Stephen Hughes
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