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Related papers: Gate tunable dark trions in monolayer WSe$_2$

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Spin-forbidden intravalley dark exciton in tungsten-based transition metal dichalcogenides (TMDCs), owing to its unique spin texture and long lifetime, has attracted intense research interest. Here, we show that we can control the dark…

Charged excitons, or X$^{\pm}$-trions, in monolayer transition metal dichalcogenides have binding energies of several tens of meV. Together with the neutral exciton X$^0$ they dominate the emission spectrum at low and elevated temperatures.…

Optically dark excitonic states play a critical role in the valleytronic, electronic, and optical properties of monolayer semiconducting transition metal dichalcogenides. Here, we investigate how electrostatic doping affects the in-plane…

We have successfully confined trions into a one-dimensional restricted space of a MoSe2 device with CNT gate electrodes. The dry transfer process, including deterministic dry transfer of aligned CNTs, has led to an hBN-encapsulated MoSe2…

Mesoscale and Nanoscale Physics · Physics 2022-12-28 Takato Hotta , Haruna Nakajima , Shohei Chiashi , Taiki Inoue , Shigeo Maruyama , Kenji Watanabe , Takashi Taniguchi , Ryo Kitaura

We perform absorption and photoluminescence spectroscopy of trions in hBN-encapsulated WSe$_2$, WS$_2$, MoSe$_2$, and MoS$_2$ monolayers, depending on temperature. The different trends for W- and Mo-based materials are excellently…

Electrical control of individual spins and photons in solids is key for quantum technologies, but scaling down to small, static systems remains challenging. Here, we demonstrate nanoscale electrical tuning of neutral and charged excitons in…

Mesoscale and Nanoscale Physics · Physics 2023-11-01 Jawaher Almutlaq , Jiangtao Wang , Linsen Li , Chao Li , Tong Dang , Vladimir Bulović , Jing Kong , Dirk Englund

The optical emission spectra of semiconducting transition-metal dichalcogenide monolayers highlight fascinating recombination processes of charged excitons (trions). When charge tunable WSe$_2$ monolayers are moderately doped with…

Mesoscale and Nanoscale Physics · Physics 2025-01-22 V. Jindal , K. Mourzidis , A. Balocchi , C. Robert , P. Li , D. Van Tuan , L. Lombez , D. Lagarde , P. Renucci , T. Taniguchi , K. Watanabe , H. Dery , X. Marie

Monolayers of semiconducting transition metal dichalcogenides are two-dimensional direct-gap systems which host tightly-bound excitons with an internal degree of freedom corresponding to the valley of the constituting carriers. Strong…

Low temperature and polarization resolved magneto-photoluminescence experiments are used to investigate the properties of dark excitons and dark trions in a monolayer of WS$_2$ encapsulated in hexagonal BN (hBN). We find that this system is…

Embedding a WS$_2$ monolayer in flakes of hexagonal boron nitride allowed us to resolve and study the photoluminescence response due to both singlet and triplet states of negatively charged excitons (trions) in this atomically thin…

Mesoscale and Nanoscale Physics · Physics 2018-06-08 D. Vaclavkova , J. Wyzula , K. Nogajewski , M. Bartos , A. O. Slobodeniuk , C. Faugeras , M. Potemski , M. R. Molas

The direct band gap character and large spin-orbit splitting of the valence band edges (at the K and K' valleys) in monolayer transition metal dichalcogenides have put these two-dimensional materials under the spot-light of intense…

Mesoscale and Nanoscale Physics · Physics 2017-04-10 Mark Danovich , Viktor Zólyomi , Vladimir I. Fal'ko

We demonstrate long trion spin lifetimes in a WSe$_2$ monolayer of up to 150 ns at 5 K. Applying a transverse magnetic field in time-resolved Kerr-rotation measurements reveals a complex composition of the spin signal of up to four distinct…

Materials Science · Physics 2017-06-08 F. Volmer , S. Pissinger , M. Ersfeld , S. Kuhlen , C. Stampfer , B. Beschoten

Monolayer transition metal dichalcogenides (TMDs) hold great promise for future information processing applications utilizing a combination of electron spin and valley pseudospin. This unique spin system has led to observation of the valley…

Mesoscale and Nanoscale Physics · Physics 2019-05-30 T. P. Lyons , S. Dufferwiel , M. Brooks , F. Withers , T. Taniguchi , K. Watanabe , K. S. Novoselov , G. Burkard , A. I. Tartakovskii

We present experimental and theoretical results on the high-quality single-layer MoS$_{2}$ which reveal the fine structure of charged excitons, i.e., trions. In the emission spectra we resolve and identify two trion peaks, T$_{1}$ and…

The intricate interplay between optically dark and bright excitons governs the light-matter interaction in transition metal dichalcogenide monolayers. We have performed a detailed investigation of the "spin-forbidden" dark excitons in WSe2…

Trions are excitonic species with a positive or negative charge, and thus, unlike neutral excitons, the flow of trions can generate a net detectable charge current. Trions under favourable doping conditions can be created in a coherent…

Applied Physics · Physics 2020-03-24 Sarthak Das , Sangeeth Kallatt , Nithin Abraham , Kausik Majumdar

Strong Coulomb interaction in monolayer transition metal dichalcogenides can facilitate nontrivial many-body effects among excitonic complexes. Many-body effects like exciton-exciton annihilation (EEA) have been widely explored in this…

Mesoscale and Nanoscale Physics · Physics 2022-04-05 Suman Chatterjee , Garima Gupta , Sarthak Das , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

Monolayer photonic materials offer a tremendous potential for on-chip optoelectronic devices. Their realization requires knowledge of optical coherence properties of excitons and trions that have so far been limited to nonlinear optical…

Mesoscale and Nanoscale Physics · Physics 2017-12-20 Gabriella D. Shepard , Jenny V. Ardelean , Daniel A. Rhodes , X. -Y. Zhu , James C. Hone , Stefan Strauf

Monolayer group VI transition metal dichalcogenides have recently emerged as semiconducting alternatives to graphene in which the true two-dimensionality (2D) is expected to illuminate new semiconducting physics. Here we investigate…

Mesoscale and Nanoscale Physics · Physics 2014-03-05 Jason S Ross , Sanfeng Wu , Hongyi Yu , Nirmal J Ghimire , Aaron M Jones , Grant Aivazian , Jiaqiang Yan , David G. Mandrus , Di Xiao , Wang Yao , Xiaodong Xu

The possibility of almost linear tuning of the band gap and of the electrical and optical properties in monolayers (MLs) of semiconducting transition metal dichalcogenide (S-TMD) alloys opens up the way to fabricate materials with on-demand…

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