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The Poisson-Boltzmann equation offers an efficient way to study electrostatics in molecular settings. Its numerical solution with the boundary element method is widely used, as the complicated molecular surface is accurately represented by…

Numerical Analysis · Mathematics 2021-08-25 Stefan D. Search , Christopher D. Cooper , Elwin van't Wout

We consider a class of nonlinear elliptic problems associated with models in biophysics, which are described by the Poisson-Boltzmann equation (PBE). We prove mathematical correctness of the problem, study a suitable class of…

Numerical Analysis · Mathematics 2020-12-15 Johannes Kraus , Svetoslav Nakov , Sergey Repin

We apply the Tensor Train (TT) approximation to construct the Polynomial Chaos Expansion (PCE) of a random field, and solve the stochastic elliptic diffusion PDE with the stochastic Galerkin discretization. We compare two strategies of the…

Numerical Analysis · Mathematics 2014-06-12 Sergey Dolgov , Boris N. Khoromskij , Alexander Litvinenko , Hermann G. Matthies

The polarizable embedding (PE) approach is a flexible embedding model where a pre-selected region out of a larger system is described quantum mechanically while the interaction with the surrounding environment is modeled through an…

Chemical Physics · Physics 2017-01-24 Erik D. Hedegård , Markus Reiher

Accurate calculation of electrostatic potential and gradient on the molecular surface is highly desirable for the continuum and hybrid modeling of large scale deformation of biomolecules in solvent. In this article a new numerical method is…

Computational Physics · Physics 2020-08-26 George Borleske , Y. C. Zhou

We propose a method that exploits sparse representation of potential energy surfaces (PES) on a polynomial basis set selected by compressed sensing. The method is useful for studies involving large numbers of PES evaluations, such as the…

Chemical Physics · Physics 2018-08-10 Prashant Rai , Khachik Sargsyan , Habib Najm , So Hirata

In this paper, we solve the linearized Poisson-Boltzmann equation, used to model the electric potential of macromolecules in a solvent. We derive a corrected trapezoidal rule with improved accuracy for a boundary integral formulation of the…

Numerical Analysis · Mathematics 2022-10-10 Federico Izzo , Yimin Zhong , Olof Runborg , Richard Tsai

Singular charge sources in terms of Dirac delta functions present a well-known numerical challenge for solving Poisson's equation. For a sharp interface between inhomogeneous media, singular charges could be analytically treated by…

Numerical Analysis · Mathematics 2019-10-02 Siwen Wang , Arum Lee , Emil Alexov , Shan Zhao

This paper presents a numerical method for variable coefficient elliptic PDEs with mostly smooth solutions on two dimensional domains. The PDE is discretized via a multi-domain spectral collocation method of high local order (order 30 and…

Numerical Analysis · Mathematics 2016-12-09 Tracy Babb , Adrianna Gillman , Sijia Hao , Per-Gunnar Martinsson

Consistency between the exchange-correlation (xc) functional used during pseudopotential construction and planewave-based electronic structure calculations is important for an accurate and reliable description of the structure and…

We present a novel numerical method for solving the elliptic partial differential equation problem for the electrostatic potential with piecewise constant conductivity. We employ an integral equation approach for which we derive a system of…

Numerical Analysis · Mathematics 2022-06-01 Kyle Bower , Kirill Serkh , Spyros Alexakis , Adam R Stinchcombe

Bootstrap embedding (BE) is a recently developed electronic structure method that has shown great success at treating electron correlation in molecules. Here, we extend BE to treat surfaces and solids where the wave function is represented…

Strongly Correlated Electrons · Physics 2023-01-18 Oinam Romesh Meitei , Troy Van Voorhis

The Poisson-Boltzmann equation is a widely used model to study the electrostatics in molecular solvation. Its numerical solution using a boundary integral formulation requires a mesh on the molecular surface only, yielding accurate…

Numerical Analysis · Mathematics 2020-09-25 Vicente Ramm , Jehanzeb H. Chaudhry , Christopher D. Cooper

The Poisson-Boltzmann (PB) model governs the electrostatics of solvated biomolecules, i.e., potential, field, energy, and force. These quantities can provide useful information about protein properties, functions, and dynamics. By…

Biomolecules · Quantitative Biology 2023-12-29 Xin Yang , Elyssa Sliheet , Reece Iriye , Daniel Reynolds , Weihua Geng

Poisson's equation has been used in VLSI global placement for describing the potential field caused by a given charge density distribution. Unlike previous global placement methods that solve Poisson's equation numerically, in this paper,…

Other Computer Science · Computer Science 2023-07-25 Wenxing Zhu , Zhipeng Huang , Jianli Chen , Yao-Wen Chang

The computational study of chemical reactions in complex, wet environments is critical for applications in many fields. It is often essential to study chemical reactions in the presence of applied electrochemical potentials, taking into…

Materials Science · Physics 2016-01-20 G. Fisicaro , L. Genovese , O. Andreussi , N. Marzari , S. Goedecker

We develop an accurate, highly efficient and scalable random batch Ewald (RBE) method to conduct simulations in the isothermal-isobaric ensemble (the NPT ensemble) for charged particles in a periodic box. After discretizing the Langevin…

Computational Physics · Physics 2022-10-19 Jiuyang Liang , Pan Tan , Liang Hong , Shi Jin , Zhenli Xu , Lei Li

Molecular dynamics simulations of biomolecules have been widely adopted in biomedical studies. As classical point-charge models continue to be used in routine biomolecular applications, there have been growing demands on developing…

Computational Physics · Physics 2020-10-28 Haixin Wei , Ruxi Qi , Junmei Wang , Piotr Cieplak , Yong Duan , Ray Luo

Constant potential molecular dynamics simulation plays important role for applications of electrochemical systems, yet the calculation of charge fluctuation on electrodes remains a computational bottleneck. We propose a highly scalable,…

Computational Physics · Physics 2025-09-30 Weihang Gao , Qi Zhou , Qianru Zhang , Zhenli Xu

We describe the numerical scheme for the discretization and solution of 2D elliptic equations with strongly varying piecewise constant coefficients arising in the stochastic homogenization of multiscale composite materials. An efficient…

Numerical Analysis · Mathematics 2019-04-01 Venera Khoromskaia , Boris N. Khoromskij , Felix Otto