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Exact calculated time evolutions in the framework of a many-electron model of itinerant magnetism provide new insights into the laser-induced ultrafast demagnetization observed in ferromagnetic (FM) transition metal thin films. The…

Strongly Correlated Electrons · Physics 2015-11-25 W. Töws , G. M. Pastor

Induced by an ultra-short laser pulse, the electronic structure of a material undergoes strong modifications leading to a fast demagnetization in magnetic materials. Induced spin-flip transitions are one of the reasons for demagnetization,…

Materials Science · Physics 2024-04-29 Sergiy Mankovsky , Svitlana Polesya , Hubert Ebert

We theoretically investigate the optically-induced demagnetization of ferromagnetic FePt using the time-dependent density functional theory (TDDFT). We compare the demagnetization mechanism in the perturbative and nonperturbative limits of…

Materials Science · Physics 2024-04-26 M. S. Mrudul , Peter M. Oppeneer

Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

Materials Science · Physics 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

Laser induced ultrafast demagnetization is the process whereby the magnetic moment of a ferromagnetic material is seen to drop significantly on a timescale of $10-100$s of femtoseconds due to the application of a strong laser pulse. If this…

Materials Science · Physics 2016-01-20 P. Elliott , K. Krieger , J. K. Dewhurst , S. Sharma , E. K. U. Gross

Ultrafast laser excitation of ferromagnetic metals gives rise to correlated, highly non-equilibrium dynamics of electrons, spins and lattice, which are, however, poorly described by the widely-used three-temperature model (3TM). Here, we…

Materials Science · Physics 2024-01-17 Markus Weißenhofer , Peter M. Oppeneer

Demagnetization in ferromagnetic transition metals driven by a femtosecond laser pulse is a fundamental problem in solid state physics, and its understanding is essential to the development of spintronics devices. Ab initio calculation of…

Materials Science · Physics 2024-01-02 Mitsuko Murakami , G. P. Zhang

Electronic excitations in a ferromagnet can trigger ultrafast spin dynamics with potential applications in a speed increase in magnetic recording. The project investigates ultrafast magnetization dynamics, which is driven in metallic layers…

Materials Science · Physics 2010-07-06 Adrian Glaubitz

Laser-induced ultrafast demagnetization is a phenomenon of utmost interest and attracts significant attention because it enables potential applications in ultrafast optoelectronics and spintronics. As a spin-orbit coupling assisted magnetic…

When a laser pulse excites a ferromagnet, its spin undergoes a dramatic change. The initial demagnetization process is very fast. Experimentally, it is found that the demagnetization time is related to the spin moment in the sample. In this…

Materials Science · Physics 2016-11-11 G. P. Zhang , M. S. Si , Thomas F. George

The microscopic origin of laser-induced ultrafast demagnetization remains an open question, to which the non-thermal electronic distribution plays a vital role at the initial stage. Herein, we investigate the connection between the…

Materials Science · Physics 2025-12-25 Yu-Hui Song , Huan-Cheng Yang , Kai Liu , Zhong-Yi Lu

New insights into the microscopic origin of itinerant ferromagnetism were recently gained from investigations of electronic lattice models within dynamical mean-field theory (DMFT). In particular, it is now established that even in the…

Strongly Correlated Electrons · Physics 2007-05-23 D. Vollhardt , N. Blümer , K. Held , M. Kollar

Irradiating a ferromagnetic material with an ultrashort laser pulse leads to demagnetization on a femtosecond timescale. We implement Elliott-Yafet type spin-flip scattering, mediated by electron-electron and electron-phonon collisions,…

Materials Science · Physics 2011-08-29 Benedikt Y. Mueller , T. Roth , M. Cinchetti , M. Aeschlimann , B. Rethfeld

The ultrafast and element-specific response of magnetic systems containing ferromagnetic 3d transition metals and 4d/5d heavy metals is of interest both from a fundamental as well as an applied research perspective. However, to date no…

In the last few decades, ultrafast demagnetization elicited by ultrashort laser pulses has been the subject of a large body of work that aims to better understand and control this phenomenon. Although specific magnetic materials' properties…

Since the discovery of ultrafast demagnetization in Ni thin films in 1996, laser-induced ultrafast spin dynamics have become a prominent research topic in the field of magnetism and spintronics. This development offers new possibilities for…

Laser-induced terahertz spin transport (TST) and ultrafast demagnetization (UDM) are central but so far disconnected phenomena in femtomagnetism and terahertz spintronics. Here, we use broadband terahertz emission spectroscopy to reliably…

Mesoscale and Nanoscale Physics · Physics 2021-05-27 R. Rouzegar , L. Brandt , L. Nadvornik , D. A. Reiss , A. L. Chekhov , O. Gueckstock , C. In , M. Wolf , T. S. Seifert , P. W. Brouwer , G. Woltersdorf , T. Kampfrath

Optically induced demagnetization of 3d metallic ferromagnets proceeds as fast as ~100 fs and is a crucial prerequisite for spintronic applications, such as ultrafast magnetization switching and spin transport. On the 100 fs time scale, the…

Following the demonstration of laser-induced ultrafast demagnetization in ferromagnetic nickel, several theoretical and phenomenological propositions have sought to uncover its underlying physics. In this work we revisit the three…

Strongly Correlated Electrons · Physics 2023-03-29 Suchetana Mukhopadhyay , Sudip Majumder , Surya Narayan Panda , Anjan Barman

A dependence of a relaxation rate on the shape of the demagnetized region for a longitudinal evolution of total magnetization to its equilibrium value following the ultrafast demagnetization is demonstrated. This shape-dependence is caused…

Materials Science · Physics 2015-01-14 I. A. Yastremsky
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