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The first theoretical investigation on the inner-shell single-photodetachment from the Si- negative ion is presented. The partial and total cross sections, the photoelectron phaseshifts, and the parameters of angular anisotropy are…

Atomic Physics · Physics 2016-05-25 Galina Schrange-Kashenock

Time-resolved ultrafast x-ray scattering from photo-excited matter is an emerging method to image ultrafast dynamics in matter with atomic-scale spatial and temporal resolutions. For a correct and rigorous understanding of current and…

Chemical Physics · Physics 2017-11-16 Gopal Dixit , Robin Santra

The fragmentation dynamics of 2,6- and 3,5-difluoroiodobenzene after iodine 4$d$ inner-shell photoionization with soft X-rays are studied using coincident electron and ion momentum imaging. By analyzing the momentum correlation between…

The dynamics and processes involved in particle-molecule scattering, including nuclear dynamics, are described and analyzed using various quantum information quantities throughout the different stages of the scattering. The main process…

Quantum Physics · Physics 2025-05-22 Martin Mendez , Federico M. Pont

Chiral molecules are widespread in nature, playing a fundamental role in bio-chemical processes and in the origin of life itself. The observation of dynamics in chiral molecules is crucial for the understanding and control of the chiral…

Ultrafast-optical-pump -- structural-probe measurements, including ultrafast electron and x-ray scattering, provide direct experimental access to the fundamental timescales of atomic motion, and are thus foundational techniques for studying…

A wide range of ultrafast phenomena in various atomic, molecular and condense matter systems is governed by electron dynamics. Therefore, the ability to image electronic motion in real space and real time would provide a deeper…

Atomic Physics · Physics 2018-02-27 Daria Popova-Gorelova

Emergent phenomena at complex-oxide interfaces have become a vibrant field of study in the past two decades due to the rich physics and a wide range of possibilities for creating new states of matter and novel functionalities for potential…

Materials Science · Physics 2024-06-19 C. -T. Kuo , G. Conti , J. E. Rault , C. M. Schneider , S. Nemšák , A. X. Gray

Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…

Atomic Physics · Physics 2016-11-02 N. Suárez , A. Chacón , M. F. Ciappina , B. Wolter , J. Biegert , M. Lewenstein

We examine x-ray scattering from an isolated organic molecule from the linear to nonlinear absorptiveregime. In the nonlinear regime, we explore the importance of both the elastic and inelastic channelsand observe the onset of nonlinear…

Chemical Physics · Physics 2021-06-09 Phay J. Ho , Adam E. A. Fouda , Kai Li , Gilles Doumy , Linda Young

Ground- and excited-state UV photoelectron spectra of thiouracils (2-thiouracil, 4-thiouracil and 2,4-dithiouracil) have been simulated using multireference configuration interaction calculations and Dyson norms as measure for the…

Chemical Physics · Physics 2021-03-16 Matthias Ruckenbauer , Sebastian Mai , Philipp Marquetand , Leticia González

The photon-ion merged-beams technique for the photoionization of mass/charge selected ionized atoms, molecules and clusters by x-rays from synchrotron radiation sources is introduced. Examples for photoionization of atomic ions are…

Atomic Physics · Physics 2017-02-22 S. Schippers , A. L. D. Kilcoyne , R. A. Phaneuf , A. Müller

The progress and the chronology in understanding the influence of electron correlations on the electronic structure of atoms and the dynamics of atomic processes are reviewed focusing on benchmark rare-gas atoms. The contributions and the…

It is proposed to use the photoelectric effect in the inner shells of the 229Th atoms to refine the energy of the 8.3-eV isomer. The calculation was performed using the Feinberg-Migdal shaking theory, which leads to the probability of…

Nuclear Theory · Physics 2023-11-07 F. F. Karpeshin

Since the discovery of electron-wave duality, electron scattering instrumentation has developed into a powerful array of techniques for revealing the atomic structure of matter. Beyond detecting local lattice variations in equilibrium…

Ionization of atoms and molecules in laser fields can lead to various interesting interference structures in the photoelectron spectrum. For the case of a super-intense extreme ultraviolet laser pulse, we identify a novel petal-like…

Atomic Physics · Physics 2022-03-29 Lei Geng , Hao Liang , K. Krajewska , Liang-You Peng , Qihuang Gong

Characterization of the inner-shell decay processes in molecules containing heavy elements is key to understanding x-ray damage of molecules and materials and for medical applications with Auger-electron-emitting radionuclides. The 1s hole…

X-Ray and Ultraviolet (UV) observations of the outer solar atmosphere have been used for many decades to measure the fundamental parameters of the solar plasma. This review focuses on the optically thin emission from the solar atmosphere,…

Solar and Stellar Astrophysics · Physics 2018-09-06 Giulio Del Zanna , Helen E. Mason

We measure the surface of CH$_3$NH$_3$PbI$_3$ single crystals by making use of two photon photoemission spectroscopy. Our method monitors the electronic distribution of photoexcited electrons, explicitly discriminating the initial…

An experimental continuous-wave (cw) pump-probe scheme is demonstrated by investigating the population and photoionization dynamics of an atomic system. Specifically, $^6$Li atoms are initially prepared in optically pumped $2^{2}S_{1/2}$…

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