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Decorating two-dimensional materials with transition-metal adatoms is an effective way to bring about new physical properties that are intriguing for applications in electronics and spintronics devices. Here, we systematically studied the…

Materials Science · Physics 2025-02-26 Min Gao , Jun Hu

Recent experimental evidence that fluorinated graphene creates local magnetic moments around F adatoms has not been supported by semilocal density-functional theory (DFT) calculations where the adsorption of an isolated F adatom induces no…

Mesoscale and Nanoscale Physics · Physics 2013-06-03 Hyun-Jung Kim , Jun-Hyung Cho

Adatom-decorated graphene offers a promising new path towards spintronics in the ultrathin limit. We combine experiment and theory to investigate the electronic properties of dilutely fluorinated bilayer graphene, where the fluorine adatoms…

Mesoscale and Nanoscale Physics · Physics 2015-10-07 Adam A. Stabile , Aires Ferreira , Jing Li , N. M. R. Peres , J. Zhu

In this paper, the work function of graphene doped by different metal adatoms and at different concentrations is investigated. Density functional theory is used to maximize the reduction of the work function. In general, the work function…

The interaction between two different materials can present novel phenomena that are quite different from the physical properties observed when each material stands alone. Strong electronic correlations, such as magnetism and…

The correlation between structural distortion and emergence of magnetism in graphene containing a single vacancy was investigated using first-principles calculations based on density functional theory (DFT). Our results have shown that a…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 Wendel S. Paz , Wanderlã L. Scopel , Jair C. C. Freitas

We report a strain-controlled tuning of magnetism in transition-metal-atom-decorated graphene. Our first-principles calculations demonstrate that strain can lead to a sudden change in the magnetic configuration of a transition metal (TM)…

Mesoscale and Nanoscale Physics · Physics 2011-08-09 Bing Huang , Jaejun Yu , Su-Huai Wei

We calculate the diffusion barrier of fluorine adatoms on doped graphene in the diluted limit using Density Functional Theory. We found that the barrier $\Delta$ strongly depends on the magnitude and character of the graphene's doping…

Mesoscale and Nanoscale Physics · Physics 2014-09-29 R. M. Guzmán-Arellano , A. D. Hernández-Nieves , C. A. Balseiro , Gonzalo Usaj

At the heart of current information nanotechnology lies the search for ideal platforms hosting the smallest possible magnets, i.e. single atoms with magnetic moments pointing out-of-plane, as requested in a binary-type of memory. For this…

The electronic transport properties of monolayer graphene have been studied before and after the deposition of a dilute coating of tungsten adatoms on the surface. For coverages up to 2.5\% of a monolayer, we find tungsten adatoms…

Mesoscale and Nanoscale Physics · Physics 2017-02-15 Jamie A. Elias , Erik A. Henriksen

There have recently been various reports of weak ferromagnetism in graphite (1,2) and synthetic carbon materials (3) such as rhombohedral C60 (4), as well as a theoretical prediction of a ferromagnetic instability in graphene sheets (5).…

Condensed Matter · Physics 2009-11-07 J. M. D. Coey , M. Venkatesan , C. B. Fitzgerald , A. P. Douvalis , I. S. Sanders

We investigate the effect of an applied uniaxial strain on the ferromagnetic instability due to long- range Coulomb interaction between Dirac fermions in graphene. In case of undeformed graphene the ferromagnetic exchange instability occurs…

Strongly Correlated Electrons · Physics 2013-04-30 Anand Sharma , Valeri N. Kotov , Antonio H. Castro Neto

Electronic structure and magnetic interactions of a Tb adatom on graphene are investigated from first principles using combination of density functional theory and multiconfigurational quantum chemistry techniques including spin-orbit…

Materials Science · Physics 2024-09-13 Monirul Shaikh , Alison Klein , Aleksander L. Wysocki

Motivated by recent studies reporting the formation of localized magnetic moments in doped graphene, we investigate the energetic cost for spin polarizing isolated impurities embedded in this material. When a well-known criterion for the…

Materials Science · Physics 2015-05-14 P. Venezuela , R. B. Muniz , A. T. Costa , D. M. Edwards , S. R. Power , M. S. Ferreira

Graphene is a model system for the study of electrons confined to a strictly two-dimensional layer1 and a large number of electronic phenomena have been demonstrated in graphene, from the fractional2, 3 quantum Hall effect to…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Jian-Hao Chen , W. G. Cullen , E. D. Williams , M. S. Fuhrer

A possibility to control magnetic properties by using electric fields is one of the most desirable characteristics for spintronics applications. Finding a suitable material remains an elusive goal, with only a few candidates found so far.…

Magnetic properties of graphene with randomly distributed magnetic defects/vacancies are studied in terms of the Kondo Hamiltonian in the mean field approximation. It has been shown that graphene with defects undergoes a magnetic phase…

Materials Science · Physics 2015-05-27 Y. G. Semenov , J. M. Zavada , K. W. Kim

We employ large-scale quantum Monte Carlo simulations to study the magnetic ordering transition among dilute magnetic moments randomly localized on the graphene honeycomb lattice, induced by long-ranged RKKY interactions at low charge…

Strongly Correlated Electrons · Physics 2010-10-25 Thomas Fabritius , Nicolas Laflorencie , Stefan Wessel

Intervalley scattering of carriers in graphene at `top' adatoms may give rise to a hidden Kekul\'e ordering pattern in the adatom positions. This ordering is the result of a rapid modulation in the electron-mediated interaction between…

Mesoscale and Nanoscale Physics · Physics 2018-05-02 L. González-Árraga , F. Guinea , P. San-Jose

We study the presence of ferromagnetism in the phase diagram of the two-dimensional honeycomb lattice close to half-filling (graphene) as a function of the strength of the Coulomb interaction and doping. We show that exchange interactions…

Strongly Correlated Electrons · Physics 2009-11-11 N. M. R. Peres , F. Guinea , A. H. Castro Neto