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The temporal resolution of sub-relativistic ultrafast electron diffraction (UED) is generally limited by radio frequency (RF) phase and amplitude jitter of the RF lenses that are used to compress the electron pulses. We theoretically show…

Accelerator Physics · Physics 2017-05-29 J. G. H. Franssen , O. J. Luiten

The temporal resolution of ultrafast electron diffraction (UED) at weakly relativistic beam energies ($\lesssim$ 100 keV) suffers from space-charge induced electron pulse broadening. We describe the implementation of a radio frequency (RF)…

Accelerator Physics · Physics 2024-05-08 Thomas Sutter , Joshua Lee , Atharva Kulkarni , Pietro Musumeci , Anshul Kogar

In modern high-gain free-electron lasers, ultra-fast photon pulses designed for studying chemical, atomic and biological systems are generated from a serial of behaviors of high-brightness electron beam at the time-scale ranging from…

Accelerator Physics · Physics 2015-10-22 Guanglei Wang , Meng Zhang , Wei Zhang , Haixiao Deng , Xueming Yang

We present a theoretical description of resonant radiofrequency (RF) deflecting cavities in TM$_{110}$ mode as dynamic optical elements for ultrafast electron microscopy. We first derive the optical transfer matrix of an ideal pillbox…

Instruments to visualize transient structural changes of inhomogeneous materials on the nanometer scale with atomic spatial and temporal resolution are demanded to advance materials science, bioscience, and fusion sciences. One such…

Accelerator Physics · Physics 2017-03-20 X. Shen , R. K. Li , U. Lundström , T. J. Lane , A. H. Reid , S. P. Weathersby , X. J. Wang

We report the experimental demonstration of femtosecond electron diffraction using high-brightness MeV electron beams. High-quality, single-shot electron diffraction patterns for both polycrystalline aluminum and single-crystal 1T-TaS2 are…

Instrumentation and Detectors · Physics 2014-01-21 Pengfei Zhu , H. Berger , J. Cao , J. Geck , Y. Hidaka , R. Kraus , S. Pjerov , Y. Shen , R. I Tobey , Y. Zhu , J. P. Hill , X. J. Wang

Pushing the limits in temporal resolution for transmission electron microscopy (TEM) requires a revolutionary change in the electron source technology. In this paper we study the possibility of employing a radiofrequency photoinjector as…

Accelerator Physics · Physics 2014-05-26 R. K. Li , P. Musumeci

While sensing in high temporal resolution is necessary for wide range of application, it is still limited nowadays due to cameras sampling rate. In this work we try to increase the temporal resolution beyond the Nyquist frequency, which is…

Signal Processing · Electrical Eng. & Systems 2022-11-28 Khen Cohen , Dan Raviv , David Mendlovic

The precision measurement of real-time electron temporal profiles is crucial for advancing electron and X-ray devices used in ultrafast imaging and spectroscopy. While high temporal resolution and large temporal window can be achieved…

One of the frontiers in electron scattering is to couple ultrafast temporal resolution with highly localized probes to investigate the role of microstructure on material properties. Here, taking advantage of the unprecedented average…

Applied Physics · Physics 2019-06-07 Fu-Hao Ji , Daniel Durham , Andrew Minor , Pietro Musumeci , Jorge Navarro , Daniele Filippetto

The possibility to obtain a three-dimensional representation of a single object with sub-$\mu$m resolution is crucial in many fields, from material science to clinical diagnostics. This is typically achieved through tomography, which…

The ability to resolve the dynamics of matter on its native temporal and spatial scales constitutes a key challenge and convergent theme across chemistry, biology, and materials science. The last couple of decades have witnessed ultrafast…

A significant contribution to the temporal resolution of an ultrafast electron diffraction (UED) instrument is arrival time jitter caused by amplitude and phase variation of radio frequency (RF) cavities. In this paper, we present a…

Accelerator Physics · Physics 2024-08-16 Tianzhe Xu , Fuhao Ji , Stephen Weathersby , Robert Joel England

Ultrafast Electron Microscopy (UEM) has been demonstrated to be an effective table-top technique for imaging the temporally-evolving dynamics of matter with subparticle spatial resolution on the time scale of atomic motion. However, imaging…

Optics · Physics 2017-08-02 M. Th. Hassan , J. S. Baskin , B. Liao , A. H. Zewail

We present the results of an experiment where a short focal length (~ 1.3 cm) permanent magnet electron lens is used to image micron-size features of a metal sample in a single shot, using an ultra- high brightness ps-long 4 MeV electron…

Accelerator Physics · Physics 2016-07-13 D. Cesar , J. Maxson , P. Musumeci , Y. Sun , J. Harrison , P. Frigola , F. H. O'Shea , H. To , D. Alesini , R. K. Li

Ultrafast electron diffraction (UED) instruments typically operate at kHz or lower repetition rates and rely on indirect detection of electrons. However, these experiments encounter limitations because they are required to use electron…

Chemical Physics · Physics 2024-08-06 Fernando Rodriguez Diaz , Mark Mero , Kasra Amini

In this work, a long-cavity semiconductor laser subject to optical feedback is exploited to generate repetitive temporal patterns with enhanced intra-pattern sample diversity. Stable limit cycle dynamics characterized by multiple frequency…

Optics · Physics 2025-10-14 Apostolos Argyris

MeV ultrafast electron diffraction (UED) is a widely used technology for ultrafast structural dynamic studies of matters in numerous areas. The development of laser wakefield accelerator (LWFA) envisions great potential of advanced…

Accelerator Physics · Physics 2024-04-22 Yu Fang , Fei Li , Jianfei Hua , Bo Guo , Linyi Zhou , Bing Zhou , Zhihao Chen , Jianyi Liu , Zheng Zhou , Yipeng Wu , Yingchao Du , Renkai Li , Wei Lu

Ultrafast-optical-pump -- structural-probe measurements, including ultrafast electron and x-ray scattering, provide direct experimental access to the fundamental timescales of atomic motion, and are thus foundational techniques for studying…

In the same manner that free-space propagation and curved glass lenses are used to shape the spatial properties of light, a combination of chromatic dispersion and devices known as time lenses may be used to reshape its temporal properties.…

Quantum Physics · Physics 2016-12-08 John M. Donohue , Morgan Mastrovich , Kevin J. Resch
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