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We experimentally demonstrate high quality factor spin wave resonances in an encapsulated thin film of the organic-based ferrimagnet vanadium tetracyanoethylene (V[TCNE]$_\textit{x~2}$) coated on an a-plane sapphire substrate by low…

Mesoscale and Nanoscale Physics · Physics 2016-09-21 Na Zhu , Xufeng Zhang , I. H. Froning , Michael E. Flatté , E. Johnston-Halperin , Hong X. Tang

We demonstrate a hybrid quantum system composed of superconducting resonator photons and magnons hosted by the organic-based ferrimagnet vanadium tetracyanoethylene (V[TCNE]$_x$). Our work is motivated by the challenge of scalably…

Integrating patterned, low-loss magnetic materials into microwave devices and circuits presents many challenges due to the specific conditions that are required to grow ferrite materials, driving the need for flip-chip and other indirect…

Vanadium tetracyanoethylene (V[TCNE]$_{x}$, $x\approx 2$) is an organic-based ferrimagnet with a high magnetic ordering temperature $\mathrm{T_C>600 ~K}$, low magnetic damping, and growth compatibility with a wide variety of substrates.…

We have fabricated hybrid magnetic complexes from V atoms and tetracyanoethylene (TCNE) ligands via atomic manipulation with a cryogenic scanning tunneling microscope. Using tunneling spectroscopy we observe spin-polarized molecular…

We demonstrate indirect electric-field control of ferromagnetic resonance (FMR) in devices that integrate the low-loss, molecule-based, room-temperature ferrimagnet vanadium tetracyanoethylene (V[TCNE]$_{x \sim 2}$) mechanically coupled to…

We report the successful extraction of spin polarized current from the organic-based room temperature ferrimagnetic semiconductor V[TCNE]x (x~2, TCNE: tetracyanoethylene; TC ~ 400 K, EG ~ 0.5 eV, s ~ 10-2 S/cm) and its subsequent injection…

Materials Science · Physics 2015-05-19 Lei Fang , K. Deniz Bozdag , Chia-Yi Chen , P. A. Truitt , A. J. Epstein , E. Johnston-Halperin

We propose an approach to realize a hybrid quantum system composed of a diamond nitrogen-vacancy (NV) center spin coupled to a magnon mode of the low-damping, low-moment organic ferrimagnet vanadium tetracyanoethylene. We derive an…

Mesoscale and Nanoscale Physics · Physics 2025-04-22 Denis R. Candido , Gregory D. Fuchs , Ezekiel Johnston-Halperin , Michael E. Flatté

We present a generic theoretical framework to describe non-reciprocal microwave circulation in a multimode cavity magnonic system and assess the optimal performance of practical circulator devices. We show that high isolation (> 56 dB),…

Applied Physics · Physics 2020-05-06 Na Zhu , Xu Han , Chang-Ling Zou , Mingrui Xu , Hong X. Tang

The molecular-based ferrimagnetic insulator V(TCNE)x has gained recent interest for efficient spin-wave excitation due to its low Gilbert damping ratio a=4E-5, and narrow ferromagnetic resonance linewidth f=1Oe. Here we report a clean spin…

Materials Science · Physics 2024-04-01 Zichen Wang , Seth Kurfman , Sarah Ursel , E. Johnston-Halperin , Henning Sirringhaus

Spintronic, spin caloritronic, and magnonic phenomena arise from complex interactions between charge, spin, and structural degrees of freedom that are challenging to model and even more difficult to predict. This situation is compounded by…

Coherent magnon modes in a truly three-dimensional (3D) magnonic crystal have not yet been investigated. This scientific gap exists despite the numerous theoretical predictions about miniband formation and edge modes with topological…

Mesoscale and Nanoscale Physics · Physics 2026-03-05 Huixin Guo , Kilian Lenz , Mateusz Gołębiewski , Ryszard Narkowicz , Jürgen Lindner , Maciej Krawczyk , Dirk Grundler

Multiferroics offer an elegant means to implement voltage-control and on the fly reconfigurability in microscopic, nanoscaled systems based on ferromagnetic materials. These properties are particularly interesting for the field of…

Nitrogen-vacancy (NV) magnetometry is a new technique for imaging spin waves in magnetic materials. It detects spin waves by their microwave magnetic stray fields, which decay evanescently on the scale of the spin-wavelength. Here, we use…

Mesoscale and Nanoscale Physics · Physics 2022-12-08 Brecht G. Simon , Samer Kurdi , Joris J. Carmiggelt , Michael Borst , Allard Katan , Toeno van der Sar

Quantum information science and engineering requires novel low-loss magnetic materials for magnon-based quantum-coherent operations. The search for low-loss magnetic materials, traditionally driven by applications in microwave electronics…

Measurements of the static magnetic susceptibility and of the nuclear magnetic resonance of multiwalled vanadium-oxide nanotubes are reported. In this nanoscale magnet the structural low-dimensionality and mixed valency of vanadium ions…

Strongly Correlated Electrons · Physics 2009-11-11 E. Vavilova , I. Hellmann , V. Kataev , C. Taeschner , B. Buechner , R. Klingeler

Magnetic insulators, such as yttrium iron garnet (Y$_3$Fe$_5$O$_{12}$), are ideal materials for ultra-low power spintronics applications due to their low energy dissipation and efficient spin current generation and transmission. Recently,…

Mesoscale and Nanoscale Physics · Physics 2016-12-05 Matthias B. Jungfleisch , Junjia Ding , Wei Zhang , Wanjun Jiang , John E. Pearson , Valentine Novosad , Axel Hoffmann

Magnon confinement and trapping refer to the localization of magnons-quasiparticles that represent collective spin-wave excitations in magnetic materials-within specific regions or structures. This concept is essential in magnonics, a…

Mesoscale and Nanoscale Physics · Physics 2026-02-10 J. Chen , H. Yu , R. Gallardo , P. Landeros , G. Gubbiotti

Magnonics is gaining momentum as an emerging technology for information processing. The wave character and Joule heating-free propagation of spin-waves hold promises for highly efficient analog computing platforms, based on integrated…

Rigidity of an ordered phase in condensed matter results in collective excitation modes spatially extending in macroscopic dimensions. Magnon is a quantum of an elementary excitation in the ordered spin system, such as ferromagnet. Being…

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