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We use one photon to simulate an n-qubit quantum system for the first time. We propose a new scheme to realize universal quantum computation in polynomial time O(n^5). A generating set of gates can be realized with high accuracy in the lab.…

Quantum Physics · Physics 2019-09-23 Xiaoqin Gao , Zhengwei Liu

The most efficient known quantum circuits for preparing unitary coupled cluster states and applying Trotter steps of the arbitrary basis electronic structure Hamiltonian involve interleaved sequences of fermionic Gaussian circuits and Ising…

Quantum Physics · Physics 2021-09-13 Nicholas C. Rubin , Joonho Lee , Ryan Babbush

This paper discusses quantum algorithms for the generator coordinate method (GCM) that can be used to benchmark molecular systems. The GCM formalism defined by exponential operators with exponents defined through generators of the Fermionic…

Quantum Physics · Physics 2024-02-14 Muqing Zheng , Bo Peng , Nathan Wiebe , Ang Li , Xiu Yang , Karol Kowalski

Electron transport in realistic physical and chemical systems often involves the non-trivial exchange of energy with a large environment, requiring the definition and treatment of open quantum systems. Because the time evolution of an open…

Advances in photonics require photon-number resolved simulations of quantum optical experiments with Gaussian states. We demonstrate a simple and versatile method to simulate the photon statistics of general multimode Gaussian states. The…

Quantum Physics · Physics 2023-03-06 Erik Fitzke , Florian Niederschuh , Thomas Walther

We present a classical algorithm for simulating universal quantum circuits composed of "free" nearest-neighbour matchgates or equivalently fermionic-linear-optical (FLO) gates, and "resourceful" non-Gaussian gates. We achieve the promotion…

Quantum Physics · Physics 2024-12-11 Oliver Reardon-Smith , Michał Oszmaniec , Kamil Korzekwa

To investigate the effect of quantum coherence on electronic energy transfer, which is the subject of current interest in photosynthesis, we solve the problem of transport for the simplest model of an aggregate of monomers interacting…

Quantum Physics · Physics 2015-03-19 J. S. Briggs , A. Eisfeld

Energy transfer within photosynthetic systems can display quantum effects such as delocalized excitonic transport. Recently, direct evidence of long-lived coherence has been experimentally demonstrated for the dynamics of the…

Quantum Physics · Physics 2008-12-06 Masoud Mohseni , Patrick Rebentrost , Seth Lloyd , Alán Aspuru-Guzik

The dynamics of the excitation energy transfer (EET) in photosynthetic complexes is an interesting question both from the perspective of fundamental understanding and the research in artificial photosynthesis. Challenges persist in…

Chemical Physics · Physics 2024-06-25 Amartya Bose , Peter L. Walters

Quantum computing can potentially provide advantages for specific computational tasks. The simulation of fermionic systems is one such task that lends itself well to quantum computation, with applications in nuclear physics and electronic…

Quantum Physics · Physics 2024-03-14 Isaac Hobday , Paul Stevenson , James Benstead

In this work, we developed an efficient quantum algorithm for the simulation of non-Markovian quantum dynamics, based on the Feynman path integral formulation. The algorithm scales polynomially with the number of native gates and the number…

Quantum Physics · Physics 2024-11-28 Avin Seneviratne , Peter L. Walters , Fei Wang

Near-unity energy transfer efficiency has been widely observed in natural photosynthetic complexes. This phenomenon has attracted broad interest from different fields, such as physics, biology, chemistry and material science, as it may…

Quantum nanosystems involve the coupled dynamics of fermions or bosons across multiple scales in space and time. Examples include quantum dots, superconducting or magnetic nanoparticles, molecular wires, and graphene nanoribbons. The number…

Mesoscale and Nanoscale Physics · Physics 2011-11-01 D. Balamurugan , Peter. J. Ortoleva

We propose an efficient protocol for digital quantum simulation of quantum chemistry problems and enhanced digital-analog quantum simulation of transport phenomena in biomolecules with superconducting circuits. Along these lines, we…

Quantum Physics · Physics 2016-06-23 L. García-Álvarez , U. Las Heras , A. Mezzacapo , M. Sanz , E. Solano , L. Lamata

The Fenna Mathews Olson (FMO) complex of green sulphur bacteria is an example of a photosynthetic pigment protein complex, in which the electronic properties of the pigments are modified by the protein environment to promote efficient…

Biomolecules · Quantitative Biology 2014-07-23 Alexander S. Fokas , Daniel J. Cole , Alex W. Chin

We propose the use of quantum optical systems to perform universal simulation of quantum dynamics. Two specific implementations that require present technology are put forward for illustrative purposes. The first scheme consists of neutral…

Quantum Physics · Physics 2007-05-23 E. Jané , G. Vidal , W. Dür , P. Zoller , J. I. Cirac

Determining how energy flows within and between molecules is crucial for understanding chemical reactions, material properties, and even vital processes such as photosynthesis. While the general principles of energy transfer are well…

Other Condensed Matter · Physics 2025-12-16 Ignacio Gustin , Chang Woo Kim , Ignacio Franco

Particles produced in high energy collisions that are charged under one of the fundamental forces will radiate proportionally to their charge, such as photon radiation from electrons in quantum electrodynamics. At sufficiently high…

High Energy Physics - Phenomenology · Physics 2021-02-17 Christian W. Bauer , Wibe A. de Jong , Benjamin Nachman , Davide Provasoli

The time-evolution of multiparty quantum correlations as quantified by monogamy scores and bipartition collections of quantum correlations is investigated for light-harvesting complexes modeled by the fully connected and the…

Quantum Physics · Physics 2015-02-11 Titas Chanda , Utkarsh Mishra , Aditi Sen De , Ujjwal Sen

Quantum gates are the building blocks of quantum circuits, which in turn are the cornerstones of quantum information processing. In this work, we theoretically investigate a single-step implementation of both a universal two- (CNOT) and…

Quantum Physics · Physics 2024-07-01 Luiz O. R. Solak , Daniel Z. Rossatto , Celso J. Villas-Boas