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Single photons are of paramount importance to future quantum technologies, including quantum communication and computation. Nonlinear photonic devices using parametric processes offer a straightforward route to generating photons, however…
Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders of magnitude higher than real-world conditions corresponding…
Two-photon absorption (TPA) fluorescence of biomarkers has been decisive in advancing the fields of biosensing and deep-tissue in vivo imaging of live specimens. However, due to the extremely small TPA cross section and the quadratic…
Entangled photon spectroscopy is a nascent field that has important implications for measurement and imaging across chemical, biology, and materials fields. Entangled photon spectroscopy potentially offers improved spatial and…
We consider a photonic crystal (PC) doped with four-level atoms whose intermediate transition is coupled near-resonantly with a photonic band-gap edge. We show that two photons, each coupled to a different atomic transition in such atoms,…
We experimentally demonstrate amplitude and phase modulation of a time-energy entangled two-photon wave function. The entangled photons are produced by spontaneous parametric down-conversion, spectrally dispersed in an prism compressor,…
We present detailed instructions for constructing and operating an apparatus to produce and detect polarization-entangled photons. The source operates by type-I spontaneous parametric downconversion in a two-crystal geometry. Photons are…
Pairs of photons entangled in their time-frequency degree of freedom are of great interest in quantum optics research and applications, due to their relative ease of generation and their high capacity for encoding information. Here we…
We show that two-photon absorption (TPA) in Rubidium atoms can be greatly enhanced by the use of a hollow-core photonic bandgap fiber. We investigate off-resonant, degenerate Doppler-free TPA on the 5S1/2 - 5D5/2 transition and observe 1%…
Entangling independent photons is not only of fundamental interest but also of crucial importance for quantum information science. Two-photon interference is a major method to entangle independent identical photons. If two photons are…
Entangled photon pairs are predicted to linearize and increase the efficiency of two-photon absorption, allowing continuous wave laser diodes to drive ultrafast time-resolved spectroscopy and nonlinear processes. Despite a range of…
It is controversial what is the true role of entanglement in two-photon virtual-state spectroscopy [Saleh et al, Phys. Rev. Lett. 80, 3483, 1998], a two-photon absorption spectroscopic technique that can retrieve information about the…
Ultrafast optical spectroscopy is a powerful technique for studying the dynamic processes of molecular systems in condensed phases. However, in molecular systems containing many dye molecules, the spectra can become crowded and difficult to…
A quantum system composed of two or more subsystems can be in an entangled state, i.e. a state in which the properties of the global system are well defined but the properties of each subsystem are not. Entanglement is at the heart of…
Nonlinear spectroscopic techniques using entangled photon pairs can provide an opportunity to exploit non-classical correlations encoded in two-photon wavefunctions to manipulate two-exciton wavefunctions. We propose an entangled photon…
Entangled photons can be used to make measurements with an accuracy beyond that possible with classical light. While most implementations of quantum metrology have used states made up of a single colour of photons, we show that entangled…
We describe a proof-of-principal experiment demonstrating a Fourier technique for measuring the shape of biphoton wavepackets. The technique is based on the use of synchronously driven fast modulators and slow (integrating) detectors.
We describe two-photon absorption processes excited by entangled pairs, but not by non-entangled pairs of the same energy and polarization. Photon states are selected for destructive interference in the non-entangled process between…
Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…
High-dimensional entanglement offers a variety of advantages for both fundamental and applied applications in quantum information science. A central building block for such applications is a programmable processor of entangled states, which…