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A much-needed solution for the efficient modeling of strong coupling between matter and optical cavity modes is offered by mean-field mixed quantum--classical dynamics, where a classical cavity field interacts self-consistently with quantum…

Chemical Physics · Physics 2023-12-13 Ming-Hsiu Hsieh , Alex Krotz , Roel Tempelaar

The dynamics of an electronic system interacting with an electromagnetic field is investigated within mixed quantum-classical theory. Beyond the classical path approximation (where we ignore all feedback from the electronic system on the…

Chemical Physics · Physics 2019-02-11 Hsing-Ta Chen , Tao E. Li , Maxim Sukharev , Abraham Nitzan , Joseph E. Subotnik

Mean-field mixed quantum--classical dynamics could provide a much-needed means to inexpensively model quantum electrodynamical phenomena, by describing the optical field and its vacuum fluctuations classically. However, this approach is…

Chemical Physics · Physics 2023-12-11 Ming-Hsiu Hsieh , Alex Krotz , Roel Tempelaar

An economic modeling approach for cavity quantum electrodynamics is provided by mean-field dynamics, wherein the optical field is described classically while a self-consistent interaction with quantum emitters is incorporated through the…

Chemical Physics · Physics 2025-12-10 Ming-Hsiu Hsieh , Alex Krotz , Roel Tempelaar

The dynamics of an electronic two-level system coupled to an electromagnetic field are simulated explicitly for one and three dimensional systems through semiclassical propagation of the Maxwell-Liouville equations. We consider three…

Mixed quantum-classical mechanics descriptions are critical to modeling coupled electron-nuclear dynamics, i.e. non-adiabatic molecular dynamics, relevant to photochemical and photophysical processes. We argue that, for polyatomic…

Chemical Physics · Physics 2018-08-21 Roman Baskov , Alexander White , Dmitry Mozyrsky

The quantum theory of electromagnetic radiation predicts characteristic statistical fluctuations for light sources as diverse as sunlight, laser radiation and molecule fluorescence. Indeed, these underlying statistical fluctuations of light…

The optical response of an electronic two-level system (TLS) coupled to an incident continuous wave (cw) electromagnetic (EM) field is simulated explicitly in one dimension by the following five approaches: (i) the coupled Maxwell-Bloch…

Optics · Physics 2019-03-19 Tao E. Li , Hsing-Ta Chen , Joseph E. Subotnik

We explore the quantum dynamics of photoassociation of Bose-Einstein condensed atoms into molecules using an optical cavity field. Inside of an optical resonator, photoassociation of quantum degenerate atoms involves the interaction of…

Quantum Gases · Physics 2015-05-13 Christopher P. Search , J. Mauricio Campuzano , Marko Zivkovic

Processes involving ultrafast laser driven electron-phonon dynamics play a fundamental role in the response of quantum systems in a growing number of situations of interest, as evidenced by phenomena such as strongly driven phase…

Materials Science · Physics 2024-03-01 Kevin Lively , Shunsuke A. Sato , Guillermo Albareda , Angel Rubio , Aaron Kelly

We investigate detailed balance for a quantum system interacting with thermal radiation within mixed quantum-classical theory. For a two-level system coupled to classical radiation fields, three semiclassical methods are benchmarked: (1)…

Chemical Physics · Physics 2019-07-17 Hsing-Ta Chen , Tao E. Li , Abraham Nitzan , Joseph E. Subotnik

Quantum path interferences or resonances in multilevel dissipative quantum systems play an important and intriguing role in the transport processes of nanoscale systems. Many previous minimalistic models used to describe the quantum path…

Quantum Physics · Physics 2013-10-22 Xin Chen

We benchmark a selection of semiclassical and perturbative dynamics techniques by investigating the correlated evolution of a cavity-bound atomic system to assess their applicability to study problems involving strong light-matter…

Quantum Physics · Physics 2020-01-29 Norah M. Hoffmann , Christian Schäfer , Niko Säkkinen , Angel Rubio , Heiko Appel , Aaron Kelly

An intriguing consequence of quantum field theory is that vacuum is not empty space; it is full of quantum fluctuating electromagnetic fields, or virtual photons, corresponding to their zero-point energy, even though the average number of…

Quantum Physics · Physics 2025-07-15 Andrey Baydin , Hanyu Zhu , Motoaki Bamba , Kaden Hazzard , Junichiro Kono

Equilibrium quantum phase transitions profoundly reshape the ground state of light-matter systems; yet, the resulting quantum correlations, such as squeezing and entanglement, remain experimentally inaccessible since they involve virtual…

Quantum Physics · Physics 2026-05-14 Gabriele Orlando , Daniele Lamberto , Franco Nori , Salvatore Savasta

Vacuum quantum fluctuations are an inescapable and fundamental feature of modern physics. By integrating cavity-enhanced or surface-modified vacuum quantum fluctuations with low-dimensional materials, a new paradigm-vacuumronics-emerges,…

Mesoscale and Nanoscale Physics · Physics 2025-12-12 Qing-Dong Jiang

The interplay of quantum fluctuations with nonlinear dynamics is a central topic in the study of open quantum systems, connected to fundamental issues (such as decoherence and the quantum-classical transition) and practical applications…

Quantum Physics · Physics 2009-11-13 Michael A. Armen , Hideo Mabuchi

Nonlinear dynamics in the fundamental interaction between a two-level atom with recoil and a quantized radiation field in a high-quality cavity is studied. We consider the strongly coupled atom-field system as a quantum-classical hybrid…

Quantum Physics · Physics 2011-11-09 S. V. Prants

Cavity quantum-electrodynamics experiments using an atom coupled to a single radiation-field mode have played a central role in testing foundations of quantum mechanics, thus motivating solid-state implementations using single quantum dots…

The rapid progress in quantum-optical experiments especially in the field of cavity quantum electrodynamics and nanoplasmonics, allows to substantially modify and control chemical and physical properties of atoms, molecules and solids by…

Chemical Physics · Physics 2022-01-24 Davis M. Welakuh , Johannes Flick , Michael Ruggenthaler , Heiko Appel , Angel Rubio
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