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The power conversion efficiency of photovoltaic devices based on semiconductor perovskites has reached ~20% after just several years of research efforts. With concomitant discoveries of other promising applications in lasers, light-emitting…

Although both epitaxial quantum dots (QDs) and colloidal nanocrystals (NCs) are quantum-confined semiconductor nanostructures, so far they have demonstrated dramatically-different exciton fine structure splittings (FSSs) at the cryogenic…

Mesoscale and Nanoscale Physics · Physics 2017-07-19 Chunyang Yin , Liyang Chen , Yan Lv , Fengrui Hu , Chun Sun , William W. Yu , Chunfeng Zhang , Xiaoyong Wang , Yu Zhang , Min Xiao

Lead halide perovskite nanocrystals are promising materials for classical and quantum light emission. To understand these outstanding properties, a thorough analysis of the band-edge exciton emission is needed which is not reachable in…

Mesoscale and Nanoscale Physics · Physics 2023-04-07 Mohamed-Raouf Amara , Zakaria Said , Caixia Huo , Aurélie Pierret , Christophe Voisin , Weibo Gao , Qihua Xiong , Carole Diederichs

Fully-inorganic cesium lead halide perovskite nanocrystals (NCs) have shown to exhibit outstanding optical properties such as wide spectral tunability, high quantum yield, high oscillator strength as well as blinking-free single photon…

We report on the optical properties of CsPbBr3 polycrystalline thin film on a single grain level. A sample comprised of isolated nanocrystals (NCs) mimicking the properties of the polycrystalline thin film grains that can be individually…

Exciton-phonon interactions govern the energy level spectrum and thus the optical response in semiconductors. In this respect, lead-halide perovskite nanocrystals represent a unique system, for which the interaction with optical phonons is…

The use of semiconductor nanocrystals in scalable quantum technologies requires characterization of the exciton coherence dynamics in an \emph{ensemble} of electronically isolated crystals in which system-bath interactions are nevertheless…

Over the last two decades, intensive research efforts have been devoted to the suppressions of photoluminescence (PL) blinking and Auger recombination in metal-chalcogenide nanocrystals (NCs), with significant progresses being made only…

Materials Science · Physics 2016-11-03 Fengrui Hu , Chunyang Yin , Huichao Zhang , Chun Sun , William W. Yu , Chunfeng Zhang , Xiaoyong Wang , Yu Zhang , Min Xiao

Cesium lead halide nanocrystals and quantum dots are prominent materials for different types of applications because of their remarkable photophysical properties. However, they are also known to exhibit the same effects observed for…

The interest in perovskite nanocrystals (NCs) such as CsPbBr$_3$ for quantum applications is rapidly raising, as it has been demonstrated that they can behave as very efficient single photon emitters. The main problem to tackle in this…

Dark ground state exciton in semiconductor nanocrystals has been a subject of much interest due to its long lifetime attractive for applications requiring long-lived electronic or spin states. Significant effort has been made recently to…

Achieving pure single-photon emission is essential for a range of quantum technologies, from optical quantum computing to quantum key distribution to quantum metrology. Among solid-state quantum emitters, colloidal lead halide perovskite…

Advances in opto-electronics require the development of materials with novel and engineered characteristics. A class of materials that has garnered tremendous interest is metal-halide perovskites, stimulated by meteoric increases in…

Perovskite nanocrystals (NCs) have attracted increasing interest for the realization of single-photon emitters, owing to their ease of chemical synthesis, wide spectral tunability, fast recombination rate, scalability, and high quantum…

Lead-halide perovskite nanocrystals (PNCs) exhibit unique optoelectronic properties, many of which originate from a purported bright-triplet exciton fine-structure. A major impediment to measuring this fine-structure is inhomogeneous…

Mesoscale and Nanoscale Physics · Physics 2022-03-09 Albert Liu

The one-photon absorption cross section of nanocrystals (NCs) of the inorganic perovskite CsPbBr$_{3}$ is studied theoretically using a multiband $\mathbf{k}\cdot\mathbf{p}$ envelope-function model combined with a treatment of intercarrier…

Mesoscale and Nanoscale Physics · Physics 2020-05-11 T. P. T. Nguyen , S. A. Blundell , C. Guet

Moir\'e potential acts as periodic quantum confinement for optically generated exciton, generating spatially ordered zero-dimensional quantum system. However, broad emission spectrum arising from inhomogeneity among moir\'e potential…

Single cesium lead bromide (CsPbBr3) nanocrystals show strong photoluminescence blinking, with on- and off- dwelling times following power-law distributions. We investigate the memory effect in the photoluminescence blinking of single…

Colloidal perovskite nanocrystals (NCs) are a well-proven platform for growing anisotropic structures. Nanowires (NWs) exhibiting a quantum confinement phenomenon and microwires (MWs), which enable lasing, are of particular interest for…

Metal-halide perovskite nanocrystals (PNCs) have emerged as leading candidates for next-generation quantum emitters, offering a unique combination of high photoluminescence quantum yield, tunable emission, short radiative lifetimes, and…

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