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Atomic-like defects in solids are not considered to be identical owing to the imperfections of host lattice. Here, we found that even under ambient conditions, negatively charged nitrogen-vacancy (NV$^-$) centers in diamond could still…
Ensembles of nitrogen-vacancy (NV) centers in diamond are versatile quantum sensors with broad applications in the physical and life sciences. The concentration of neutral substitutional nitrogen ([N$_\text{s}^0$]) strongly influences…
Understanding the profile of a qubit's wavefunction is key to its quantum applications. Unlike conducting systems, where a scanning tunneling microscope can be used to probe the electron distribution, there is no direct method for…
Spin squeezed states provide a seminal example of how the structure of quantum mechanical correlations can be controlled to produce metrologically useful entanglement. Such squeezed states have been demonstrated in a wide variety of…
Quantum sensors based on nitrogen vacancy (NV) centers in diamond have been a central topic in the sensing community for more than a decade. The extraordinary properties at room temperature of the spin system in diamond have made it one of…
Efficient readout of individual electronic spins associated with atom-like impurities in the solid state is essential for applications in quantum information processing and quantum metrology. We demonstrate a new method for efficient spin…
Chemical sensors with high sensitivity that can be used in extreme conditions and can be miniaturized are of high interest in science and industry. The Nitrogen-vacancy (NV) center in diamond is an ideal candidate as a nanosensor due to the…
We experimentally isolate, characterize and coherently control up to six individual nuclear spins that are weakly coupled to an electron spin in diamond. Our method employs multi-pulse sequences on the electron spin that resonantly amplify…
Near-surface nitrogen-vacancy (NV) centers have been created in diamond through low energy implantation of 15N to sense electron spins that are external to the diamond. By performing double resonance experiments, we have verified the…
Nitrogen-Vacancy (NV) spin in diamond is a versatile quantum sensor, being able to measure physical quantities such as magnetic field, electric field, temperature, and pressure. In the present work, we demonstrate a multiplexed sensing of…
The lower critical magnetic field, $H_{c1}$, of superconductors is measured by using ensembles of NV-centers-in-diamond optical magnetometry. The technique is minimally invasive, and has sub-gauss field sensitivity and sub-$\mu$m spatial…
Detecting individual spins--including stable and metastable states--represents a fundamental challenge in quantum sensing with broad applications across condensed matter physics, quantum chemistry, and single-molecule magnetic resonance…
Magnetic Resonance Imaging (MRI) can characterize and discriminate among tissues using their diverse physical and biochemical properties. Unfortunately, submicrometer screening of biological specimens is presently not possible, mainly due…
The decoherence of point defect qubits is often governed by the electron spin-nuclear spin hyperfine interaction that can be parameterized by using ab inito calculations in principle. So far most of the theoretical works have focused on the…
Diamond has been extensively investigated recently due to a wide range of potential applications of nitrogen-vacancy (NV) defect centers existing in a diamond lattice. The applications include magnetometry and quantum information…
Ensembles of nitrogen-vacancy (NV) centers in diamond are widely used as AC magnetometers. While such measurements are usually performed using standard (XY) dynamical decoupling (DD) protocols at room temperature, we study the sensitivities…
We demonstrate fluorescence thermometry techniques with sensitivities approaching 10 mK Hz^(-1/2) based on the spin-dependent photoluminescence of nitrogen vacancy (NV) centers in diamond. These techniques use dynamical decoupling protocols…
The detection of ensembles of spins under ambient conditions has revolutionized the biological, chemical, and physical sciences through magnetic resonance imaging and nuclear magnetic resonance. Pushing sensing capabilities to the…
The sensitivity of a practical quantum magnetometer is challenged by both inhomogeneous coupling between sensors and environment and errors in quantum control. Based on the physical criteria of modern quantum sensing, we present a robust…
To use batteries as large-scale energy storage systems it is necessary to measure and understand their degradation \textit{in-situ} and \textit{in-operando}. As a battery's degradation is often the result of molecular processes inside the…