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The transmission of linearly and circularly polarized waves are studied both theoretically and experimentally for chiral metasurfaces formed by arrays of metallic square helices. The helical particles of the metasurfaces are constructed of…

Classical Physics · Physics 2019-09-13 Shengzhe Wu , Vladimir V. Yachin , Vitalii I. Shcherbinin , Vladimir R. Tuz

Many biological and synthetic materials self-assemble into helical or twisted aggregates. The shape is determined by a complex interplay between elastic forces and the orientation and chirality of the constituent molecules. We study this…

Soft Condensed Matter · Physics 2007-05-23 Robin L. B. Selinger , Jonathan V. Selinger , Anthony P. Malanoski , Joel M. Schnur

When circularly polarized light interacts with a nanostructure, the optical response depends on the geometry of the structure. If the nanostructure is chiral (i.e., it cannot be superimposed on its mirror image), then its optical response,…

Understanding how nanostructure and nanomechanics influence physical material properties on the micro- and macroscale is an essential goal in soft condensed matter research. Mechanisms governing fragmentation and chirality inversion of…

Soft Condensed Matter · Physics 2017-05-19 Gustav Nyström , Jozef Adamcik , Ivan Usov , Mario Arcari , Raffaele Mezzenga

We use continuum theory to show that chirality is a key thermodynamic control parameter for the aggregation of biopolymers: chirality produces a stable disperse phase of hexagonal bundles under moderately poor solvent conditions, as has…

Soft Condensed Matter · Physics 2009-11-13 Gregory M. Grason , Robijn F. Bruinsma

Chiral photonics opens new pathways to manipulate light-matter interactions and tailor the optical response of meta-surfaces and -materials by nanostructuring nontrivial patterns. Chirality of matter, such as that of molecules, and light,…

Optics · Physics 2022-02-16 Oliver Mey , Arash Rahimi-Iman

The inherently weak chiroptical responses of natural materials limit their usage for controlling and enhancing chiral light-matter interactions. Recently, several nanostructures with subwavelength scale dimensions were demonstrated, mainly…

Chiral twisting of the molecular orientation within the layer of a smectic-A liquid crystal has been investigated using circular dichroism spectroscopy. The results indicate that a rotation of the layers away from the alignment direction is…

Soft Condensed Matter · Physics 2009-10-31 M. S. Spector , S. K. Prasad , B. T. Weslowski , R. D. Kamien , J. V. Selinger , B. R. Ratna , R. Shashidar

We demonstrate formation of hierarchical structures in two-dimensional systems with multiple length scales in the inter-particle interaction. These include states such as clusters of clusters, concentric rings, clusters inside a ring, and…

Superconductivity · Physics 2013-09-25 Christopher N. Varney , Karl A. H. Sellin , Qingze Wang , Hans Fangohr , Egor Babaev

We studied a collection of chiral active particles (CAP) on a two dimensional substrate using extensive numerical study. Particles interact through soft repulsive interaction. The activity and chirality of particles is tuned by varying…

Soft Condensed Matter · Physics 2022-08-22 Vivek Semwal , Jayam Joshi , Shradha Mishra

Understanding the condensed-phase behavior of chiral molecules is important in biology, as well as in a range of technological applications, such as the manufacture of pharmaceuticals. Here, we use molecular dynamics simulations to study a…

Statistical Mechanics · Physics 2023-12-27 Pablo M. Piaggi , Roberto Car , Frank H. Stillinger , Pablo G. Debenedetti

We show that plane parabolic flow in a microfluidic channel causes nonmotile helically-shaped bacteria to drift perpendicular to the shear plane. Net drift results from the preferential alignment of helices with streamlines, with a…

Mesoscale and Nanoscale Physics · Physics 2010-04-07 Marcos , Henry C. Fu , Thomas R. Powers , Roman Stocker

Chiral symmetry breaking is ubiquitous in biological systems, from DNA to bacterial suspensions. A key unresolved problem is how chiral structures may spontaneously emerge from achiral interactions. We study a simple model of bacterial…

Soft Condensed Matter · Physics 2016-08-18 Rebekka E. Breier , Robin L. B. Selinger , Giovanni Ciccotti , Stephan Herminghaus , Marco G. Mazza

We experimentally demonstrate that individual molecules of formic acid are chiral even when they are in the vibronic ground state, which has a planar equilibrium structure. We ionize the C 1s shell of the molecule and record the…

We study a two-dimensional chiral active crystal composed of underdamped chiral active particles. These particles, characterized by intrinsic handedness and persistence, interact via linear forces derived from harmonic potentials. Chirality…

Soft Condensed Matter · Physics 2024-12-25 Umberto Marini Bettolo Marconi , Lorenzo Caprini

Chirality refers to the asymmetry of objects that cannot be superimposed on their mirror image. It is a concept that exists in various scientific fields and has profound consequences. Although these are perhaps most widely recognized within…

Chirality is a concept that one object is not superimposable on its mirror image by translation and rotation. In particular, chiral plasmonics have been widely investigated due to their excellent optical chiral properties, and have led to…

Optics · Physics 2023-07-18 Yuqing Cheng , Mengtao Sun

Efficient chirality sorting is now highly demanded to separate assembled mesoscopic chiral structures which are of very special physical properties rather than their achiral counterparts or those at the single-particle level. However, the…

Soft Condensed Matter · Physics 2019-07-03 Jie Su , Huijun Jiang , Zhonghuai Hou

The assembly of filamentous bundles with controlled diameters is common in biological systems and desirable for the development of nanomaterials. We discuss dynamical simulations and free energy calculations on patchy spheres with chiral…

Soft Condensed Matter · Physics 2015-05-18 Yasheng Yang , Robert B. Meyer , Michael F. Hagan

Recent liquid-crystalline (LC) research is focused on structurally new molecular systems distinct from simple nematic or smectic phases. Sophisticated molecular shape may reveal structural complexity, combining helicity and polarity.…