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We report the observation of second harmonic generation with high conversion efficiency $\sim 0.005\%$ in the terahertz regime from thin films of the topological insulator Bi$_2$Se$_3$ that exhibit the linear photogalvanic effect, measured…

Strongly Correlated Electrons · Physics 2024-06-11 Jonathan Stensberg , Xingyue Han , Zhuoliang Ni , Xiong Yao , Xiaoyu Yuan , Debarghya Mallick , Akshat Gandhi , Seongshik Oh , Liang Wu

High-harmonic generation (HHG) in solids has rapidly emerged as a promising platform for creating compact attosecond sources and probing ultrafast electron dynamics. Resonant metasurfaces are essential for enhancement of the otherwise small…

High-harmonic generation (HHG) in the two topological phases of a finite, one-dimensional, periodic structure is investigated using a self-consistent time-dependent density functional theory (TDDFT) approach. For harmonic photon energies…

Optics · Physics 2018-04-26 Dieter Bauer , Kenneth K. Hansen

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

Atomic Physics · Physics 2015-10-15 Christian Buth

Second-harmonic generation (SHG) is a fundamental nonlinear optical process widely used in photonics; however, it is strictly forbidden in the bulk of centrosymmetric materials due to their inversion symmetry. Nevertheless, applying an…

Graphene is a nonlinear material which can be used as a saturable absorber, frequency mixer and frequency multiplier. We investigate the third harmonic generation from graphene lying on different substrates, consisting of a dielectric…

Mesoscale and Nanoscale Physics · Physics 2017-02-09 N. A. Savostianova , S. A. Mikhailov

We show that the divergence of extreme ultraviolet pulses from high harmonic generation, which is directly linked to the shape and size of the refocused beam, can be controlled by the relative delay between the fundamental and its intense…

We present a theoretical framework for nonlinear optics of graphene and other 2D materials in layered structures. We derive a key equation to find the effective electric field and the sheet current density in the 2D material for given…

Optics · Physics 2018-12-27 J. L. Cheng , J. E. Sipe , N. Vermeulen , C. Guo

We report on high-order harmonic generation in the two-band superconductor MgB$_2$ driven by intense terahertz electromagnetic pulses. Third- and fifth-order harmonics are resolved in time domain and investigated as a function of…

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

High-order harmonic generation (HHG) in the relativistic regime is employed to obtain zeptosecond pulses of $\gamma$-rays. The harmonics are generated from atomic systems in counterpropagating strong attosecond laser pulse trains of linear…

Atomic Physics · Physics 2007-07-20 Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

We study second harmonic generation in centrosymmetric Weyl semimetal with broken time reversal symmetry. We calculate electric current density at the double frequency of the propagating electromagnetic field in the presence of applied…

Mesoscale and Nanoscale Physics · Physics 2017-03-03 A. A. Zyuzin , A. Yu. Zyuzin

We theoretically investigate the double-resonance Raman spectrum of monolayer graphene down to infrared laser excitation energies. By using first-principles density functional theory calculations, we improve upon previous theoretical…

Mesoscale and Nanoscale Physics · Physics 2025-05-21 Lorenzo Graziotto , Francesco Macheda , Thibault Sohier , Matteo Calandra , Francesco Mauri

Graphene was shown to have strongly nonlinear electrodynamic properties. In particular, being irradiated by an electromagnetic wave with the frequency $\omega$, it can efficiently generate higher frequency harmonics. Here we predict that in…

Mesoscale and Nanoscale Physics · Physics 2015-12-04 N. A. Savostianova , S. A. Mikhailov

Sub-wavelength graphene structures support localized plasmonic resonances in the terahertz and mid-infrared spectral regimes. The strong field confinement at the resonant frequency is predicted to significantly enhance the light-graphene…

Harmonic generation in underdense spatially homogeneous plasma is generally expected to be inefficient: in an unmagnetized uniform plasma the fundamental and its harmonics cannot be phase-matched, resulting in third-harmonic generation…

Plasma Physics · Physics 2026-01-21 S. Cao , M. R. Edwards

The generation of high-order harmonics in quasi-one-dimensional graphene nanoribbons (GNRs) initiated by intense coherent radiation is investigated. A microscopic theory describing the extreme nonlinear optical response of GNRs is…

Mesoscale and Nanoscale Physics · Physics 2020-07-15 H. K. Avetissian , B. R. Avchyan , G. F. Mkrtchian , K. A. Sargsyan

Applying the semiclassical model, we identify two connected effects in intraband high-harmonic generation (HHG): (1) propagation time from the point of emission at the source to the point of detection, (2) beyond-electric-dipole corrections…

Atomic Physics · Physics 2024-06-12 Simon Vendelbo Bylling Jensen , Lars Bojer Madsen

Solid-state materials have recently emerged as a new stage of strong-field physics and attosecond science. The mechanism of the electron dynamics driven by an ultrashort intense laser pulse is under intensive discussion. Here we…

Materials Science · Physics 2020-04-23 Kenichi L. Ishikawa , Yasushi Shinohara , Takeshi Sato , Tomohito Otobe

The effect of slow light on second harmonic generation in a periodically poled $\chi^{(2)}$ nonlinear medium is investigated theoretically. A linear $\pi$ phase shifted grating is used to slow the group velocity of the fundamental frequency…

Optics · Physics 2022-02-02 Thomas E. Maybour , Devin H. Smith , Peter Horak
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