Related papers: Michelson Interferometry of High-order Harmonic Ge…
High-order sideband generation (HSG), as an analogue of the interband processes in high-harmonic generation (HHG) in solids, is a nonperturbative nonlinear optical phenomenon in semiconductors that are simultaneously driven by a relatively…
High-order harmonic generation (HHG) provides a powerful optical tool for probing ultrafast dynamics on the attosecond timescale. While its mechanisms in gases and solids are well-established, understanding nonlinear optical responses in…
We generate high-order harmonics of a mid-infrared laser from a silicon single crystal and find their origin in the recollision of coherently accelerated electrons with their holes, analogously to the atomic and molecular case, and to ZnO…
The higher order harmonic generation process in the nonperturbative regime at the interaction of coherent electromagnetic radiation with the AB-stacked bilayer graphene at high Fermi energies is considered. The applied coherent…
High-order harmonic generation (HHG) in simultaneous intense near-infrared (NIR) laser light and brilliant x rays above an inner-shell absorption edge is examined. A tightly bound inner-shell electron is transferred into the continuum.…
Using time-dependent density functional theory, high-harmonic generation (HHG) is studied in one-dimensional structures of sizes from a single nucleus up to hundreds of nuclei. The HHG cutoff is observed to extent linearly with the system…
Second harmonic generation (SHG) is a nonlinear optical response arising exclusively from broken inversion symmetry in the electric-dipole limit. Recently, SHG has attracted widespread interest as a versatile and noninvasive tool for…
We theoretically demonstrate the quenching effect in below-threshold high harmonic generation (HHG) by using the time-dependent density-functional theory (TDDFT) and solving the time-dependent Schr\"{o}dinger equation (TDSE). It is shown…
Time-domain analysis of harmonic fields with sub-cycle resolution is now experimentally viable due to the emergence of sensitive, on-chip techniques for petahertz-scale optical-field sampling. We demonstrate how such a time-domain,…
High-order frequency mixing in graphene using a two-color radiation field consisting of the fundamental and the second harmonic fields of an ultrashort linearly polarized laser pulse is studied. It is shown that the harmonics originated…
Two-dimensional materials offer a versatile platform to study high-harmonic generation (HHG), encompassing as limiting cases bulk-like and atomic-like harmonic generation [Tancogne-Dejean and Rubio, Science Advance \textbf{4}, eaao5207…
High-harmonic spectroscopy is a promising candidate for imaging electronic structures and dynamics in condensed matter by all-optical means and with unprecedented temporal resolution. We investigate harmonic spectra from finite, hexagonal…
Applying time-dependent local density approximation (TDLDA), we study the high-order harmonic generation (HHG) of ethylene subjected to the one-color ($\omega=2.72$ eV) and the two-color ($\omega_1=2.72$ eV and $\omega_2=5.44$ eV)…
The properties of an electron in a typical solid are modified by the interaction with the crystal ions, leading to the formation of a quasiparticle: the polaron. Such polarons are often described using the Fr\"ohlich Hamiltonian, which…
Using dynamical Hartree-Fock mean-field theory, we study the high-harmonic generation (HHG) in the fullerene molecules C$_{60}$ and C$_{70}$ under strong pump wave driving. We consider a strong-field regime and show that the output harmonic…
One key parameter in the high-order harmonic generation (HHG) phenomenon is the exact frequency of the generated harmonic field. Its deviation from perfect harmonics of the laser frequency can be explained considering (i) the single-atom…
Interferometric measurements of high-harmonics induced by multiple laser fields in an emerging field of research that promises optimized yield of harmonics, and time and space-resolved nonlinear spectroscopy. Most of the measurements have…
We propose and experimentally demonstrate a scheme allowing to reach noncollinear phase-matching of high harmonic generation in solids, which may potentially lead to an enhancement of the generation efficiency. The principle is based on…
Nonlinear light-matter interaction and, in particular, high-harmonic generation (HHG) are fundamentally interesting and frequently discussed as versatile probes of quantum materials with potential for optical information processing…
We report here on results of experimental-theoretical investigation of high-order harmonic generation (HHG) in layers of CdSe semiconductor quantum dots of different sizes and a reference bulk CdSe thin film. We observe a strong decrease in…