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Attosecond chemistry involves developing strategies to manipulate electronic coherent waves in molecules, which can influence the outcome of photoinduced reactions. While recent progress in this field calls for investigations of…

Chemical Physics · Physics 2026-04-22 Evan Munaro-Langloÿs , Franck Lépine , Victor Despré

Collective electron dynamics in plasmonic nanosystems can unfold on timescales in the attosec- ond regime and the direct measurements of plasmonic near-field oscillations is highly desirable. We report on numerical studies on the…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Frederik Süßmann , Matthias F. Kling

We theoretically analyse an autonomous clock comprising a nanoelectromechanical system, which undergoes self-oscillations driven by electron tunnelling. The periodic mechanical motion behaves as the clockwork, similar to the swinging of a…

Quantum Physics · Physics 2024-03-06 Oisin Culhane , Michael J. Kewming , Alessandro Silva , John Goold , Mark T. Mitchison

Electrons in atoms and molecules can not react immediately to the action of intense laser field. A time lag (about 100 attoseconds) between instants of the field maximum and the ionization-rate maximum emerges. This lag characterizes the…

Atomic Physics · Physics 2021-04-01 J. Y. Che , C. Chen , S. Wang , G. G. Xin , Y. J. Chen

We analyze the attosecond electron dynamics in hydrogen molecular ion driven by an external intense laser field using ab-initio numerical simulations of the corresponding time-dependent Schr{\"{o}}dinger equation and Bohmian trajectories.…

Chemical Physics · Physics 2015-05-20 Norio Takemoto , Andreas Becker

The coupling of electronic and nuclear motion in polyatomic molecules is at the heart of attochemistry. The molecular properties, transient structures and reaction mechanism of these many-body quantum objects are defined on the level of…

Chemical Physics · Physics 2024-03-12 David Schwickert , Andreas Przystawik , Dian Diaman , Detlef Kip , Jon P. Marangos , Tim Laarmann

Attosecond science is well developed for atoms and promising results have been obtained for molecules and solids. Here, we review the first steps in developing attosecond time-resolved measurements in liquids. These advances provide access…

Other Condensed Matter · Physics 2020-09-11 H. J. Wörner , A. Schild , D. Jelovina , I. Jordan , C. Perry , T. T. Luu , Z. Yin

High harmonic light sources make it possible to access attosecond time-scales, thus opening up the prospect of manipulating electronic wave packets for steering molecular dynamics. However, two decades after the birth of attosecond physics,…

Measuring and controlling the ionization dynamics by intense laser fields has recently led to important breakthroughs, from the investigation of tunneling time delays to attosecond molecular imaging by electron holography. In these…

The present review addresses the technical advances and the theoretical developments to realize and rationalize attosecond-science experiments that reveal a new dynamical time scale ($10^{-15}$-$10^{-18}$ s), with a particular emphasis on…

Chemical Physics · Physics 2020-02-07 Denitsa Baykusheva , Hans Jakob Wörner

Photoionization as a half-scattering process is not instantaneous. Usually, time delays in photoionization are of the order of few tens of attoseconds (1 as = 10$^{-18}$ s). While going from a single atom to a nano-object, one can expect…

Irrotational ow of a spherical thin liquid layer surrounding a rigid core is described using the defocusing nonlinear Schrodinger equation. Accordingly, azimuthal moving nonlinear waves are modeled by periodic dark solitons expressed by…

Pattern Formation and Solitons · Physics 2021-08-04 A. S. Carstea , A. Ludu

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso

Recent experiments on measuring time-delays during tunnelling of cold atoms through an optically created potential barrier are reinvigorating the controversial debate regarding possible time-delays during light-induced tunnelling of an…

Attosecond angular streaking measurements have revealed deep insights into the timing of tunnel ionization processes of atoms in intense laser fields. So far experiments of this type have been performed only with a cold-target recoil-ion…

Atomic Physics · Physics 2013-10-21 Matthias Weger , Jochen Maurer , André Ludwig , Lukas Gallmann , Ursula Keller

The present work focuses on the characterisation of the amount of orbital angular momentum (OAM) encoded in the twisted attosecond pulses via energy- and angle-resolved attosecond streaking in pump-probe setup. It is found that the…

Atomic Physics · Physics 2020-06-03 Irfana N. Ansari , Deependra S. Jadoun , Gopal Dixit

In the semiclassical picture of photoionization process in intense laser fields, the ionization rate solely depends on the amplitude of the electric field and the final photoelectron momentum corresponds to the instant of ionization of the…

Atomic Physics · Physics 2019-05-09 Li Guo , Shilin Hu , Mingqing Liu , Zheng Shu , Xiwang Liu , Jie Li , Weifeng Yang , Ronghua Lu , Shensheng Han , Jing Chen

High-precision hydrogen spectroscopy is an active field which helps to determine the Rydberg constant and proton charge radius, tests bound-state QED, and can search for Beyond Standard Model (BSM) Physics. Additionally, with recent…

Atomic Physics · Physics 2022-06-15 S. F. Cooper , C. Rasor , R. G. Bullis , A. D. Brandt , D. C. Yost