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Phonon dispersion is widely used to elucidate the vibrational properties of materials. As an emerging technique, momentum-resolved vibrational spectroscopy in scanning transmission electron microscopy (STEM) offers an unparalleled approach…

Materials Science · Physics 2024-06-07 Aowen Li , Paul Zeiger , Zuxian He , Mingquan Xu , Stephen J. Pennycook , Ján Rusz , Wu Zhou

Direct measurement of local phonon dispersion in individual nanostructures can greatly advance our understanding of their electrical, thermal, and mechanical properties. However, such experimental measurements require extremely high…

Mesoscale and Nanoscale Physics · Physics 2021-03-02 Ruishi Qi , Ning Li , Jinlong Du , Ruochen Shi , Yang Huang , Xiaoxia Yang , Lei Liu , Zhi Xu , Qing Dai , Dapeng Yu , Peng Gao

The phonon dispersions of monolayer and few-layer graphene (AB bilayer, ABA and ABC trilayers) are investigated using the density-functional perturbation theory (DFPT). Compared with the monolayer, the optical phonon $E_{2g}$ mode at…

Materials Science · Physics 2009-11-13 Jia-An Yan , W. Y. Ruan , M. Y. Chou

The unique optical properties of graphene, with broadband absorption and ultrafast response, make it a critical component of optoelectronic and spintronic devices. Using time-resolved momentum microscopy with high data rate and high dynamic…

Transition metal dichalcogenide monolayers and heterostructures are highly tunable material systems that provide excellent models for physical phenomena at the two-dimensional (2D) limit. While most studies to date have focused on electrons…

The breakdown of translational symmetry at heterointerfaces leads to the emergence of new phonon modes localized near the interface. These interface phonons play an essential role in thermal/electrical transport properties in devices…

Materials Science · Physics 2022-01-05 Ruishi Qi , Ruochen Shi , Yuanwei Sun , Yuehui Li , Mei Wu , Ning Li , Jinlong Du , Kaihui Liu , Chunlin Chen , Dapeng Yu , En-Ge Wang , Peng Gao

The interaction of graphene with metallic substrates reveals phenomena and properties of great relevance for applications in nanotechnology. In this review, the vibrational characterization by means of various inelastic scattering…

Materials Science · Physics 2016-01-08 Antonio Politano

While phonons and their related properties have been studied comprehensively in bulk materials, a thorough understanding of surface phonons for nanoscale objects remains elusive. Infra-red imaging methods with photons or electrons exist,…

Instrumentation and Detectors · Physics 2021-04-21 Xiaoyan Li , Georg Haberfehlner , Ulrich Hohenester , Odile Stéphan , Gerald Kothleitner , Mathieu Kociak

The electron-phonon interaction in monolayer graphene is investigated by using density functional perturbation theory. The results indicate that the electron-phonon interaction strength is of comparable magnitude for all four in-plane…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 K. M. Borysenko , J. T. Mullen , E. A. Barry , S. Paul , Y. G. Semenov , J. M. Zavada , M. Buongiorno Nardelli , K. W. Kim

Raman spectroscopy has become an essential technique to characterize and investigate graphene and many other two-dimensional materials. However, there still lacks consensus on the Raman signature and phonon dispersion of atomically thin…

We investigate the long-wavelength dispersion of longitudinal and transverse optical phonon modes in polar two-dimensional materials, multilayers, and their heterostructures. Using analytical models and density-functional perturbation…

Materials Science · Physics 2017-08-02 Thibault Sohier , Marco Gibertini , Matteo Calandra , Francesco Mauri , Nicola Marzari

The interplay between substrate interactions and electron-phonon coupling in two-dimensional (2D) materials presents a significant challenge in understanding and controlling their electronic properties. Here, we present a comparative study…

Materials Science · Physics 2025-01-15 Amjad Al Taleb , Wen Wan , Giorgio Benedek , Miguel M. Ugeda , Daniel Farías

The properties of pristine, free-standing graphene monolayers prepared by mechanical exfoliation of graphite are investigated. The graphene monolayers, suspended over open trenches, are examined by means of spatially resolved Raman…

Materials Science · Physics 2009-01-08 Stephane Berciaud , Sunmin Ryu , Louis E. Brus , Tony F. Heinz

The electronic and vibrational properties of 2D materials are dramatically altered by the formation of a moir\'e superlattice. The lowest-energy phonon modes of the superlattice are two acoustic branches (called phasons) that describe the…

Spectroscopies utilizing free electron beams as probes offer detailed information on the reciprocal-space excitations of 2D materials such as graphene and transition metal dichalcogenide monolayers. Yet, despite the attention paid to such…

Materials Science · Physics 2024-02-08 Andrew W. Rossi , Marc R. Bourgeois , Caleb Walton , David J. Masiello

Quantised lattice vibrations (i.e., phonons) in solids are robust and unambiguous fingerprints of crystal structures and of their symmetry properties. In metals and semimetals, strong electron-phonon coupling may lead to so-called Kohn…

We carried out measurements on nanoelectromechanical systems based on multilayer graphene sheets suspended over trenches in silicon oxide. The motion of the suspended sheets was electrostatically driven at resonance using applied…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 D. Garcia-Sanchez , A. M. van der Zande , A. San Paulo , B. Lassagne , P. L. McEuen , A. Bachtold

The enormous stiffness and low density of graphene make it an ideal material for nanoelectromechanical (NEMS) applications. We demonstrate fabrication and electrical readout of monolayer graphene resonators, and test their response to…

Van der Waals materials and their heterostructures offer a versatile platform for studying a variety of quantum transport phenomena due to their unique crystalline properties and the exceptional ability in tuning their electronic spectrum.…

Mesoscale and Nanoscale Physics · Physics 2019-08-05 P. Kumaravadivel , M. T. Greenaway , D. Perello , A. Berdyugin , J. Birkbeck , J. Wengraf , S. Liu , J. H. Edgar , A. K. Geim , L. Eaves , R. Krishna Kumar

Properties of phonons - quanta of the crystal lattice vibrations - in graphene have attracted strong attention of the physics and engineering communities. Acoustic phonons are the main heat carriers in graphene near room temperature while…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Denis L. Nika , Alexander A. Balandin
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