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Ba2YIrO6, a Mott insulator, with four valence electrons in Ir5+ d-shell (5d4) is supposed to be non-magnetic, with Jeff = 0, within the atomic physics picture. However, recent suggestions of non-zero magnetism have raised some fundamental…

Strongly Correlated Electrons · Physics 2019-01-03 Birender Singh , G. A. Cansever , T. Dey , A. Maljuk , S. Wurmehl , B. Büchner , Pradeep Kumar

We present a systematic study of the structure and lattice dynamics at room temperature, and the phonon behavior at low temperatures in orthorhombic Gd$_{1-x}$Y$_{x}$MnO$_{3}$ manganites, with 0 $\leq$ x $\leq$ 0.4, using powder x-ray…

Strongly Correlated Electrons · Physics 2014-12-31 R. Vilarinho , E. C. Queirós , A. Almeida , P. B. Tavares , J. Agostinho Moreira

We analyze the temperature dependence of the electron spin resonance linewidth above the critical region in exchange-coupled magnetic insulators. The focus is on separating the contributions to the linewidth from spin-spin interactions,…

Materials Science · Physics 2017-06-27 M. Acikgoz , D. L. Huber

We present the Raman scattering results on layered 2D semiconducting ferromagnetic compound CrSiTe$_3$. Four Raman active modes, predicted by symmetry, have been observed and assigned. The experimental results are supported by DFT…

Materials Science · Physics 2018-10-16 A. Milosavljević , A. Šolajić , J. Pešić , Yu Liu , C. Petrovic , N. Lazarević , Z. V. Popović

Polarization- and temperature-dependent Raman data along with theoretical simulations are presented for the Kagome ferromagnet Fe_3Sn_2. Eight out of nine expected phonon modes were identified. The experimental energies compare well with…

Spin-phonon coupling originated from spin-lattice correlation depends upon different exchange interactions in transition metal oxides containing 3d magnetic ions. Spin-lattice coupling can influence the coupling mechanism in magnetoelectric…

Strongly Correlated Electrons · Physics 2021-09-09 P. Pal , Shalini Badola , P. K. Biswas , Ranjana R. Das , Surajit Saha , S. D. Kaushik , P. N. Vishwakarma , A. K. Singh

Inelastic light scattering studies on single crystal of electron-doped Ca(Fe0.95Co0.05)2As2 superconductor, covering the tetragonal to orthorhombic structural transition as well as magnetic transition at TSM ~ 140 K and superconducting…

We perform thermodynamic and inelastic neutron scattering (INS) measurements to study the lattice dynamics (phonons) of a cubic collinear antiferromagnet Cu$_3$TeO$_6$ which hosts topological spin excitations (magnons). While the specific…

The interplay between spin dynamics and lattice vibration has been suggested as an important part of the puzzle of high-temperature superconductivity. Here we report the strong interaction between spin fluctuation and phonon in SmFeAsO, a…

Superconductivity · Physics 2010-10-29 L. Zhang , P. F. Guan , D. L. Feng , X. H. Chen , S. S. Xie , M. W. Chen

We employ an optical pump-probe technique to study coherent phonon oscillations in Ca$_2$RuO$_4$. We find that oscillation-amplitude of an $A_g$ symmetric phonon mode is strongly suppressed at 260 K, a putative transition point of orbital…

Strongly Correlated Electrons · Physics 2018-10-24 Min-Cheol Lee , Choong H. Kim , Inho Kwak , J. Kim , S. Yoon , Byung Cheol Park , Bumjoo Lee , F. Nakamura , C. Sow , Y. Maeno , T. W. Noh , K. W. Kim

We report on the temperature dependent Raman spectroscopic studies of orthorombic distorted perovskite YCrO3 in the temperature range of 20-300K. Temperature dependence of DC-magnetization measurement under field cooled and zero field…

Materials Science · Physics 2013-09-30 Yogesh Sharma , Satyaprakash Sahoo , W. Perez , Ram S. Katiyar

MnV$_2$O$_4$ in the spinel structure is known to exhibit coupled orbital and spin ordering, and its Raman spectra show interesting anomalies in its low-temperature phase. With a goal to explain this behavior involving coupled spins and…

Materials Science · Physics 2020-05-27 Dibyendu Dey , T. Maitra , U. V. Waghmare , A. Taraphder

Utilizing magnetic susceptibility, specific heat, thermal expansion and IR spectroscopy we provide experimental evidence that the two subsequent antiferromagnetic transitions in ZnCr_2S_4 at T_N1 = 15 K and T_N2= 8 K are accompanied by…

Strongly Correlated Electrons · Physics 2009-11-11 J. Hemberger , T. Rudolf , H. -A. Krug von Nidda , F. Mayr , A. Pimenov , V. Tsurkan , A. Loidl

The detailed temperature dependence of the infrared-active mode in Fe$_{1.03}$Te ($T_N\simeq 68$ K) and Fe$_{1.13}$Te ($T_N\simeq 56$ K) has been examined, and the position, width, strength, and asymmetry parameter determined using an…

Strongly Correlated Electrons · Physics 2016-05-18 C. C. Homes , Y. M. Dai , J. Schneeloch , R. D. Zhong , G. D. Gu

Dynamical correlations of Jeff = 1/2 isospins in the paramagnetic state of spin-orbital Mott insu- lator Sr2IrO4 was revealed by resonant magnetic x-ray diffuse scattering. We found two-dimensional antiferromagnetic fluctuation with a large…

Strongly Correlated Electrons · Physics 2015-06-04 S. Fujiyama , H. Ohsumi , T. Komesu , J. Matsuno , B. J. Kim , M. Takata , T. Arima , H. Takagi

Direct experimental evidence of spin-phonon coupling in CrSBr is provided by the temperature dependent Cr L-edge resonant inelastic x-ray scattering (RIXS) spectra. Zone-center optical phonons are observed exclusively in the low-temperature…

Sr2IrO4 exhibits a novel insulating state assisted by spin-orbit interactions. A series of polycrystalline samples of Sr2-xIrO4 have been synthesized. It is found that deep Sr-vacancies of Sr2-xIrO4 greatly reduce the rotation of IrO6…

Strongly Correlated Electrons · Physics 2016-11-01 Xuanyong Sun , S. L. Liu , Haiyun Wang , Bin Li , Jie Cheng , Z. H. Wang

The collective magnetic excitations in the spin-orbit Mott insulator (Sr$_{1-x}$La$_x$)$_2$IrO$_4$ ($x=0,\,0.01,\,0.04,\, 0.1$) were investigated by means of resonant inelastic x-ray scattering. We report significant magnon energy gaps at…

Spin-orbit interaction in Sr$_2$IrO$_4$ leads to the realization of the $J_{\mathrm{eff}}$ = 1/2 state and also induces an insulating behavior. Using large-shift Raman spectroscopy, we found two high-energy excitations of the d-shell…

Strongly Correlated Electrons · Physics 2015-07-15 Jhih-An Yang , Yi-Ping Huang , Michael Hermele , Tongfei Qi , Gang Cao , Dmitry Reznik

We report inelastic light scattering studies on Ca(Fe0.97Co0.03)2As2 in a wide spectral range of 120-5200 cm-1 from 5K to 300K, covering the tetragonal to orthorhombic structural transition as well as magnetic transition at Tsm ~ 160K. The…

Superconductivity · Physics 2014-07-11 Pradeep Kumar , D. V. S. Muthu , L. Harnagea , S. Wurmehl , B. Büchner , A. K. Sood