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Quantum-inspired superresolution methods surpass the Rayleigh limit in imaging, or the analogous Fourier limit in spectroscopy. This is achieved by carefully extracting the information carried in the emitted optical field by engineered…

We describe numerically the ionization process induced by linearly and circularly polarized XUV attosecond laser pulses on an aligned atomic target, specifically, the excited state…

Atomic Physics · Physics 2021-05-26 Juan J. Omiste , Lars Bojer Madsen

We study population distributions and lasing actions of N_2^+ driven by femtosecond lasers with various wavelengths, and uncover an efficient ionic excitation mechanism induced by synchronized ionization and multiphoton resonance. Our…

Air-lasing from single ionized N$_2^+$ molecules induced by laser filamentation in air has been intensively investigated and the mechanisms responsible for lasing are currently highly debated. We use ultrafast nitrogen K-edge spectroscopy…

Recolliding electrons are responsible for many of the interesting phenomena observed in the interaction of strong laser fields with atoms and molecules. We show that in multielectron targets such as C60 a new important recollision pathway…

Atomic Physics · Physics 2009-11-13 M. Ruggenthaler , S. V. Popruzhenko , D. Bauer

A single-photon Fock state has been generated by means of conditional preparation from a two-photon state emitted in the process of spontaneous parametric down-conversion. A recently developed high-frequency homodyne tomography technique…

Quantum Physics · Physics 2007-05-23 Alessandro Zavatta , Silvia Viciani , Marco Bellini

A femtosecond frequency-doubled Erbium-doped fiber laser with adjustable pulse repetition rate is developed and applied in two-photon excited fluorescence microscopy. The all-fiber laser system provides the fundamental pulse at 1560 nm…

We propose a general technique to retrieve the information of dipole-forbidden resonances in the autoionizing region. In the simulation, a helium atom is pumped by an isolated attosecond pulse in the extreme ultraviolet (EUV) combined with…

Atomic Physics · Physics 2014-03-28 Wei-Chun Chu , Toru Morishita , C. D. Lin

In molecular aggregates, multiple delocalized exciton states interact with phonons, making the state-resolved spectroscopic monitoring of dynamics challenging. We propose a protocol that combines photon-entanglement-enhanced narrowband…

Quantum Physics · Physics 2026-04-24 Arunangshu Debnath , Shaul Mukamel

Photo-induced phase transitions have been intensively studied owing to the ability to control a material of interest in the ultrafast manner, which can induce exotic phases unable to be attained at equilibrium. However, the key mechanisms…

We report fully differential photoelectron spectra from an {\it ab-inito} coupled channels treatment of CO$_2$. Photoionization by laser pulses centered at 400 nm and 800 nm wavelength are considered, with arbitrary molecular alignment and…

Atomic Physics · Physics 2017-09-05 Vinay Pramod Majety , Armin Scrinzi

We study spectroscopy of artificial solid-state four-level quantum system. This system is formed by two coupled superconducting flux qubits. When multiple driving frequency of the applied microwaves matches the energy difference between any…

We report on high resolution Fourier-transform spectroscopy of fluorescence to the a^3\Sigma_u^+ state excited by two-photon or two-step excitation from the X^1\Sigma_g^+ state to the 2^3\Pi_g state in the molecule K_2. These spectroscopic…

Atomic Physics · Physics 2009-11-13 A. Pashov , P. Popov , H. Knöckel , E. Tiemann

We develop a new method for high-precision tomography of ion qubit registers under conditions of limited distinguishability of its logical states. It is not always possible to achieve low error rates during the readout of the quantum states…

Quantum Physics · Physics 2023-07-07 Yu. I. Bogdanov , I. A. Dmitriev , B. I. Bantysh , N. A. Bogdanova , V. F. Lukichev

The single-electron energy and static charge-lattice deformation correlations have been calculated for the first excited state of a two-site Holstein model within perturbative expansions using different standard phonon bases obtained…

Condensed Matter · Physics 2009-10-31 Jayita Chatterjee , A. N. Das

Until recently it was believed that photosynthesis, a fundamental process for life on earth, could be fully understood with semi-classical models. However, puzzling quantum phenomena have been observed in several photosynthetic…

Time- and angle-resolved photoelectron spectroscopy with 13 fs temporal resolution is used to follow the different stages in the formation of a Fermi-Dirac distributed electron gas in graphite after absorption of an intense 7 fs laser…

The electronic and nuclear dynamics in methanol, following 156~nm photoexcitation, are investigated by combining a detailed analysis of time-resolved photoelectron spectroscopy experiments with electronic structure calculations. The…

Time- and angle-resolved photoemission spectroscopy has played an important role in revealing the non-equilibrium electronic structures of solid-state materials. The implementation of high harmonic generation to obtain a higher photon…

Strongly Correlated Electrons · Physics 2022-06-29 Takeshi Suzuki , Shik Shin , Kozo Okazaki

Precision spectroscopy of atomic and molecular ions offers a window to new physics, but is typically limited to species with a cycling transition for laser cooling and detection. Quantum logic spectroscopy has overcome this limitation for…