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We present the structural, magnetic, thermal and ab-plane electronic transport properties of single crystals of CaCu1.7As2 grown by the self-flux technique that were investigated by powder x-ray diffraction, magnetic susceptibility chi,…

Superconductivity · Physics 2013-08-20 V. K. Anand , D. C. Johnston

Rare-earth pyrochlores are known to exhibit exotic magnetic phenomena. We report a study of crystal growth and characterizations of a new rare-earth compound Er$_2$AlSbO$_7$, in which Al$^{3+}$ and Sb$^{5+}$ ions share the same positions…

The oxide pyrochlore Bi$_2$Ti$_2$O$_7$ is in some ways analogous to perovskite PbTiO$_3$, in that Bi$_2$Ti$_2$O$_7$ has two cations, Bi$^{3+}$ and Ti$^{4+}$ in oxidation states that are normally associated with a propensity to off-center.…

Materials Science · Physics 2007-12-13 Craig J. Fennie , Ram Seshadri , Karin M. Rabe

Single crystals of KOs2O6 have been grown in a sealed quartz ampoule. Detailed single crystal X-ray diffraction studies at room temperature show Bragg peaks that violate Fd-3m symmetry. With a comparative structure refinement the structure…

Superconductivity · Physics 2009-11-11 G. Schuck , S. M. Kazakov , K. Rogacki , N. D. Zhigadlo , J. Karpinski

The structural and electrical properties of Ti-N films deposited by reactive sputtering depend on their growth parameters, in particular the Ar:N2 gas ratio. We show that the nitrogen percentage changes the crystallographic phase of the…

We report the growth of single crystals of SrCu2As2, SrCu2Sb2, SrCu2(As{0.84}Sb{0.16})2 and BaCu2Sb2 using the self-flux technique and their structural, magnetic, thermal and transport properties that were investigated by powder x-ray…

Superconductivity · Physics 2012-09-11 V. K. Anand , P. Kanchana Perera , Abhishek Pandey , R. J. Goetsch , A. Kreyssig , D. C. Johnston

The phonon and crystal field excitations in several rare earth titanate pyrochlores are investigated. Magnetic measurements on single crystals of Gd2Ti2O7, Tb2Ti2O7, Dy2Ti2O7 and Ho2Ti2O7 are used for characterization, while Raman…

We have measured neutron diffraction patterns in a single crystal sample of the pyrochlore compound Er$_2$Ti$_2$O$_7$ in the antiferromagnetic phase (T=0.3\,K), as a function of the magnetic field, up to 6\,T, applied along the [110]…

Strongly Correlated Electrons · Physics 2015-05-19 H. B. Cao , I. Mirebeau , A. Gukasov , P. Bonville , C. Decorse

Lithium doped sodium niobate is an ecofriendly piezoelectric material that exhibits a variety of structural phase transitions with composition and temperature. We have investigated the phase stabilities of an important composition…

The magnetization, crystal structure, and thermal expansion of a nearly stoichiometric Sr$_{1.04(3)}$Er$_{2.09(6)}$O$_{4.00(1)}$ single crystal have been studied by PPMS measurements and in-house and high-resolution synchrotron X-ray powder…

Strongly Correlated Electrons · Physics 2014-10-27 Hai-Feng Li , Andrew Wildes , Binyang Hou , Cong Zhang , Berthold Schmitz , Paul Meuffels , Georg Roth , Thomas Brückel

We report structural and magnetic properties studies of large high quality single-crystals of the frustrated magnet, Nd$_2$Zr$_2$O$_7$. Powder x-ray diffraction analysis confirms that Nd$_2$Zr$_2$O$_7$ adopts the pyrochlore structure.…

Strongly Correlated Electrons · Physics 2015-05-18 M. Ciomaga Hatnean , M. R. Lees , O. A. Petrenko , D. S. Keeble , G. Balakrishnan , M. J. Gutmann , V. V. Klekovkina , B. Z. Malkin

We report a structural and thermodynamic study of the "stuffed spin ice" material Ho2TiO5 (i.e., Ho2(Ti1.33Ho0.67)O6.67), comparing samples synthesized through two different routes. Neutron powder diffraction and electron diffraction reveal…

Materials Science · Physics 2009-11-13 G. C. Lau , B. G. Ueland , M. L. Dahlberg , R. S. Freitas , Q. Huang , H. W. Zandbergen , P. Schiffer , R. J. Cava

Thin films of phase pure pyrochlore Gd2Ti2O7 have been synthesized by RF magnetron sputtering. The films were prepared from oxide targets in 50%O2/Ar atmosphere and deposited on 111 YSZ substrates at a temperature of 800C. The pyrochlore…

In terms of a semi-phenomenological exchange charge model, we have obtained estimates of parameters of the crystal field and parameters of the electron-deformation interaction in terbium titanate Tb2Ti2O7 with a pyrochlore structure. The…

Strongly Correlated Electrons · Physics 2014-06-17 Vera Klekovkina , Boris Malkin

The Mott-insulating rare-earth titanates (RTiO$_3$, R being a rare-earth ion) are an important class of materials that encompasses interesting spin-orbital phases as well as ferromagnet-antiferromagnet and insulator-metal transitions. The…

Little is so far known about the magnetism of the $\rm A_2B_2O_7$ monoclinic layered perovskites that replace the spin-ice supporting pyrochlore structure for $r_A/r_B>1.78$. We show that high quality monoclinic Pr$_2$Ti$_2$O$_7$ single…

A2Ir2O7 iridates were proven to crystallise in the geometrically frustrated pyrochlore structure, which remains stable upon rare-earth cation substitution, temperature variation, and external pressure application. However, the change of…

Strongly Correlated Electrons · Physics 2024-08-05 Daniel Staško , Petr Proschek , Jiří Prchal , Milan Klicpera

We report an extensive study on the zero field ground state of a powder sample of the pyrochlore $\mathrm{Yb_2Ti_2O_7}$. A sharp heat capacity anomaly that labels a low temperature phase transition in this material is observed at 280 mK.…

Thermal decomposition behaviors of TiH2 powder under a flowing helium atmosphere and in a low vacuum condition have been studied by using in-situ EXAFS technique. By an EXAFS analysis containing the multiple scattering paths including H…

Materials Science · Physics 2015-06-17 Ying-Li Zhou , Li-Rong Zheng , Sheng-Qi Chu , Min Wu , Peng-Fei An , Jing Zhang , Tian-Dou Hu

The single crystal growth, structure, and basic magnetic properties of ErMgGaO4 are reported. The structure consists of triangular layers of magnetic ErO6 octahedra separated by a double layer of randomly occupied non-magnetic (Ga,Mg)O5…

Materials Science · Physics 2018-10-16 F. Alex Cevallos , Karoline Stolze , Robert J. Cava