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Related papers: Halide perovskites: Is it all about the interfaces…

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We report a study on the interface between polar high-k materials and the Si(001)-(2X1) reconstructed surface with LaAlO3 taken as a prototype material. The construction of the interface is based on the prior growth of metal lines followed…

Materials Science · Physics 2015-06-25 Isabelle Devos , Pierre Boulenc

The low ionization energy of an $A$ site molecule is a very important factor, which determines the thermodynamical stability of $A$PbI$_3$ hybrid halide perovskites, while the size of the molecule governs the stable phase at room…

Materials Science · Physics 2018-02-13 Chao Zheng , Oleg Rubel

The defect-activity in halide perovskites remains a critical factor for the application in optoelectronics. The imperfections (vacancies, anti-sites, interstitials) formed in the lattice of the halide perovskites were considered as a main…

As single junction thin-film technologies, both Si heterojunction (HIT) and Perovskite based solar cells promise high efficiencies at low cost. One expects that a tandem cell design with these cells connected in series will improve the…

General Physics · Physics 2015-07-02 Reza Asadpour , Raghu V. K. Chavali , M. Ryyan Khan , Muhammad A. Alam

Perovskites are promising next-generation absorber materials for low-cost and high-efficiency solar cells. Although perovskite cells are configured similar to the classical solar cells, their operation is unique and requires development of…

Mesoscale and Nanoscale Physics · Physics 2018-02-01 Xingshu Sun , Reza Asadpour , Wanyi Nie , Aditya D. Mohite , Muhammad A. Alam

With the rapid evolution of lead halide perovskite solar cells, there are considerable evidences that the mobile ions strongly impact their properties. However, except the activation energy, the other properties of ionic migration are…

Materials Science · Physics 2018-06-21 Ningbo Yi , Gang Li , Yuhan Wang , Shuai Wang , Kaiyang Wang , Qinghai Song , Shumin Xiao

The buried interface between the electron transport layer and the perovskite layer suffers from severe interface defects and imperfect energy level alignment. To address this issue, this study employs a multifunctional organic molecule,…

Materials Science · Physics 2024-09-02 Xianhu Wu , Jieyu Bi , Guanglei Cu , Nian Liu , Gaojie Xia , Jilong Sun , Jiaxin Jiang , Ning Lu , Ping Li , Chunyi Zhao , Zewen Zuo , Min Gu

Organic-inorganic halide perovskites recently have emerged as a promising material for highly effective light-emitting diodes (LEDs) and solar cells (SCs). Despite efficiencies of both perovskite SCs and LEDs are already among the best, the…

Halide perovskites are a promising class of materials for optoelectronic and photovoltaic applications, exhibiting high power conversion efficiency due to strong light absorption and long carrier diffusion lengths. While various aspects of…

Metal halide perovskite semiconductors have outstanding optoelectronic properties. Although these perovskites are defect-tolerant electronically, defects hamper their long-term stability and cause degradation. Density functional theory…

Materials Science · Physics 2021-09-02 Haibo Xue , Geert Brocks , Shuxia Tao

Safe, all-solid-state lithium metal batteries enable high energy density applications, but suffer from instabilities during operation that lead to rough interfaces between the metal and electrolyte and subsequently cause void formation and…

Materials Science · Physics 2024-08-07 Salem Mosleh , Emil Annevelink , Venkatasubramanian Viswanathan , L. Mahadevan

A central goal of modern materials physics and nanoscience is control of materials and their interfaces to atomic dimensions. For interfaces between polar and non-polar layers, this goal is thwarted by a polar catastrophe that forces an…

Materials Science · Physics 2007-05-23 Naoyuki Nakagawa , Harold Y. Hwang , David A. Muller

SiC is set to enable a new era in power electronics impacting a wide range of energy technologies, from electric vehicles to renewable energy. Its physical characteristics outperform silicon in many aspects, including band gap, breakdown…

2D organic-inorganic hybrid perovskites (2DHPs) consist of alternating anionic metal-halide and cationic organic layers. They have widely tunable structural and optical properties. We review the role of the organic cation in defining the…

Materials Science · Physics 2022-04-28 Daniel B. Straus , Cherie R. Kagan

Microscopic pathways of structural phase transitions are difficult to probe because they occur over multiple, disparate time and length scales. Using $in$ $situ$ nanoscale cathodoluminescence microscopy, we visualize the thermally-driven…

Advances in photovoltaic technology are a viable route to contribute to cleaner and more sustainable energy solutions, placing perovskite-based materials among the best candidates for solar energy conversion. However, some challenges must…

At photoelectrosynthetic interfaces, an electrochemical reaction is driven by excited charge-carriers from a semiconducting photoabsorber. Structure and composition of this interface determine both the electronic and electrochemical…

Chemical Physics · Physics 2022-05-30 Matthias M. May , Wolfram Jaegermann

Halide perovskites belong to an important family of semiconducting materials with unique electronic properties that enable a myriad of applications, especially in photovoltaics and optoelectronics. Their optical properties, including…

GaP/Si(100) is considered as pseudomporphic virtual substrate for III/V-on-Si integration in order to reduce defects related to polar-on-nonpolar heteroepitaxy. The atomic structure of the GaP/Si(100) heterointerface is decisive to yield…

The last five years have witnessed a remarkable progress in the field of lead halide perovskite materials and devices. Examining the existing body of literature reveals staggering inconsistencies in the reported results among different…