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We report the enhancement of the optical second harmonic signal in non-centrosymmetric semiconductor CdS quantum dots, when they are placed in close contact with isolated silver nanoparticles. The intensity enhancement is about 1000. We…

Mesoscale and Nanoscale Physics · Physics 2012-02-15 Pablo M. Jais , Catalina von Bilderling , Andrea V. Bragas

We demonstrate generation and frequency doubling of unit charge vortices in a linear astigmatic resonator. Topological instability of the double charge harmonic vortices leads to well separated vortex cores that are shown to rotate, and…

Optics · Physics 2011-04-21 O-K Lim , B Boland , M Saffman , W. Krolikowski

We introduce a new mechanism for second-harmonic generation through geometrically rectifying-funneling-ballistic electrons in THz optical resonators. Our resonant rectifiers inherently act as second-order harmonic generators, rectifying…

Mesoscale and Nanoscale Physics · Physics 2025-05-01 Hue T. B. Do , Gregory K. Ngirmang , Wu Lin , Michel Bosman

The nonlinear process of second harmonic generation (SHG) in monolayer (1L) transition metal dichalcogenides (TMD), like $WS_2$, strongly depends on the polarization state of the excitation light. Combining plasmonic nanostructures with…

Optics · Physics 2021-10-08 Florian Spreyer , Claudia Ruppert , Philip Georgi , Thomas Zentgraf

Because of the importance of second harmonic generation in some nonlinear media, in this paper, we investigated induced second harmonic generation in diamond where there is no intrinsic second order susceptibility, X(2). The electric field…

Optics · Physics 2015-11-19 Mahboubeh Ghalandari

Second harmonic generation (SHG) is a nonlinear optical response arising exclusively from broken inversion symmetry in the electric-dipole limit. Recently, SHG has attracted widespread interest as a versatile and noninvasive tool for…

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

When a laser pulse impinges on a molecule which is invariant under certain symmetry operations selection rules for harmonic generation (HG) arise. In other words: symmetry controls which channels are open for the deposition and emission of…

Atomic Physics · Physics 2009-11-07 D. Bauer , F. Ceccherini

Lattice resonances in nanoparticle arrays recently have gained a lot of attention because of the possibility to produce spectrally narrow resonant features in transmission and reflection as well as significantly increase absorption in the…

Optics · Physics 2018-11-07 Viktoriia E. Babicheva , Andrey B. Evlyukhin

In this Letter, it is experimentally and theoretically shown that weak odd harmonics generated during the propagation of an infrared ultrashort ultra-intense pulse unexpectedly modify the nonlinear properties of the medium and lead to a…

Optics · Physics 2015-06-18 P. Béjot , G. Karras , F. Billard , E. Hertz , B. Lavorel , E. Cormier , O. Faucher

We study numerically the interaction between an intense circularly polarized laser field and an electron moving in a potential which has a discrete cylindrical symmetry with respect to the laser pulse propagation direction. This setup…

Atomic Physics · Physics 2009-11-07 F. Ceccherini , D. Bauer

We show that nonlinear multipolar interference allows achieving not only unidirectional, but also non-reciprocal nonlinear generation from a nanoelement, with the direction of the nonlinearly produced light decoupled from that of at least…

Optics · Physics 2015-10-13 Ekaterina Poutrina , Augustine Urbas

Nonlinear metasurfaces have become prominent tools for controlling and engineering light at the nanoscale. Usually, the polarization of the total generated third harmonic is studied. However, diffraction orders may present different…

On the basis of the Edward-Kornfeld formulation, we study the effective susceptibility of secondharmonic generation (SHG) in colloidal crystals, which are made of graded metallodielectric nanoparticles with an intrinsic SHG susceptibility…

Optics · Physics 2008-03-24 J. P. Huang , Y. C. Jian , C. Z. Fan , K. W. Yu

Plasmonic metasurfaces have emerged as a promising platform for enhancing a range of nonlinear optical processes, offering compact geometry and flexibility in light manipulation. Second order nonlinear processes, like second harmonic…

We employ transformation optics to optimize the generic nonlinear wave interaction of second-harmonic generation from a pair of touching metallic wires. We demonstrate a 10 orders of magnitude increase in the second-harmonic scattering…

Optical materials with centrosymmetry, such as silicon and germanium, are unfortunately absent of second-order nonlinear optical responses, hindering their developments in efficient nonlinear optical devices. Here, a design with an array of…

Optics · Physics 2022-06-17 C. Fang , Q. Yang , Q. Yuan , L. Gu , X. Gan , Y. Shao , Y. Liu , G. Han , Y. Hao

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

Atomic Physics · Physics 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

We have investigated second harmonic generation (SHG) from Ag-coated LiNbO3 (LN) core-shell nanocuboids and found that giant SHG can occur via deliberately designed double plasmonic resonances. By controlling the aspect ratio, we can tune…

Optics · Physics 2014-11-19 Ming-Liang Ren , Si-Yuan Liu , Ben-Li Wang , Bao-Qin Chen , Jiafang Li , Zhi-Yuan Li

High-order harmonic generation by a bicircular field, which consists of two coplanar counter-rotating circularly polarized fields of frequency $r\omega$ and $s\omega$ ($r$ and $s$ are integers), is investigated for a polyatomic molecule.…

Atomic Physics · Physics 2016-10-05 Senad Odžak , Elvedin Hasović , Dejan B. Milošević