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A first-principles-derived approach is developed to study the effects of uncompensated depolarizing electric fields on the properties of Pb(Zr,Ti)O$_3$ ultrathin films for different mechanical boundary conditions. A rich variety of…

Materials Science · Physics 2009-11-10 Igor Kornev , Huaxiang Fu , L. Bellaiche

We consider an equation modeling the evolution of a viscous liquid thin film wetting a horizontal solid substrate destabilized by an electric field normal to the substrate. The effects of the electric field are modeled by a lower order…

Analysis of PDEs · Mathematics 2012-07-03 Cyril Imbert , Antoine Mellet

The depolarization fields set up to due to uncompensated surface charges in a ferroelectric thin film can suppress the ferroelectric phase below a critical size. Recent experiments show that 180 degree domain structures can help to…

Materials Science · Physics 2007-05-23 Rajeev Ahluwalia , David J. Srolovitz

Strain engineering of perovskite oxide thin films has proven to be an extremely powerful method for enhancing and inducing ferroelectric behavior. In ferroelectric thin films and superlattices, the polarization is intricately linked to…

In epitaxially strained ferroelectric thin films and superlattices, the ferroelectric transition temperature can lie above the growth temperature. Ferroelectric polarization and domains should then evolve during the growth of a sample, and…

We present a theoretical description of the influence of misfit strain on mobile defects dynamics in thin strained ferroelectric films. Self-consistent solutions obtained by coupling the Poissons equation for electric potential with…

The transient acoustic response of a free-standing, polycrystalline thin Au film upon femtosecond optical excitation has been studied by time-resolved Debye-Scherrer X-ray diffraction using ultrashort Cu K$_{\alpha}$ X-ray pulses from a…

Mesoscale and Nanoscale Physics · Physics 2019-12-11 W. Lu , M. Nicoul , U. Shymanovich , F. Brinks , M. Afshari , A. Tarasevitch , D. von der Linde , K. Sokolowski-Tinten

Exploiting the emerging nanoscale periodicities in epitaxial, single-crystal thin films is an exciting direction in quantum materials science: confinement and periodic distortions induce novel properties. The structural motifs of interest…

The transmission and reflection spectra from a right-handed chiral sculptured zirconia thin film are calculated using the coupled wave theory and the Bruggeman homogenization formalism in conjunction with the experimental data for the…

Optics · Physics 2009-03-17 Ferydon Babaei , Hadi Savaloni

We report first-principle atomistic simulations on the effect of local strain gradients on the nanoscale domain morphology of free-standing PbTiO$_3$ ultrathin films. First, the ferroelectric properties of free films at the atomic level are…

Materials Science · Physics 2015-06-22 G. D. Belletti , S. D. Dalosto , Silvia Tinte

We present the first analytical study of phase transitions in ferroelastic-ferroelectric epitaxial thin films on exactly solvable model. The emerging domain structure with domains of equal width (which may be exponentially large on a "soft"…

Statistical Mechanics · Physics 2009-10-31 A. M. Bratkovsky , A. P. Levanyuk

The time evolution of the electron density and the resulting time dependence of X-ray diffraction peak intensity in a crystal irradiated by highly intense femtosecond pulses of an XFEL is investigated theoretically on the basis of rate…

Atomic Physics · Physics 2013-11-26 A. Leonov , D. Ksenzov , A. Benediktovitch , I. Feranchuk , U. Pietsch

The effect of polarization fatigue on the Rayleigh coefficients of ferroelectric lead zirconate titanate (PZT) thin film was systematically investigated. It was found that electrical fatigue strongly affects the Rayleigh behaviour of the…

Materials Science · Physics 2015-06-19 X. J. Lou , H. J. Zhang , Z. D. Luo , F. P. Zhang , Y. Liu , Q. D. Liu , A. P. Fang , B. Dkhil , M. Zhang , X. B. Ren , H. L. He

Many ferroelectric devices are based on doped lead zirconate titanate (PZT) ceramics with compositions near the morphotropic phase boundary (MPB), at which the relevant material's properties approach their maximum. Based on a synchrotron…

We construct a comprehensive theory of the electrodynamic response of ferroelectric ultra-thin films containing periodic domain textures (PDT) with 180{\deg} polarization-oriented domains. The focal point of the theory is the…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 I. Luk'yanchuk , A. Sené , V. Vinokour

We present simulations of Bragg Coherent X-ray Diffractive Imaging (CXDI) data from finite crystals in the frame of the dynamical theory of x-ray diffraction. The developed approach is based on numerical solution of modified Takagi-Taupin…

Materials Science · Physics 2017-08-30 A. G. Shabalin , O. M. Yefanov , V. L. Nosik , V. A. Bushuev , I. A. Vartanyants

The spatiotemporal response of crystals in x-ray Bragg diffraction resulting from excitation by an ultra-short, laterally confined x-ray pulse is studied theoretically. The theory presents an extension of the analysis in symmetric…

Optics · Physics 2012-10-22 Yuri Shvyd'ko , Ryan Lindberg

Using resonant soft X-ray techniques we follow the magnetic behavior of a strained epitaxial film of CoCr2O4, a type-II multiferroic. The film is [110]-oriented, such that both the ferroelectric and ferromagnetic moments can coexist in…

Domain wall dynamics in ferromagnets is complicated by internal degrees of freedom of the domain walls. We develop a model of domain walls in disordered thin films with perpendicular magnetic anisotropy capturing such features, and use it…

Statistical Mechanics · Physics 2022-03-08 Audun Skaugen , Lasse Laurson

ZrO2:10%SiO2 thinfilms have been deposited on fused silica substrate by reactive electron beam co-evaporation technique at different oxygen partial pressure. The structural analysis shows tetragonal phase with residual tensile stress in the…

Materials Science · Physics 2020-09-22 S. Jena , R. B. Tokas , S. Thakur , N. K. Sahoo