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Raman spectroscopy together with density functional calculations were used to study lattice dynamics in a layered honeycomb cobaltite Na$_3$Co$_2$SbO$_6$, which can host a field-induced phase related with the Kitaev physics. We show that…

Strongly Correlated Electrons · Physics 2024-05-10 Yu. S. Ponosov , E. V. Komleva , E. A. Pankrushina , D. Mikhailova , S. V. Streltsov

The novel ferroelectric-like structural transition observed in metallic LiOsO$_3$ [Y. Shi et al., Nat. Mater. 12, 1024 (2013)], has invoked many theoretical and experimental interests. In this work, we have performed polarized and…

Materials Science · Physics 2017-03-09 Feng Jin , Anmin Zhang , Jianting Ji , Kai Liu , Le Wang , Youguo Shi , Yong Tian , Xiaoli Ma , Qingming Zhang

The temperature and magnetic field dependence of lattice and carrier excitations in MnSi is studied in detail using inelastic light scattering. The pure symmetry components of the electronic response are derived from the polarization…

Strongly Correlated Electrons · Physics 2014-07-23 H. -M. Eiter , P. Jaschke , R. Hackl , A. Bauer , M. Gangl , C. Pfleiderer

We report results of an investigation of the temperature dependence of the magnon and phonon frequencies in NiO. A combination of Brillouin - Mandelstam and Raman spectroscopies allowed us to elucidate the evolution of the phonon and magnon…

Materials Science · Physics 2017-10-25 M. M. Lacerda , F. Kargar , E. Aytan , R. Samnakay , B. Debnath , J. X. Li , A. Khitun , R. K. Lake , J. Shi , A. A. Balandin

We report Electron Paramagnetic Resonance measurements on single crystalline and powder samples of Nd_0.5Ca_0.5MnO_3 across the charge-ordering transition at T_co=240 K down to the antiferromagnetic ordering transition at T_N = 140 K. The…

Strongly Correlated Electrons · Physics 2021-05-26 Janhavi P. Joshi , Rajeev Gupta , A. K. Sood , S. V. Bhat , A. R. Raju , C. N. R. Rao

RuO$_{2}$ has been proposed as the prototypical altermagnetic material. However, several reports have recently questioned its intrinsic magnetic ordering, leading to conflicting findings, especially in thin film heterostructures pointing to…

We performed an optical spectroscopy study of electronic and magnetic excitations for a rare-earth system with a single electron quasi-localized in the f-shell on an ion at high-symmetry crystallographic site in application to CeB$_{6}$…

Strongly Correlated Electrons · Physics 2019-06-25 Mai Ye , H. -H. Kung , Priscila F. S. Rosa , Eric D. Bauer , Zachary Fisk , G. Blumberg

The doping dependence of the micro-Raman spectra of high quality La_{2-x}Sr_xCuO_4 microcrystals with x=0.0-0.45 has been investigated in the region 10-300 K. The phonon at ~100 cm^{-1} of the orthorhombic phase shows a classical soft mode…

Superconductivity · Physics 2009-11-13 D. Lampakis , E. Liarokapis , C. Panagopoulos

The polarized Raman spectra of layered ruthenates of the Srn+1RunO3n+1 (n=1,2,3) Ruddlesden-Popper series were measured between 10 and 300 K. The phonon spectra of Sr3Ru2O7 and Sr4Ru3O10 confirmed earlier reports for correlated rotations of…

Materials Science · Physics 2009-11-10 M. N. Iliev , V. N. Popov , A. P. Litvinchuk , M. V. Abrashev , J. Backstrom , Y. Y. Sun , R. L. Meng , C. W. Chu

We report on optical measurements of the 1D Heisenberg antiferromagnet KCuF3. The crystal-field excitations of the Cu2+ ions have been observed and their temperature dependence can be understood in terms of magnetic and exchange-induced…

Strongly Correlated Electrons · Physics 2009-11-13 J. Deisenhofer , I. Leonov , M. V. Eremin , Ch. Kant , P. Ghigna , F. Mayr , V. V. Iglamov , V. I. Anisimov , D. van der Marell

Synthetic powder, ore samples and mineral single crystals of goethite ($\alpha-$FeOOH) were investigated with polarized Raman spectroscopy at temperatures from 300 K to 473 K. The symmetry of the vibrational modes, observed in different…

Materials Science · Physics 2020-06-24 M. V. Abrashev , V. G. Ivanov , B. S. Stefanov , N. D. Todorov , J. Rosell , V. Skumryev

By applying a quantum Monte Carlo procedure based on the loop algorithm we investigate thermodynamic properties of the two-dimensional antiferromagnetic S=1/2 Heisenberg model coupled to Einstein phonons on the bonds. The temperature…

Strongly Correlated Electrons · Physics 2009-11-10 Carsten H. Aits , Ute Löw

We present a comprehensive $^{31}$P and $^{65}$Cu nuclear magnetic resonance (NMR) study of the layered van der Waals magnet CuCrP$_2$S$_6$. The compound exhibits a sequence of structural and magnetic phase transitions: a high-temperature…

Strongly Correlated Electrons · Physics 2026-04-06 C. S. Saramgi , L. F. Prager , S. Selter , Y. Shemerliuk , S. Aswartham , B. Büchner , H. -J. Grafe , K. M. Ranjith

The synthesis of SrRuO3 under high-pressure oxygen produces a nonstoichiometric form with randomly distributed vacancies on the Ru-sites, along with a significantly reduced ferromagnetic ordering temperature. In order to gain additional…

Magneto-Raman spectroscopy is applied to study spin-phonon coupling in the layered two-dimensional (2D) van der Waals antiferromagnet CrSBr. We report on the effects of temperature and external magnetic field on Raman-active phonons of…

Materials Science · Physics 2025-03-20 Urszula D. Wdowik , Vaibhav Varade , Jana Vejpravova , Dominik Legut

We present direct evidence of above room temperature magneto-electricity in single-phase Li0.05Ti0.02Ni0.93O with above-ambient antiferromagnetic ordering. Temperature-hysteresis in warming/cooling heat-flow thermograms establishes a…

Materials Science · Physics 2015-09-15 Jitender Kumar , Pankaj K. Pandey , A. M. Awasthi

Raman and Photoluminescence (PL) experiments on correlated metallic La$_{0.7}$Sr$_{0.3}$MnO$_{3}$ have been carried out using different excitation wavelengths as a function of temperature from 15 K to 300 K. Our data suggest a Raman mode…

Condensed Matter · Physics 2009-10-28 Rajeev Gupta , A. K. Sood , R. Mahesh , C. N. R. Rao

We report on high-field magnetization, specific-heat and electron spin resonance (ESR) studies of the quasi-two-dimensional spin-1/2 Heisenberg antiferromagnet [Cu(pyz)2(HF2)]PF6. The frequency-field diagram of ESR modes below TN = 4.38 K…

Strongly Correlated Electrons · Physics 2011-03-10 E. Cizmar , S. A. Zvyagin , R. Beyer , M. Uhlarz , M. Ozerov , Y. Skourski , J. L. Manson , J. A. Schlueter , J. Wosnitza

We report a Raman study of the effect of temperature on the self-energies of optical phonons in a number of transition metals with hexagonal-close-packed structure. Anisotropic softening of phonon energies and narrowing of phonon linewidths…

Materials Science · Physics 2017-01-04 Yu. S. Ponosov , S. V. Streltsov

Infrared reflectance spectra of an epitaxial Bi2FeCrO6 thin film prepared by pulsed laser deposition on LaAlO3 substrate were recorded between 10 and 900 K. No evidence for a phase transition to the paraelectric phase was observed, but some…

Materials Science · Physics 2009-01-06 S. Kamba , D. Nuzhnyy , R. Nechache , K. Zaveta , D. Niznansky , E. Santava , C. Harnagea , A. Pignolet