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Related papers: Multiple Aging Mechanisms in Ferroelectric Deutera…

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Anomalously large dielectric aging is found in the high-susceptibility plateau ferroelectric regime of ~95% deuterated potassium dihydrogen phosphate (DKDP). Much less aging is found in non-deuterated KDP. Optical images of the DKDP domain…

Materials Science · Physics 2017-09-27 Rachel Hecht , Eugene V. Colla , M. B. Weissman

A mechanism of point defect migration triggered by local depolarization fields is shown to explain some still inexplicable features of aging in acceptor doped ferroelectrics. A drift-diffusion model of the coupled charged defect transport…

Materials Science · Physics 2009-11-13 Yuri A. Genenko

Migration of charged point defects triggered by the local random depolarization field is shown to plausibly explain aging of poled ferroelectric ceramics providing reasonable time and acceptor concentration dependences of the emerging…

Materials Science · Physics 2010-01-22 Yu. A. Genenko , J. Glaum , O. Hirsch , H. Kungl , M. J. Hoffmann , T. Granzow

We provide a fundamental insight into the microscopic mechanisms of the ageing processes. Using large scale molecular dynamics simulations of the prototypical ferroelectric material PbTiO3, we demonstrate that the experimentally observed…

Materials Science · Physics 2017-11-01 J. B. J. Chapman , R. E. Cohen , A. V. Kimmel , D. M. Duffy

The structural, dielectric, and thermodynamic properties of the hydrogen-bonded ferroelectric crystal potassium dihydrogen phosphate ($\mathbf{KH_2PO_4}$), KDP for short, differ significantly from those of DKDP ($\mathbf{KD_2PO_4}$). It is…

Computational Physics · Physics 2024-04-15 Bingjia Yang , Pinchen Xie , Roberto Car

We investigate the quantum-mechanical localization of protonated and deterated isotopes in the symmetric low-barrier hydrogen-bonds of potassium dihydrogen phosphate (KDP) crystals in the paraelectric phase. The spatial density…

Materials Science · Physics 2010-02-09 Varadharajan Srinivasan , Roberto Car , Daniel Sebastiani

We characterize in details the aging properties of the ferroelectric phase of K Ta_{1-x} Nb_x O_3 (KTN), where both rejuvenation and (partial) memory are observed. In particular, we carefully examine the frequency dependence of several…

Condensed Matter · Physics 2009-10-31 J. P. Bouchaud , P. Doussineau , T. de Lacerda-Arôso , A. Levelut

It is known that the permittivity of the ferroelectric films is affected by several phenomena, which deteriorate the material quality (e.g. the redistribution of the crystal lattice defects, appearance of the electrode-adjacent…

Materials Science · Physics 2008-12-12 Pavel Mokry

The relaxor ferroelectric (PbMn$_{1/3}$Nb$_{2/3}$O$_3$)$_{1-x}$(PbTiO$_3$)$_{x}$, $x=0.1$, (PMN/PT(90/10)) is found to exhibit several regimes of complicated aging behavior. Just below the susceptibility peak there is a regime exhibiting…

Materials Science · Physics 2009-11-11 Lambert K. Chao , Eugene V. Colla , M. B. Weissman

We analyse the aging dynamics of the one-dimensional Fredrickson-Andersen (FA) model in the nonequilibrium regime following a low temperature quench. Relaxation then effectively proceeds via diffusion limited pair coagulation (DLPC) of…

Statistical Mechanics · Physics 2007-05-23 Peter Mayer , Peter Sollich

Aging dynamics in thin films of poly(methyl methacrylate) (PMMA) have been investigated through dielectric measurements for different types of aging processes. The dielectric constant was found to decrease with increasing aging time at an…

Soft Condensed Matter · Physics 2009-11-10 Koji Fukao , Aiko Sakamoto

The modification of the ac conductivity and the complex permittivity of conducting polypyrrole was monitored throughout a two years thermal aging at 343K. Reduction of the cross-over frequency is correlated with the degradation of…

Materials Science · Physics 2011-10-04 I. Sakellis , A. N. Papathanassiou , J. Grammatikakis

We consider ferroelectric phase transitions in both short-circuited and biased ferroelectric-semiconductor films with a space (depletion) charge which leads to some unusual behavior. It is shown that in the presence of the charge the…

Statistical Mechanics · Physics 2009-10-31 A. M. Bratkovsky , A. P. Levanyuk

Aging limits lithium-ion battery lifetime and must be understood to improve durability and performance, requiring a detailed understanding of how aging alters the availability of cyclable lithium and the integrity of active particles. In…

Deuterium fractionation is considered as an important process to infer the chemical ages of prestellar cores in filaments. We present here the first magneto-hydrodynamical simulations including a chemical network to study deuterium…

Aging to the equilibrium liquid state of organic glasses is studied. The glasses were prepared by cooling the liquid to temperatures just below the glass transition. Aging following a temperature jump was studied by measuring the dielectric…

Soft Condensed Matter · Physics 2013-01-29 Tina Hecksher , Niels Boye Olsen , Kristine Niss , Jeppe C. Dyre

The effect of physical aging of semi-conducting polypyrrole at ambient temperature for two years duration on the dielectric loss at various pressures is investigated. Changes of the dielectric loss spectra and the modification of the values…

Materials Science · Physics 2010-10-04 I. Sakellis , A. N. Papathanassiou , J. Grammatikakis

Physical aging is one of the non-equilibrium phenomena where physical properties change over time due to structural relaxation. Aging in spin glass systems has been explained by a trap model on the temperature-independent energy landscape.…

Statistical Mechanics · Physics 2025-09-08 Ayata Ueno , Tomoko Mizuguchi , Takashi Odagaki

We present new experimental results on the dielectric constant in orientational glasses K$_{1-x}$Li$_x$TaO$_3$ (KLT) with x < 0.05, together with the detailed (analytic and numerical) study of a model which attributes the observed aging to…

Statistical Mechanics · Physics 2009-10-31 F. Alberici-Kious , J_P Bouchaud , L. F. Cugliandolo , P. Doussineau , A. Levelut

An evidence that the dielectric ageing in the polydomain Pb(Zr0.45Ti0.55)O3 thin films is controlled by progressive pinning of 180 domain walls is presented. To provide such a conclusion, we use a general method, which is based on the study…

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