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We examine the structural relaxation of glassy materials at finite temperatures, considering the effect of activated rearrangements and long-range elastic interactions. Our three-dimensional mesoscopic relaxation model shows how the…

Soft Condensed Matter · Physics 2023-12-20 Gieberth Rodriguez-Lopez , Kirsten Martens , Ezequiel E. Ferrero

Soft solids with tunable mechanical response are at the core of new material technologies, but a crucial limit for applications is their progressive aging over time, which dramatically affects their functionalities. The generally accepted…

Soft Condensed Matter · Physics 2017-08-02 Mehdi Bouzid , Jader Colombo , Lucas Vieira Barbosa , Emanuela Del Gado

We use confocal microscopy to directly visualize the dynamics of aging colloidal glasses. We prepare a colloidal suspension at high density, a simple model system which shares many properties with other glasses, and initiate experiments by…

Disordered Systems and Neural Networks · Physics 2009-11-07 Rachel E. Courtland , Eric R. Weeks

It has recently been shown that thermal active glasses can display physical aging behavior comparable to that of passive glasses, although there are some notable distinctions due to the intrinsic non-equilibrium nature of active matter. The…

Soft Condensed Matter · Physics 2024-06-12 Giulia Janzen , Liesbeth M. C. Janssen

The influence of static stress and alternating loading direction on the potential energy and mechanical properties of amorphous alloys is investigated using molecular dynamics simulations. The model glass is represented via a binary mixture…

Soft Condensed Matter · Physics 2021-02-09 Nikolai V. Priezjev

The interrelation of dynamic processes active on separated time-scales in glasses and viscous liquids is investigated using a model displaying two time-scale bifurcations both between fast and secondary relaxation and between secondary and…

Disordered Systems and Neural Networks · Physics 2015-03-19 Andrea Crisanti , Luca Leuzzi , Matteo Paoluzzi

Complex spatiotemporal structures develop during the process of aging glasses after cooling and of rejuvenating glasses upon heating. The key to understanding these structures is the interplay between the activated reconfiguration events…

Soft Condensed Matter · Physics 2008-12-17 Peter G. Wolynes

Molecular dynamics simulations are used to investigate the effects of deformation on the segmental dynamics in an aging polymer glass. Individual particle trajectories are decomposed into a series of discontinuous hops, from which we obtain…

Soft Condensed Matter · Physics 2015-05-19 Mya Warren , Joerg Rottler

The microscopic dynamics of spontaneously aged and rejuvenated glassy Laponite is investigated through X-ray photon correlation spectroscopy. Two different behaviours of the intensity autocorrelation functions are observed depending on the…

Soft Condensed Matter · Physics 2023-09-06 Roberta Angelini , Barbara Ruzicka

We use large-scale molecular dynamics simulations to study the kinetics of the liquid-gas phase separation if the temperature is lowered across the glass transition of the dense phase. We observe a gradual change from phase separated…

Statistical Mechanics · Physics 2011-06-01 Vincent Testard , Ludovic Berthier , Walter Kob

The correlations of the free-energy landscape of mean-field spin glasses at different temperatures are investigated, concentrating on models with a first order freezing transition. Using a ``potential function'' we follow the metastable…

Disordered Systems and Neural Networks · Physics 2009-10-30 A. Barrat , S. Franz , G. Parisi

Vapour deposition can directly produce ultrastable glasses, which are similar to conventional glasses aged over thousands of years. The highly mobile surface layer is believed to accelerate the ageing process of vapour-deposited glasses,…

Soft Condensed Matter · Physics 2016-10-20 Xin Cao , Huijun Zhang , Yilong Han

We study by light microscopy a soft glass consisting of a compact arrangement of polydisperse elastic spheres. We show that its slow and non-stationary dynamics results from the unavoidable small fluctuations of temperature, which induce…

Soft Condensed Matter · Physics 2009-11-11 Sylvain Mazoyer , Luca Cipelletti , Laurence Ramos

We report experimental measurements of particle dynamics in a colloidal glass in order to understand the dynamical heterogeneities associated with the cooperative motion of the particles in the glassy regime. We study the local and global…

Soft Condensed Matter · Physics 2007-05-23 P. Wang , C. Song , H. A. Makse

In the context of the random first order transition theory we use an extended mode coupling theory of the glass transition that includes activated events to account for spatiotemporal structures in aging and rejuvenating glasses. We…

Disordered Systems and Neural Networks · Physics 2015-06-15 Apiwat Wisitsorasak , Peter G. Wolynes

We study the aging dynamics in a model for dense simple liquids, in which particles interact through a hard-core repulsion complemented by a short-ranged attractive potential, of the kind found in colloidal suspensions. In this system, at…

Statistical Mechanics · Physics 2007-05-23 G. Foffi , E. Zaccarelli , S. Buldyrev , F. Sciortino , P. Tartaglia

We consider the dynamics of a diluted mean-field spin glass model in the aging regime. The model presents a particularly rich heterogeneous behavior. In order to catch this behavior, we perform a **spin-by-spin analysis** for a **given…

Disordered Systems and Neural Networks · Physics 2009-11-07 Andrea Montanari , Federico Ricci-Tersenghi

The coupling of active, self-motile particles to topological constraints can give rise to novel non-equilibrium dynamical patterns that lack any passive counterpart. Here we study the behavior of self-propelled rods confined to a compact…

Statistical Mechanics · Physics 2018-08-21 Liesbeth M. C. Janssen , Andreas Kaiser , Hartmut Löwen

We discuss the microscopic mechanisms by which low-temperature amorphous states, such as ultrastable glasses, transform into equilibrium fluids, after a sudden temperature increase. Experiments suggest that this process is similar to the…

Statistical Mechanics · Physics 2016-07-05 Robert L. Jack , Ludovic Berthier

It is well established that glassy materials can undergo aging, i.e., their properties gradually change over time. There is rapidly growing evidence that dense active and living systems also exhibit many features of glassy behavior, but it…

Statistical Mechanics · Physics 2022-03-29 Giulia Janzen , Liesbeth M. C. Janssen