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Many areas of chemistry are devoted to the challenge of understanding, predicting, and controlling the behavior of strongly localized electrons. Examples include molecular magnetism and luminescence, color centers in crystals,…

Chemical Physics · Physics 2022-09-08 R. Matthias Geilhufe , Jeffrey D. Rinehart

Scattering probes the internal structure of quantum systems. We calculate the two-particle elastic scattering phase shift for a short-ranged interaction on a quantum computer. Short-ranged interactions with a large scattering length or…

Nuclear Theory · Physics 2024-06-14 Muhammad Yusf , Ling Gan , Cameron Moffat , Gautam Rupak

We show that multichannel quantum defect theory (MQDT) can be applied successfully as an efficient computational method for cold molecular collisions in Li+NH, which has a deep and strongly anisotropic interaction potential. In this…

Chemical Physics · Physics 2013-05-10 James F. E. Croft , Jeremy M. Hutson

The R-matrix method is a fully-quantum time-independent scattering method, used to simulate nuclear, electron-atom, electron-ion, electron-molecule scattering and more. Here, a novel R-matrix method, RmatReact, is presented as applied to…

Chemical Physics · Physics 2019-12-20 T. Rivlin , L. K. McKemmish , K. E. Spinlove , J. Tennyson

Over the past decade, massive modeling practices on low temperature plasma (LTP) reveal that input data such as microscopic scattering cross sections are crucial to output macroscopic phenomena. In Monte Carlo collision (MCC) modeling on…

Plasma Physics · Physics 2023-08-14 Wei Yang

We propose a hybrid quantum-classical framework to solve the elastic scattering phase shift of two well-bound nuclei in an uncoupled channel. Within this framework, we develop a many-body formalism in which the continuum scattering states…

Nuclear Theory · Physics 2024-08-14 Peiyan Wang , Weijie Du , Wei Zuo , James P. Vary

Studying chemical reactions, particularly in the gas phase, relies heavily on computing scattering matrix elements. These elements are essential for characterizing molecular reactions and accurately determining reaction probabilities.…

Quantum Physics · Physics 2024-04-24 Sumit Suresh Kale , Sabre Kais

We present a new general algorithm for calculating arbitrary jet cross sections in arbitrary scattering processes to next-to-leading accuracy in perturbative QCD. The algorithm is based on the subtraction method. The key ingredients are new…

High Energy Physics - Phenomenology · Physics 2009-10-28 Stefano Catani , Michael H. Seymour

This paper deals with the theory of collisions between two ultracold particles with a special focus on molecules. It describes the general features of the scattering theory of two particles with internal structure, using a time-independent…

Atomic Physics · Physics 2017-03-28 Goulven Quéméner

This paper introduces students and instructors to the use of Scilab for calculating phase shifts from phenomenological potentials in nuclear, atomic, and molecular scattering, beginning with a Riccati-type nonlinear differential equation…

Physics Education · Physics 2024-04-30 Anil Khachi

We present a general formulation of multichannel quantum-defect theory (MQDT) for anisotropic long-range potentials. The theory unifies the treatment of atomic and molecular interactions of all types, and greatly expands the set of…

Atomic Physics · Physics 2020-08-19 Bo Gao

Elastic scattering of a twisted (Bessel) electron beam by CO$_2$ molecules is studied theoretically at high energies. The molecule's structure is optimized using coupled cluster theory and density functional theory with…

Quantum Physics · Physics 2026-04-20 Raul Sheldon Pinto , Rakesh Choubisa

Quantum scattering calculations for strongly interacting molecular systems are computationally demanding due to the large number of molecular states coupled by the anisotropy of atom - molecule interactions. We demonstrate that thermal rate…

Chemical Physics · Physics 2026-01-06 Xuyang Guo , Kirk W. Madison , James L. Booth , Roman V. Krems

Small-angle X-ray or neutron scattering (SAXS/SANS/SAS) is widely used to obtain structural information on biomolecules or soft-matter complexes in solution. Deriving a molecular interpretation of the scattering signals requires methods for…

Biological Physics · Physics 2022-08-16 Leonie Chatzimagas , Jochen S. Hub

Rigorous quantum scattering calculations on ultracold molecular collisions in external fields present an outstanding computational problem due to strongly anisotropic atom-molecule interactions that depend on the relative orientation of the…

Atomic Physics · Physics 2020-12-03 Masato Morita , Jacek Kłos , Timur V. Tscherbul

A simple Monte Carlo procedure is described for simulating the multiple scattering and absorption of electrons with the incident energy in the range 1-50 keV moving through a slab of uniformly distributed material of given atomic number,…

Materials Science · Physics 2007-05-23 Nima Ghal-eh , Mohammad Farhad Rahimi , Mehrnoush Manouchehri

We present a multichannel quantum-defect theory for slow atomic collisions that takes advantages of the analytic solutions for the long-range potential, and both the energy and the angular-momentum insensitivities of the short-range…

Atomic Physics · Physics 2009-11-11 Bo Gao , Eite Tiesinga , Carl J. Williams , Paul S. Julienne

Integrable Quantum Field Theories can be solved exactly using bootstrap techniques based on their elastic and factorisable S-matrix. While knowledge of the scattering amplitudes reveals the exact spectrum of particles and their on-shell…

Statistical Mechanics · Physics 2023-03-30 M. Lencsés , G. Mussardo , G. Takács

We present the point-coupling Hamiltonian as a model for frequency-independent linear optical devices acting on propagating optical modes described as a continua of harmonic oscillators. We formally integrate the Heisenberg equations of…

Quantum Physics · Physics 2019-10-30 Rahul Trivedi , Kevin Fischer , Sattwik Deb Mishra , Jelena Vuckovic

An approach has been devised and tested for preserving the molecular geometry and taking into account energetic considerations during Reverse Monte Carlo modeling. Instead of the commonly used fixed neighbour constraints, where molecules…

Disordered Systems and Neural Networks · Physics 2012-06-15 Orsolya Gereben , Laszlo Pusztai