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Conditional probability density functional theory has recently been used to derive the temperature dependence of the Perdew-Burke-Ernzerhof (PBE) generalized gradient approximation (GGA) for the exchange-correlation (XC) free energy. We…

The isostructural {\alpha}-{\gamma} phase transition in cerium is analyzed using density-functional theory with different exchange-correlation functionals, in particular the PBE0 hybrid functional and the exact- exchange plus correlation in…

Strongly Correlated Electrons · Physics 2015-06-11 Marco Casadei , Xinguo Ren , Patrick Rinke , Angel Rubio , Matthias Scheffler

Batteries are critical for electrified transportation and aviation, yet thermodynamic understanding of electrode materials remains lacking, as indicated by the often-seen violation of the second law of thermodynamics of open-circuit voltage…

Chemical Physics · Physics 2025-07-16 Archie Mingze Yao , Amal Sebastian , Venkatasubramaian Viswanathan

In comparison with the accurate data on the on-top electron density n(0) in the proton-embedded electron gas with the density parameter r_s in the range 1-12 obtained by diffusion Monte Carlo (DMC) simulations, we have successfully…

Materials Science · Physics 2018-07-18 Yasutami Takada

Most methods for estimating configurational entropy from molecular simulation data yield upper limits except for harmonic systems where they are exact. Problems arise at diffusive systems and the presence of conformational transitions.…

Chemical Physics · Physics 2019-10-22 Jürgen Schlitter , Matthias Massarczyk

The development of novel materials for vacuum electron sources in particle accelerators is an active field of research that can greatly benefit from the results of \textit{ab initio} calculations for the characterization of the electronic…

Materials Science · Physics 2021-06-01 Holger-Dietrich Saßnick , Caterina Cocchi

Supersolidity in a dipolar Bose-Einstein condensate (BEC), which is the coexistence of crystalline density modulation and global phase coherence, emerges from the interplay of contact interactions, long-range dipole-dipole forces, and…

Quantum Gases · Physics 2025-10-29 Changjian Yu , Jinbin Li , Kui-Tian Xi

Thermal density functional theory calculations often use the Mermin-Kohn-Sham scheme, but employ ground-state approximations to the exchange-correlation (XC) free energy. In the simplest solvable nontrivial model, an asymmetric Hubbard…

Strongly Correlated Electrons · Physics 2016-06-29 Justin C Smith , Aurora Pribram-Jones , Kieron Burke

Equilibrium Constant Differential Equations (ECDE) are derived for several nanoconfined elemental bimolecular reactions in the frameworks of statistical mechanics and the ideal gas model. The ECDEs complement the well-known…

Chemical Physics · Physics 2020-07-15 Leonid Rubinovich , Micha Polak

Density functional theory (DFT) is the de facto approach for predicting self-consistent-field electronic structures of ground-state configurations of complex atoms, molecules, and solids and providing their property data for materials…

Materials Science · Physics 2024-01-30 Zi-Kui Liu

The structural, electronic, mechanical and thermal properties of Ir$_{1-x}$Rh$_{x}$ alloys were studied systematically using ab initio density functional theory at different concentrations (x = 0.00, 0.25, 0.50, 0.75, 1.00). A Special…

Materials Science · Physics 2015-06-15 S. Ahmed , M. Zafar , M. Shakil , M. A. Choudhary

We construct a replica technique to perturbatively compute the odd entanglement entropy (OEE) for bipartite mixed states in $\text{T}\bar{\text{T}}$ deformed CFT$_2$s. This framework is then utilized to obtain the leading order correction…

High Energy Physics - Theory · Physics 2023-12-21 Debarshi Basu , Saikat Biswas , Ankur Dey , Boudhayan Paul , Gautam Sengupta

Static correlation error(SCE) inevitably emerges when a dissociation of a covalent bond is described with a conventional denstiy-functional theory (DFT) for electrons. SCE gives rise to a serious overshoot in the potential energy at the…

Computational Physics · Physics 2020-08-10 Hideaki Takahashi

Extended X-ray absorption fine structure (EXAFS) spectra are sensitive to thermal disorder and are often used to probe local lattice dynamics. Variations in interatomic distances induced by atomic vibrations are described by the…

Materials Science · Physics 2024-10-28 Alexei Kuzmin , Vitalijs Dimitrijevs , Inga Pudza , Aleksandr Kalinko

Simulation of warm dense matter requires computational methods that capture both quantum and classical behavior efficiently under high-temperature, high-density conditions. Currently, density functional theory molecular dynamics is used to…

Chemical Physics · Physics 2015-10-21 Attila Cangi , Aurora Pribram-Jones

We consider the symmetry-resolved R\'{e}nyi and entanglement entropies for two-dimensional conformal field theories on a circle at nonzero temperature. We assume a unique ground state with a nonzero mass gap induced by the system's finite…

High Energy Physics - Theory · Physics 2023-06-14 Mostafa Ghasemi

We develop the first order gradient correction to the exchange-correlation free energy of the homogeneous electron gas for use in finite temperature density functional calculations. Based on this we propose and implement a simple…

Computational Physics · Physics 2015-06-22 Travis Sjostrom , Jerome Daligault

We introduce a method to carry out zero-temperature calculations within density functional theory (DFT) but without relying on the Born-Oppenheimer (BO) approximation for the ionic motion. Our approach is based on the finite-temperature…

Materials Science · Physics 2018-11-21 Grigory Kolesov , Efthimios Kaxiras , Efstratios Manousakis

The soft wall AdS/QCD holographic model provides simple estimates for the spectra of light mesons and glueballs satisfying linear Regge trajectories. It is also an interesting tool to represent the confinement/deconfinement transition of a…

High Energy Physics - Theory · Physics 2021-07-07 Nelson R. F. Braga , Octavio C. Junqueira

Lattice thermal conductivity ($\kappa_{\rm L}$) is a crucial characteristic of crystalline solids with significant implications for practical applications. While the higher order of anharmonicity of phonon gas model is commonly used for…

Materials Science · Physics 2024-04-10 Jiacheng Wei , Zhonghao Xia , Yi Xia , Jiangang He