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We present the results from an extensive atomistic molecular dynamics simulation study of poly(ethylene oxide) (PEO) doped with various amounts of lithium-bis(trifluoromethane)sulfonimide (LiTFSI) salt under the influence of external…

Soft Condensed Matter · Physics 2021-03-10 Alina Wettstein , Diddo Diddens , Andreas Heuer

Water-in-Salt-Electrolytes (WiSEs) are a promising class of next-generation electrolytes. Unlike classical dilute electrolytes or more conventional battery electrolytes, WiSEs are characterised by their super-concentrated salt concentration…

We study the effects of charge-regulated acid/base equilibrium on the swelling of polyelectrolyte gels, by considering a combination of the Poisson-Boltzmann theory and a two-site charge-regulation model based on the Langmuir adsorption…

Soft Condensed Matter · Physics 2023-08-02 Bin Zheng , Yael Avni , David Andelman , Rudolf Podgornik

The study of the structural behaviour of pure and multi-component lipids at various temperatures and the interaction of these multi-component lipids with pharmaceutically important drugs carry huge importance. Here, we investigated the…

Soft Condensed Matter · Physics 2021-03-26 Prantar Dutta , Debabrata Pramanik , Jayant K. Singh

The nature of electrostatic interactions involving polyanions modulate the properties of both synthetic and biological macromolecules. Although intensely studied for decades the interplay of many length scales has prevented a complete…

Soft Condensed Matter · Physics 2011-03-11 Ngo Minh Toan , Bae-Yeun Ha , D. Thirumalai

The addition of filler particles to polymer electrolytes is known to increment their ionic conductivity (IC). A detailed understanding of how the interactions between the constituent materials are responsible for the enhancement, remains to…

Materials Science · Physics 2021-03-19 Andres Villa , Juan Carlos Verduzco , Joseph A. Libera , Ernesto E. Marinero

We model cyclic voltammetry experiments on supported lipid films where a non-trivial dependence of the capacitance on the applied voltage is observed. Previously, based on a mean-field treatment of the Flory-Huggins type, under the…

Soft Condensed Matter · Physics 2010-07-28 Andrey V. Brukhno , Anna Akinshina , Zachary Coldrick , Andrew Nelson , Stefan Auer

We present a pedagogical review of the swelling thermodynamics and phase transitions of polymer gels. In particular, we discuss how features of the volume phase transition of the gel's osmotic equilibrium is analogous to other transitions…

Soft Condensed Matter · Physics 2019-06-13 Michael S. Dimitriyev , Ya-Wen Chang , Paul M. Goldbart , Alberto Fernández-Nieves

Hydrogels which are hydrophilic and porous materials have recently emerged as promising systems for filtration applications. In our study, we prepare hydrogel membranes by the photopolymerization of a mixture of poly (ethylene glycol)…

Liquid crystalline polymers are materials of considerable scientific interest and technological value to society [1-3]. An important subset of such materials exhibit rubber-like elasticity; these can combine the remarkable optical…

The electric double layer is an important structure that appears at charged liquid interfaces, and it determines the performance of various electrochemical devices such as supercapacitors and electrokinetic energy converters. Here the…

Soft Condensed Matter · Physics 2023-08-15 Haruto Iwasaki , Yasuyuki Kimura , Yuki Uematsu

In this chapter polyelectrolyte intelligent gels are examined along three broad lines. The effects of different physical, chemical and biological stimuli on gels response are analysed and mechanisms of response are outlined. The broad range…

Soft Condensed Matter · Physics 2012-10-15 Piero Chiarelli , Danilo De Rossi

Plasma electrolytic oxidation (PEO) is a technique used to create oxide-ceramic coatings on lightweight metals, such as aluminium, magnesium, and titanium. PEO is known for producing coatings with high corrosion resistance and strong…

A swollen phase, in which the mean repeat distance of lipid bilayers is larger than the other phases, is found between the liquid-crystalline phase and the interdigitated gel phase in DPPC aqueous solution. Temperature, pressure and ethanol…

Soft Condensed Matter · Physics 2009-03-13 H. Seto , M. Hishida , H. Nobutou , N. L. Yamada , M. Nagao , T. Takeda

Electrochemical devices often consist of multicomponent electrolyte solutions. Two processes influence the overall dynamics of these devices: the formation of electrical double layers and chemical conversion due to redox reactions. However,…

Chemical Physics · Physics 2022-06-20 Nathan Jarvey , Filipe Henrique , Ankur Gupta

Elastic interactions arising from a difference of lattice spacing between two coherent phases can have a strong influence on the phase separation (coarsening) of alloys. If the elastic moduli are different in the two phases, the elastic…

Mathematical Physics · Physics 2015-06-26 P. Fratzl , O. Penrose , J. L. Lebowitz

In electrochemical systems, the structure of electrical double layers (EDLs) near electrode surfaces is crucial for energy conversion and storage functions. While the electrodes in real-world systems are usually heterogeneous, to date the…

Electropolymerization plays a critical role in the electrochemical systems. In this chapter, we address such role within the context of interplay between kinetics and energetics. The trains of chin radical reactions leads to the formation…

Chemical Physics · Physics 2019-04-18 Asghar Aryanfar , Agustin J. Colussi , Laleh M. Kasmaee , Michael R. Hoffmann

The two-phase composite approach of Estrin et al. (1998) describes an evolving dislocation cell structure. Mckenzie et al. (2007) enhanced the model to capture the effects of hydrostatic pressure and temperature during severe plastic…

Materials Science · Physics 2013-03-08 C. B. Silbermann , A. V. Shutov , J. Ihlemann

Recent studies have pointed the importance of polyelectrolyte assembly in the elaboration of innovative nanomaterials. Beyond their structures, many important questions on the thermodynamics of association remain to be answered. Here, we…

Materials Science · Physics 2021-09-21 L. Vitorazi , N. Ould-Moussa , S. Sekar , J. Fresnais , W. Loh , J. -P. Chapel , J. -F. Berret