Related papers: Two-photon excitation spectroscopy of 1,5--Dipheny…
Two-photon excitation spectroscopy with broad spectral span is demonstrated at Doppler-limited resolution. We describe first Fourier transform two-photon spectroscopy of an atomic sample with two mode-locked laser oscillators in a dual-comb…
An experimental study of the long range behavior of the ground state X^1\Sigma^+_g of Sr_2 is performed by high resolution spectroscopy of asymptotic vibrational levels and the use of available photoassociation data. Ground state levels as…
We study resonant two-color two-photon ionization of Helium via the 1s3p 1P1 state. The first color is the 15th harmonic of a tunable titanium sapphire laser, while the second color is the fundamental laser radiation. Our method uses…
This is the first in a series of two papers investigating the effect of electron-phonon coupling in two-dimensional Fourier transformed electronic spectroscopy. We present a series of one- and two-dimensional nonlinear spectroscopic…
Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…
The 3p\pi D^1\Pi_u state of the H_2 molecule was reinvestigated with different techniques at two synchrotron installations. The Fourier-Transform spectrometer in the vacuum ultraviolet wavelength range of the DESIRS beamline at the SOLEIL…
Atomic excitation to excited states in strong laser field is the key to high-order harmonic generation below ionization threshold, yet remains unclear mainly due to the lack of proper detection methods. We propose a frequency-resolved…
We describe a proof-of-principal experiment demonstrating a Fourier technique for measuring the shape of biphoton wavepackets. The technique is based on the use of synchronously driven fast modulators and slow (integrating) detectors.
A high resolution study of the electronic states 1^1\Sigma^+_u and 1^1\Pi_u which belong to the asymptote 4^1D + 5^1S and of the state 2(A)^1\Sigma^+_u, which correlates to the asymptote 5^1P + 5^1S, is performed by Fourier-transform…
Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy…
Information technology demands high-speed optoelectronic devices, but going beyond the one terahertz (THz) barrier is challenging due to the difficulties associated with generating, detecting, and processing high-frequency signals. Here, we…
We propose and demonstrate a versatile technique to measure the lifetime of the one-phonon Fock state using two-color pump-probe Raman scattering and spectrally-resolved, time-correlated photon counting. Following pulsed laser excitation,…
Excited-state vibrations are crucial for determining photophysical and photochemical properties of molecular compounds. Stimulated Raman scattering can coherently stimulate and probe molecular vibrations with optical pulses, but it is…
Spectroscopy of gases under high-pressure conditions is of interest in various fields such as plasma physics and astrophysics. Recently, it has also been proposed to utilize a high-pressure noble gas environment as a thermalization medium…
We report observation of two-photon emission from coherently excited vibrational state of solid parahydrogen, known as one of quantum solids. The coherent state between the ground and the excited states is prepared by stimulated Raman…
We describe a high-resolution spectroscopy method, in which the detection of single excitation events is enhanced by a complete loss of coherence of a superposition of two ground states. Thereby, transitions of a single isolated atom nearly…
We experimentally demonstrate amplitude and phase modulation of a time-energy entangled two-photon wave function. The entangled photons are produced by spontaneous parametric down-conversion, spectrally dispersed in an prism compressor,…
We analyze Photo-Electron Spectra (PES) for a variety of excitation mechanisms from a simple mono-frequency laser pulse to involved combination of pulses as used, e.g., in attosecond experiments. In the case of simple pulses, the peaks in…
In this paper, we describe an experiment which was conducted to explore the macro-coherent amplification mechanism using a two-photon emission process from the first vibrationally-excited state of para-hydrogen molecule. Large coherence in…
Single-molecule fluorescence spectroscopy is a powerful method that avoids ensemble averaging, but its temporal resolution is limited by the fluorescence lifetime to nanoseconds at most. At the ensemble level, two-dimensional spectroscopy…