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Ultrafast broadband ultraviolet radiation is of importance in spectroscopy and photochemistry, since high photon energies enable single-photon excitations and ultrashort pulses allow time-resolved studies. Here we report the use of…

Although supercontinuum sources are readily available for the visible and near infrared, and recently also for the mid-IR, many areas of biology, chemistry and physics would benefit greatly from the availability of compact, stable and…

We report generation of spectrally bright vacuum ultraviolet (VUV) and deep UV (DUV) coherent radiations driven by quantum coherence in tunnel-ionized carbon monoxide (CO) molecules. Our technique allows us to switch between multiple…

Many fields such as bio-spectroscopy and photochemistry often require sources of vacuum ultraviolet (VUV) pulses featuring a narrow linewidth and tunable over a wide frequency range. However, the majority of available VUV light sources do…

Optics · Physics 2020-06-11 Rinat Tyumenev , Philip St. J. Russell , David Novoa

Vacuum ultraviolet (VUV) light is critical for the study of molecules and materials, but the generation of femtosecond pulses in the VUV region at high repetition rates has proven difficult. Here, we demonstrate the efficient generation of…

We demonstrate sensitive high-resolution stimulated Raman measurements of hydrogen using a hollow-core photonic crystal fiber (HC-PCF). The Raman transition is pumped by a narrow linewidth (<50 kHz) 1064 nm continuous-wave (CW) fiber laser.…

Optics · Physics 2015-06-16 Philip G. Westergaard , Mikael Lassen , Jan C. Petersen

We report the generation of a purely vibrational Raman comb, extending from the vacuum ultraviolet (184 nm) to the visible (478 nm), in hydrogen-filled kagom\'e-style photonic crystal fiber pumped at 266 nm. Stimulated Raman scattering and…

We report on a highly-efficient experimental scheme for the generation of deep-ultraviolet ultrashort light pulses using four-wave mixing in gas-filled kagom\'e-style photonic crystal fiber. By pumping with ultrashort, few $\mu$J, pulses…

We demonstrate, for the first time, the application of rare-gas filled hollow-core photonic crystal fibres (HC-PCFs) as tuneable ultraviolet light sources in femtosecond pump-probe spectroscopy. The time-resolved photoelectron imaging…

Laser-driven high-order harmonic generation (HHG) provides tabletop sources of broadband extreme-ultraviolet (XUV) light with excellent spatial and temporal coherence. These sources are typically operated at low repetition rates,…

We report generation of an ultrafast supercontinuum extending into the mid- infrared in gas-filled single-ring hollow-core photonic crystal fiber (SR-PCF) pumped by 1.7 $\mu$m light from an optical parametric amplifier. The simple fiber…

The recent breakthroughs in laser-driving 229Th nuclear transition have created an urgent demand for coherent vacuum-ultraviolet (VUV) sources delivering high spectral brightness at the critical 148.38 nm isomer energy. However, generating…

Continuous-wave coherent radiation in the vacuum ultraviolet (VUV)wavelength region at 121 nm will be essential for future laser-cooling of trapped antihydrogen [1]. Cold antihydrogen will enable both tests of the fundamental symmetry…

Optics · Physics 2012-08-20 Daniel Kolbe , Martin Scheid , Jochen Walz

We report a novel scheme for the generation of dense clusters of Raman sidebands. The scheme uses a broadband-guiding hollow-core photonic crystal fiber (HC-PCF) filled with a mixture of H2, D2, and Xe for efficient interaction between the…

Optics · Physics 2016-11-24 Pooria Hosseini , Amir Abdolvand , Philip St. J. Russell

We present the use of linearly down-tapered gas-filled hollow-core photonic crystal fiber in a single-stage, pumped with pulses from a compact infrared laser source, to generate a supercontinuum carrying significant spectral power in the…

High harmonic generation (HHG) enables extreme ultraviolet radiation with table-top setups. Its exceptional properties, such as coherence and (sub)-femtosecond pulse durations, have led to a diversity of applications. Some of these require…

Large-area quantum networks based on optical fibers allow photons at near-infrared wavelengths to travel with minimal loss. Quantum frequency conversion is a method to alter the wavelength of a single photon while maintaining its quantum…

Quantum Physics · Physics 2025-06-09 Anica Hamer , Frank Vewinger , Michael H. Frosz , Simon Stellmer

Ultraviolet frequency combs enable applications ranging from precision spectroscopy to atomic clocks by addressing the electronic transitions of atoms and molecules. Access to ultraviolet light via integrated nonlinear optics is usually…

Recent demonstrations of high-harmonic generation (HHG) at very high repetition frequencies (~100 MHz) may allow for the revolutionary transfer of frequency combs to the vacuum ultraviolet (VUV). This advance necessitates unifying optical…

The unique ring-shaped intensity patterns and helical phase fronts of optical vortices make them useful in many applications. Here we report for the first time efficient Raman frequency conversion between vortex modes in twisted…

Optics · Physics 2020-04-22 S. Davtyan , Y. Chen , M. H. Frosz , P. ST. J. Russell , D. Novoa
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