Related papers: Fano's propensity rule in angle-resolved attosecon…
The photoelectric effect is not truly instantaneous, but exhibits attosecond delays that can reveal complex molecular dynamics. Sub-femtosecond duration light pulses provide the requisite tools to resolve the dynamics of photoionization.…
We describe in detail how attosecond delays in laser-assisted photoionization can be computed using perturbation theory based on two-photon matrix elements. Special emphasis is laid on above-threshold ionization, where the electron…
We investigate a conjecture used in recent experiments to reconstruct the complete dynamics of Fano autoionisation processes out of measured spectral amplitudes [Gruson et al, Science 354 734 (2016); Beaulieu el al, Science 358 1288 (2017);…
We present a new theoretical approach to attosecond laser-assisted photo- and Compton ionization. Attosecond x-ray absorption and scattering are described by $\hat{\mathrsfs{S}}^{(1,2)}$-matrices, which are coherent superpositions of…
We show that Fano interference explains how point contact spectroscopy in heavy electron materials probes the emergence of the Kondo heavy electron liquid below the same characteristic temperature T* as that seen in many other experiments,…
We construct the formula for the photonuclear total absorption cross section using the projection method and the unitarity relation. Our treatment is very effective when interference effects in the absorption processes on a nucleon are…
A detailed theoretical study of the optical absorption in self-assembled quantum dots is presented in this paper. A rigorous atomistic strain model as well as a sophisticated electronic band structure model are used to ensure accurate…
Multi-photon absorption is a well-known phenomenon. With atom lasers a similar process could take place for massive particles, the ionization of an atom or molecule by the successive interaction with various particles. This process would…
Two-photon atomic ionization driven by time-locked XUV and IR pulses allows to study dynamics of Fano resonances in time and energy domains. Different time evolution of the two interfering pathways leading to a Fano resonance can be…
We study atomic autoionization processes in the time domain. With the emerging attosecond extreme vacuum ultraviolet and soft x-ray pulses, we first address how to characterize the time evolution of the decay of a discrete state into a…
Collisional absorption of laser light in a homogeneous, under-dense plasma is studied by a new particle-in-cell (PIC) simulation code considering one-dimensional slab-plasma geometry. Coulomb collisions between charge particles in plasma…
Surface enhanced Raman spectra from molecules (bipyridyl ethylene) adsorbed on gold dumbells are observed to become increasingly asymmetric (Fano-like) at higher incident light intensity. The electronic temperature (inferred from the…
The Fano lineshape arises from the interference of two excitation pathways to reach a continuum. Its generality has resulted in a tremendous success in explaining the lineshapes of many one-dimensional spectroscopies - absorption, emission,…
An optical Fano resonance, which is caused by birefringence control rather than frequency selection, is discovered. Such birefringence-induced Fano resonance comes with fast-switching radiation. The resonance condition $\varepsilon_t<…
We investigate the possibility to use transient absorption of a coherent bound electron wave packet in hydrogen as an attosecond pulse characterization technique. In recent work we have shown that photoionization of such a coherent bound…
Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of…
Photocatalytic reactions often exhibit fast kinetics and high product selectivity, qualities which are desirable but difficult to achieve simultaneously in thermally driven processes. However, photo-driven mechanisms are poorly understood…
Narrow optical resonances of atoms or molecules have immense significance in various precision measurements, such as testing fundamental physics and the generation of primary frequency standards. In these studies, accurate transition…
We consider the time-delayed coincidence counting of two photons emitted in a cascade by a single particle (atom, molecule, nucleus, etc). The time-dependence of the probability amplitude of the second photon in the cascade has a sharply…
We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by…