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We present experimental results on the preparation of a desired quantum state in a two-level system with the maximum possible fidelity using driving protocols ranging from generalizations of the linear Landau-Zener protocol to…

Quantum Physics · Physics 2012-11-08 N. Malossi , M. G. Bason , M. Viteau , E. Arimondo , R. Mannella , O. Morsch , D. Ciampini

Excited states are the key species in photocatalysis, while the critical parameters that govern their applications are: i) excitation energy, ii) accessibility, and iii) lifetime. However, in molecular transition metal-based…

We develop a method for executing robust and selective transfer of populations between a single level and pre-selected superpositions of energy eigenstates. Viewed in the frequency domain, our method amounts to executing a series of…

Quantum Physics · Physics 2009-11-13 Evgeny A. Shapiro , Valery Milner , Moshe Shapiro

We demonstrate that Optimal Control Theory (OCT) with a state-dependent constraint which depends on the state of the system at each instant can reproduce the famous counterintuitive mechanism of Stimulated Raman adiabatic passage (STIRAP).…

Quantum Physics · Physics 2017-01-09 Amine Jaouadi , Mamadou Ndong

We propose a cooling scheme to prepare stationary entanglement of neutral atoms in the Rydberg blockade regime by combination of periodically collective laser pumping and dissipation. In each cycle, the controlled unitary dynamics process…

Quantum Physics · Physics 2022-09-07 Wei-Lin Mu , Xiao-Xuan Li , Xiao-Qiang Shao

The possibility of coherent population trapping in two electron states with aligned spins (ortho-system) is evidenced. From the analysis of a three-level atomic system containing two electrons, and driven by the two laser fields needed for…

Quantum Physics · Physics 2009-11-07 J. Mompart , R. Corbalan , L. Roso

We consider performing adiabatic rapid passage (ARP) using frequency-swept driving pulses to excite a collection of interacting two-level systems. Such a model arises in a wide range of many-body quantum systems, such as cavity QED or…

Mesoscale and Nanoscale Physics · Physics 2012-08-21 R. T. Brierley , C. Creatore , P. B. Littlewood , P. R. Eastham

We extend our hybrid linear-method/accelerated-descent variational Monte Carlo optimization approach to excited states and investigate its efficacy in double excitations. In addition to showing a superior statistical efficiency when…

Chemical Physics · Physics 2022-02-24 Leon Otis , Isaac M. Craig , Eric Neuscamman

We present a novel approach for analytically reducing a family of time-dependent multi-state quantum control problems to two-state systems. The presented method translates between $SU(2)XSU(2)$ controlled $n^{2}$-state systems and two-state…

Quantum Physics · Physics 2018-05-09 Alon Padan , Haim Suchowski

We consider state transfer between two qubits - effective two-level systems represented by Rydberg atoms - via a common mode of a microwave cavity at finite temperature. We find that when both qubits have the same coupling strength to the…

Quantum Physics · Physics 2018-04-16 Lőrinc Sárkány , József Fortágh , David Petrosyan

We propose a two-photon micromaser-based scheme for the generation of a nonclassical state from a mixed state. We conclude that a faster, as well as a higher degree of field purity is achieved in comparison to one-photon processes. We…

Quantum Physics · Physics 2016-02-16 A. F. Gomes , J. A. Roversi , A. Vidiella-Barranco

We present a blueprint for a maser with a single three-level transmon superconducting artificial atom. The system can be pumped coherently via a two-photon process, and to achieve high population inversion, the relaxation rate of the…

Quantum Physics · Physics 2021-01-15 A. A. Sokolova , G. P. Fedorov , E. V. Il'ichev , O. V. Astafiev

Realizing efficient and controlled state transfer is necessary for implementing a wide range of classical and quantum information protocols. Recent studies have demonstrated that both asymmetric and symmetric state transfer can be achieved…

Quantum Physics · Physics 2025-10-13 Qi-Cheng Wu , Yu-Liang Fang , Yan-Hui Zhou , Jun-Long Zhao , Yi-Hao Kang , Qi-Ping Su , Chui-Ping Yang

The optimal control of population transfer for multi-level systems is investigated from the perspective of quantum geometry. Firstly, the general theoretical framework of optimizing the stimulated Raman adiabatic passage (STIRAP) scheme…

Quantum Physics · Physics 2025-12-24 Guan-Qiang Li , Yu-Qi Zhang , Hao Guo , You-Jiao Dong , Zhi-Yu Lin , Ping Peng

We show that a two-level non-Hermitian Hamiltonian with constant off-diagonal exchange elements can be analyzed exactly when the underlying exceptional point is perfectly encircled in the complex plane. The state evolution of this system is…

Shortcut to adiabaticity in various quantum systems has attracted much attention with the wide applications in quantum information processing and quantum control. In this paper, we concentrate on stimulated Raman shortcut-to-adiabatic…

Quantum Physics · Physics 2016-12-21 Yi-Chao Li , Xi Chen

We propose a method to transfer the population and control the state of two-level and three-level atoms speeding-up Adiabatic Passage techniques while keeping their robustness versus parameter variations. The method is based on…

Quantum Physics · Physics 2010-09-20 Xi Chen , I. Lizuain , A. Ruschhaupt , D. Guery-Odelin , J. G. Muga

We use the effective Hamiltonian that we recently fitted against the first 306 experimentally observed vibronic transitions of NO2 [J. Chem. Phys. 119, 5923 (2003)] to investigate the time domain nonadiabatic dynamics of this molecule on…

Chemical Physics · Physics 2011-11-09 Michaël Sanrey , Marc Joyeux

We study Rosen-Zener transition (RZT) in a nonlinear two-level system in which the level energies depend on the occupation of the levels, representing a mean-field type of interaction between the particles. We find that the nonlinearity…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Di-Fa Ye , Li-Bin Fu , Jie Liu

We examine the stability of population transfer in two- and three-level systems against unwanted additional transitions. This population inversion is achieved by using recently proposed schemes called "shortcuts to adiabaticity". We…

Quantum Physics · Physics 2017-03-14 Anthony Kiely , Andreas Ruschhaupt