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An interferometer with effectively infinite maximum optical path difference removes the dominant resolution limitation for interferometric spectroscopy. We present mass-correlated rotational Raman spectra that represent the world's highest…
We report the broadband absorption spectrum of the $3\nu_{2}$ band of $^{14}$NH$_{3}$ near 4 $\mu m$. The data were recorded using a mid-infrared frequency comb coupled to a homebuilt Fourier-transform spectrometer with a resolution of…
We discuss the laser frequency comb as a near infrared astronomical wavelength reference, and describe progress towards a near infrared laser frequency comb at the National Institute of Standards and Technology and at the University of…
Mid-infrared (mid-IR) spectroscopy offers unparalleled sensitivity for the detection of trace gases, solids and liquids, which is based on the existence of strong telltale vibrational bands in this part of the spectrum. It was shown more…
We report on a comb-locked cavity ring-down spectrometer developed for high-precision, SI-traceable, molecular spectroscopy of air-broadened CO2 gas samples. The experimental setup relies on the use of a singly-resonant optical parametric…
Astronomical precision spectroscopy underpins searches for life beyond Earth, direct observation of the expanding Universe and constraining the potential variability of physical constants across cosmological scales. Laser frequency combs…
With the aim of utilizing arrayed waveguide gratings for multi-object spectroscopy in the field of astronomy, we outline several ways in which standard telecommunications grade chips should be modified. In particular, by removing the…
The broadband, coherent nature of narrow-linewidth fiber frequency combs is exploited to measure the full complex spectrum of a molecular gas through multi-heterodyne spectroscopy. We measure the absorption and phase shift experienced by…
We radically simplify coherently averaged dual-comb spectroscopy by introducing a real-time self-correction system: a radio frequency system-on-chip computes each incoming dual-comb interferogram's phase, frequency, and arrival time;…
Femtosecond interferometry combined with acousto-optical phase modulation is an effective approach to implement various types of coherent nonlinear and multidimensional spectroscopy schemes. The high sensitivity of this method has recently…
We have performed sub-Doppler spectroscopy on the narrow intercombination line of cold calcium atoms using the amplified output of a femtosecond laser frequency comb. Injection locking of a 657-nm diode laser with a femtosecond comb allows…
Radial velocity (RV) surveys supported by high precision wavelength references (notably ThAr lamps and I2 cells) have successfully identified hundreds of exoplanets; however, as the search for exoplanets moves to cooler, lower mass stars,…
We demonstrate incoherent broadband cavity enhanced absorption spectroscopy in the mid-infrared wave- length range from 3000 to 3450 nm using an all-fiber based supercontinuum source. Multi-components gas detection is performed and…
Direct comb spectroscopy is a useful tool for obtaining highly accurate spectroscopic information. However, as the number of comb modes is very large and the optical energy is dispersed over them, the optical energy per each comb mode is…
The GraF instrument using a Fabry-Perot interferometer cross-dispersed with a grating was one of the first integral-field and long-slit spectrographs built for and used with an adaptive optics system. We describe its concept, design,…
Quantum metrology has been shown to surpass classical limits of correlation, resolution, and sensitivity. It has been introduced to interferometric Radar schemes, with intriguing preliminary results. Even quantum-inspired detection of…
Near-infrared (NIR) hyperspectral imaging has become a critical tool in modern analytical science. However, conventional NIR hyperspectral imaging systems face challenges including high cost, bulky instrumentation, and inefficient data…
We demonstrate coherent dual frequency-comb spectroscopy for detecting variations in greenhouse gases. High signal-to-noise spectra are acquired spanning 5990 to 6260 cm^-1 (1600 to 1670 nm) covering ~700 absorption features from CO2, CH4,…
Coplanar waveguide resonators are central to the thriving field of circuit quantum electrodynamics. Recently, we have demonstrated the generation of a broadband microwave-frequency comb spectrum using a superconducting quantum interference…
Mid-infrared (mid-IR) frequency combs have broad applications in molecular spectroscopy and chemical/biological sensing. Recently developed microresonator-based combs in this wavelength regime could enable portable and robust devices using…