Related papers: Femtosecond Covariance Spectroscopy
Ultrafast lasers have become one of the most powerful tools in coherent nonlinear optical spectroscopy. Short pulses enable direct observation of fast molecular dynamics, whereas broad spectral bandwidth offers ways of controlling nonlinear…
Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…
The correlated behavior of electrons determines the structure and optical properties of molecules, semiconductor and other systems. Valuable information on these correlations is provided by measuring the response to femtosecond laser…
High peak power ultrafast lasers are widely used in nonlinear spectroscopy but often limit its spectral resolution because of the broad frequency bandwidth of ultrashort laser pulses. Improving the resolution by achieving spectrally narrow…
We demonstrate numerically a method of focusing two-photon field inside one-dimensional random media. The approach is based on coherent control of backscattering achieved by adaptive spectral pulse shaping. The spectral phases of a…
We investigate the effect of incoherent perturbations on atomic photoionization due to a femtosecond mid-infrared laser pulse by solving the time-dependent stochastic Schr\"odinger equation. For a weak laser pulse which causes almost no…
Alternative machine learning approaches that are computationally light with low latency and can work with only a small training dataset are needed for applications where the insatiable demand of deep learning methods for computing power and…
Linear off-resonant X-ray Raman techniques are capable of detecting the ultrafast electronic coherences generated when a photoexcited wave packet passes through a conical intersection. A hybrid femtosecond or attosecond probe pulse is…
We present a novel approach to transient Raman spectroscopy, which combines stochastic probe pulses and a covariance-based detection to measure stimulated Raman signals in alpha-quartz. A coherent broadband pump is used to simultaneously…
The experiments with weak collinear probe pulses for time reversal noninvariance study in optics are proposed and discussed.
We demonstrate a novel technique of coherent Raman spectroscopy with a femtosecond laser. We apply to a molecular sample a sequence of pairs of ultrashort excitation and probe pulses, with a linearly increasing time delay between the two…
The filamentational instability of spatially broadband femtosecond optical pulses in air is investigated by means of a kinetic wave equation for spatially incoherent photons. An explicit expression for the spatial amplification rate is…
X-ray absorption spectroscopy (XAS) is a powerful and well established technique with sensitivity to elemental and chemical composition. Despite these advantages, its implementation has not kept pace with the development of ultrafast pulsed…
Conventional femtosecond coherent laser spectroscopy predominantly focuses on the temporal phase coherence through time- or frequency-resolved methods. In this work, we suggest an alternative experimental framework based on spatial phase…
Self-action nonlinearity is a key aspect -- either as a foundational element or a detrimental factor -- of several optical spectroscopies and photonic devices. Supercontinuum generation, wavelength converters and chirped pulse amplification…
We investigate the effect of phase modulation of laser beams on the coherent and incoherent non-linear signals arising from the interaction of femtosecond pulses with matter. We observe that two collinear beams, whose phases are modulated…
Many experiments in biological and medical sciences currently use multiphoton microscopy as a core imaging technique. To date, solid-state lasers are most commonly used as excitation beam sources. However, the most demanding applications…
Noise manifests ubiquitously in nonlinear spectroscopy, where multiple sources contribute to experimental signals generating interrelated unwanted components, from random point-wise fluctuations to structured baseline signals. Mitigating…
High brightness and low coherence laser sources with wideband tunability are essential for many full-field imaging applications aiming for high contrast and speckle free performance. However, this combination of parameters is challenging to…
We describe an experiment to measure the emitted real-time electric field from an ultrafast third-order nonlinear optical interaction in molecules, using a phase-tracked spectral interferometry scheme. By combining a software lock-in…