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Excitonic insulators (EI) arise from the formation of bound electron-hole pairs (excitons) in semiconductors and provide a solid-state platform for quantum many-boson physics. Strong exciton-exciton repulsion is expected to stabilize…

Tuning many-body electronic phases by an external handle is of both fundamental and practical importance in condensed matter science. The tunability mirrors the underlying interactions, and gigantic electric, optical and magnetic responses…

Strongly Correlated Electrons · Physics 2021-10-04 Q. He , X. Que , L. Zhou , M. Isobe , D. Huang , H. Takagi

An excitonic insulator is a material that hosts an exotic ground state, where an energy gap opens due to spontaneous condensation of bound electron-hole pairs. Ta$_2$NiSe$_5$ is a promising candidate for this type of material, but the…

Realizing an excitonic insulator phase from narrow-gap semiconductors remains challenging, as unambiguous experimental signatures are difficult to establish. Ta$_2$NiSe$_5$ has been widely regarded as a leading candidate, yet the nature of…

Materials Science · Physics 2025-12-11 Keyu Wei , Yixuan Luo , Kenji Watanabe , Takashi Taniguchi , Yanfeng Guo , Xiaoxiang Xi

The excitonic insulator is an intriguing electronic phase of quasi-condensed excitons. A prominent candidate is the small bandgap semiconductor Ta2NiSe5, in which excitons are believed to undergo a BEC-like transition. But experimental…

Ta2NiSe5 is considered a promising excitonic insulator (EI) candidate with slight phonon contributions, since it exhibits a tiny orthorhombic-to-monoclinic structural distortion at 328 K without any superlattice structure. Our synchrotron…

Strongly Correlated Electrons · Physics 2018-08-08 Akitoshi Nakano , Takumi Hasegawa , Shinya Tamura , Naoyuki Katayama , Satoshi Tsutsui , Hiroshi Sawa

Bound electron-hole pairs in semiconductors known as excitons can form a coherent state at low temperatures akin to a BCS condensate. The resulting phase is known as the excitonic insulator and has superfluid properties. Here we…

Strongly Correlated Electrons · Physics 2025-06-06 L. Maisel Licerán , H. T. C. Stoof

The layered chalcogenide Ta2NiSe5 has recently attracted much interest as a strong candidate for the long sought excitonic insulator (EI). Since the physical properties of an EI are expected to depend sensitively on the external pressure,…

Strongly Correlated Electrons · Physics 2023-01-31 H. Okamura , T. Mizokawa , K. Miki , Y. Matsui , N. Noguchi , N. Katayama , H. Sawa , M. Nohara , Y. Lu , H. Takagi , Y. Ikemoto , T. Moriwaki

Many-body interactions can produce novel ground states in a condensed-matter system. For example, interacting electrons and holes can spontaneously form excitons, a neutral bound state, provided that the exciton binding energy exceeds the…

We reveal an ultrafast purely electronic phase transition in \TNS, which is a plausible excitonic insulator, after excited by an ultrafast infrared laser pulse. Specifically, the order parameter of the strong electron-hole binding shrinks…

Strongly Correlated Electrons · Physics 2020-07-01 Tangwei Tang , Hongyuan Wang , Shafeng Duan , Yuanyuan Yang , Chaozhi Huang , Yanfeng Guo , Dong Qian , Wentao Zhang

We study the electronic phase diagram of the excitonic insulator candidates Ta$_2$Ni(Se$_{1-x}$S$_x$)$_5$ [x=0, ... ,1] using Raman spectroscopy. Critical excitonic fluctuations are observed, that diminish with $x$ and ultimately shift to…

Strongly Correlated Electrons · Physics 2021-12-30 Pavel A. Volkov , Mai Ye , Himanshu Lohani , Irena Feldman , Amit Kanigel , Girsh Blumberg

The search for intrinsic excitonic insulators (EI) has long been confounded by coexisting electron-phonon coupling in bulk materials. Although the ground state of an EI may be difficult to differentiate from density-wave orders or other…

Electron-hole pair excitations in semiconductors have been predicted to be able to give rise to a highly correlated many-body ground state, the excitonic insulator (EI). Under appropriate conditions below a critical temperature (Tc),…

Strongly Correlated Electrons · Physics 2023-01-18 Aidan Delgado , Carolin Dusold , Jingwei Jiang , Adam Cronin , Steven G. Louie , Felix R. Fischer

We study the excitonic insulating (EI) phase in the two-band Hubbard models on the Penrose tiling. Performing the real-space mean-field calculations systematically, we obtain the ground state phase diagrams for the vertex and center models.…

Strongly Correlated Electrons · Physics 2020-05-14 Ken Inayoshi , Yuta Murakami , Akihisa Koga

The excitonic insulator is an elusive electronic phase exhibiting a correlated excitonic ground state. Materials with such a phase are expected to have intriguing properties such as excitonic high-temperature superconductivity. However,…

Strongly Correlated Electrons · Physics 2021-12-07 Dominik Christiansen , Malte Selig , Mariana Rossi , Andreas Knorr

Coulomb attraction between electrons and holes in a narrow-gap semiconductor or a semimetal is predicted to lead to an elusive phase of matter dubbed 'excitonic insulator'. However, direct observation of such electronic instability remains…

Strongly Correlated Electrons · Physics 2021-08-09 Kwangrae Kim , Hoon Kim , Jonghwan Kim , Changil Kwon , Jun Sung Kim , B. J. Kim

We investigate the non-equilibrium electronic structure and characteristic time scales in a candidate excitonic insulator, Ta$_2$NiSe$_5$, using time- and angle-resolved photoemission spectroscopy with a temporal resolution of 50 fs.…

The interplay between topology and correlations can generate a variety of quantum phases, many of which remain to be explored. Recent advances have identified monolayer WTe2 as a promising material for doing so in a highly tunable fashion.…

The layered chalcogenide Ta$_{2}$NiSe$_{5}$ has been proposed to host an excitonic condensate in its ground state, a phase that could offer a unique platform to study and manipulate many-body states at room temperature. However, identifying…

Strongly Correlated Electrons · Physics 2021-03-30 Hope M. Bretscher , Paolo Andrich , Prachi Telang , Anupam Singh , Luminita Harnaga , Ajay K. Sood , Akshay Rao

We present an angle-resolved photoemission study of the electronic band structure of the excitonic insulator Ta$_2$NiSe$_5$, as well as its evolution upon Sulfur doping. Our experimental data show that while the excitonic insulating phase…