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The convergent iterative procedure for solving the groundstate Schroedinger equation is extended to derive the excitation energy and the wave function of the low-lying excited states. The method is applied to the one-dimensional quartic…

Quantum Physics · Physics 2009-11-13 R. Friedberg , T. D. Lee , W. Q. Zhao

We introduce a simple generalization of the well known geminal wavefunction already applied in Quantum Chemistry to atoms and small molecules. The main feature of the proposed wavefunction is the presence of the antisymmetric geminal part…

Condensed Matter · Physics 2009-11-10 Michele Casula , Sandro Sorella

Density functional calculations of Rydberg excited states up to high energy are carried out for several molecules using an approach where the orbitals are variationally optimized by converging on saddle points on the electronic energy…

In the realm of photochemistry, the significance of double excitations (also known as doubly-excited states), where two electrons are concurrently elevated to higher energy levels, lies in their involvement in key electronic transitions…

Chemical Physics · Physics 2024-07-15 Fábris Kossoski , Martial Boggio-Pasqua , Pierre-François Loos , Denis Jacquemin

Solving excited states is a challenging task for interacting systems. For one-dimensional critical systems, however, excited states can be directly accessed from the eigenvectors of the local effective Hamiltonian that is constructed from…

Strongly Correlated Electrons · Physics 2026-05-28 Denise Cocchiarella , Mingru Yang , Yueshui Zhang , Mari Carmen Bañuls , Hong-Hao Tu , Yuhan Liu

We present an implementation of range separated functionals utilizing the Slater-function on grids in real space in the projector augmented waves method. The screened Poisson equation is solved to evaluate the necessary screened exchange…

Computational Physics · Physics 2018-07-11 Rolf Würdemann , Michael Walter

We introduce a systematically improvable family of variational wave functions for the simulation of strongly correlated fermionic systems. This family consists of Slater determinants in an augmented Hilbert space involving "hidden"…

Strongly Correlated Electrons · Physics 2022-08-18 Javier Robledo Moreno , Giuseppe Carleo , Antoine Georges , James Stokes

A unified electrodynamic approach to the guided-wave excitation theory is generalized to the waveguiding structures containing a hypothetical space-dispersive medium with drifting charge carriers possessing simultaneously elastic,…

Classical Physics · Physics 2009-10-31 A. A. Barybin

Using a set of oscillator strengths and excited-state dipole moments of near full configuration interaction (FCI) quality determined for small compounds, we benchmark the performances of several single-reference wave function methods (CC2,…

Chemical Physics · Physics 2021-06-14 Rudraditya Sarkar , Martial Boggio-Pasqua , Pierre-François Loos , Denis Jacquemin

Compact and accurate wave functions can be constructed by quantum Monte Carlo methods. Typically, these wave functions consist of a sum of a small number of Slater determinants multiplied by a Jastrow factor. In this paper we study the…

Condensed Matter · Physics 2009-10-30 Chien-Jung Huang , C. J. Umrigar , M. P. Nightingale

We study the mass spectra of excited baryons with the use of the lattice QCD simulations. We focus our attention on the problem of the level ordering between the positive-parity excited state N'(1440) (the Roper resonance) and the…

High Energy Physics - Lattice · Physics 2009-11-11 Kiyoshi Sasaki , Shoichi Sasaki , Tetsuo Hatsuda

Variational perturbation theory is used to determine the decay rates of metastable states across a cubic barrier of arbitrary height. For high barriers, a variational resummation procedure is applied to the complex energy eigenvalues…

Quantum Physics · Physics 2016-08-15 H. Kleinert , I. Mustapic

A multi-reference configuration mixing scheme is used to describe the ground state, characterized by well defined spin and space group symmetry quantum numbers as well as doping fractions $N_{e}/N_{sites}$, of one dimensional Hubbard…

Strongly Correlated Electrons · Physics 2015-06-18 R. Rodríguez-Guzmán , Carlos A. Jiménez-Hoyos , Gustavo E. Scuseria

The complete active space self-consistent field (CASSCF) method is the principal approach employed for studying strongly correlated systems. However, exact CASSCF can only be performed on small active spaces of ~20 electrons in ~20 orbitals…

Computational Physics · Physics 2021-12-22 Daniel S. Levine , Diptarka Hait , Norm M. Tubman , Susi Lehtola , K. Birgitta Whaley , Martin Head-Gordon

We derive a model Hamiltonian whose ground state expectation value of any two-body operator coincides with that obtained with the Jastrow correlated wave function of the many-body Fermi system. Using this Hamiltonian we show that the…

Nuclear Theory · Physics 2009-10-22 R. Cenni , S. Fantoni

We address an old problem in lattice gauge theory - the computation of the spectrum and wave functions of excited states. Our method is based on the Hamiltonian formulation of lattice gauge theory. As strategy, we propose to construct a…

High Energy Physics - Lattice · Physics 2015-05-27 A. Hosseinizadeh , G. Melkonyan , H. Kröger , M. McBreen , N. Scheu

A gas of atoms some of which are in excited electronic state is under consideration. Since the lifetime of an excited state is to great extent larger than the time required for establishing the equilibrium over translational degrees of…

Condensed Matter · Physics 2007-05-23 O. Derzhko , R. Levitskii , O. Chernyavskii

The free energy landscapes of several fundamental processes are characterized by high barriers separating long-lived metastable states. In order to explore these type of landscapes enhanced sampling methods are used. While many such methods…

Chemical Physics · Physics 2019-04-12 Jayashrita Debnath , Michele Invernizzi , Michele Parrinello

We propose optimal estimators for bispectra from excited states. Two common properties of such bispectra are the enhancement in the collinear limit, and the prediction of oscillating features. We review the physics behind excited states and…

Cosmology and Nongalactic Astrophysics · Physics 2015-09-30 P. Daniel Meerburg , Moritz Münchmeyer

We present the ground and excited state spectra of singly, doubly and triply-charmed baryons by using dynamical lattice QCD. A large set of baryonic operators that respect the symmetries of the lattice and are obtained after subduction from…

High Energy Physics - Lattice · Physics 2014-01-23 M. Padmanath , Robert G. Edwards , Nilmani Mathur , Michael Peardon
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