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The addition of filler particles to polymer electrolytes is known to increment their ionic conductivity (IC). A detailed understanding of how the interactions between the constituent materials are responsible for the enhancement, remains to…

Materials Science · Physics 2021-03-19 Andres Villa , Juan Carlos Verduzco , Joseph A. Libera , Ernesto E. Marinero

The electrophoretic behaviour of flexible polyelectrolyte chains ranging from single monomers up to long fragments of hundred repeat units is studied by a mesoscopic simulation approach. Abstracting from the atomistic details of the…

Soft Condensed Matter · Physics 2015-05-13 Kai Grass , Christian Holm

A set of uniform carbon microspheres (CS) whose diameters have the order of $ 0.125 \mu m$ to $10 \mu m $ was prepared from aqueous sucrose solution by means of hydrothermal carbonization of sugar molecules. A pressed pellet was composed by…

Mesoscale and Nanoscale Physics · Physics 2016-11-29 Cesar A. Nieves , Idalia Ramos , Nicholas J. Pinto , Natalya A. Zimbovskaya

We consider equilibrium statistical mechanics of a simplified model for the ideal conductor electrode in an interface contact with a classical semi-infinite electrolyte, modeled by the two-dimensional Coulomb gas of pointlike $\pm$ unit…

Statistical Mechanics · Physics 2009-11-11 L. Samaj , Z. Bajnok

It can be seen by Dynamic Electrical Analysis that the electrical properties of polyetherimide at temperatures above the glass transition are strongly influenced by space charge. We have studied space charge relaxation in two commercial…

Materials Science · Physics 2021-04-01 M. Mudarra , J. Sellares , J. C. Canadas , J. A. Diego

Using Poisson-Boltzmann equation and linear response theory, we derive an effective interaction potential due to a fixed charge distribution in a solution containing polyelectrolytes and point salt. We obtain an expression for the effective…

Soft Condensed Matter · Physics 2016-01-08 Sandipan Dutta , and Y. S. Jho

Based on the method of compact groups of inhomogeneities, we formulate new mixing rules for suspensions of charged insulating particles. They express the quasistatic conductivity and permittivity of a suspension in terms of the effective…

Soft Condensed Matter · Physics 2017-07-18 M. Ya. Sushko , V. Ya. Gotsulskiy , M. V. Stiranets

The new generation of manufacturing technologies such as e.g. additive manufacturing and automated fiber placement has enabled the development of material systems with desired functional and mechanical properties via particular designs of…

Applied Physics · Physics 2019-03-12 Marco Salviato , Sean E. Phenisee

In this study, we propose a theoretical framework to investigate the interactions between flexible polymer chains, specifically polyelectrolytes (PEs). By calculating the system's free energy while considering position-dependent mutual…

Soft Condensed Matter · Physics 2024-05-13 Souradeep Ghosh

The electrical conductivity is calculated for regular inhomogeneous two component isotropic medium in which droplets of one phase with conductivity sigma_2 are embedded in another, with conductivity sigma_1. An expression is formulated…

Statistical Mechanics · Physics 2007-05-23 V. V. Kabanov , K. Zagar , D. Mihailovic

A living polymers transition is found in molecular dynamics simulations of a charge-symmetric size-asymmetric electrolyte with no anisotropic interactions. The fluid has strong polymeric character at low temperatures, where it consists of…

Statistical Mechanics · Physics 2007-05-23 Sorin Bastea

Highly filled conductive polymer composites (CPCs) are widely used in applications such as bipolar plate materials for polymer electrolyte membrane fuel cells and redox flow batteries, electromagnetic interference shielding and sensors due…

Materials Science · Physics 2023-01-03 Thomas Larsen , Tom Larsen , Søren J. Andreasen , Jesper D. C. Christiansen

We consider a binary mixture of chemically active particles, that produce or consume solute molecules, and that interact with each other through the long-range concentrations fields they generate. We analytically calculate the effective…

Soft Condensed Matter · Physics 2024-04-09 Pierre Illien , Ramin Golestanian

The change of the structure of concentrated colloidal suspensions upon addition of non-adsorbing polymer is studied within a two-component, Ornstein-Zernicke based liquid state approach. The polymers' conformational degrees of freedom are…

Soft Condensed Matter · Physics 2009-10-31 M. Fuchs , K. S. Schweizer

The broadening in photoelectron spectra of polymers can be attributed to several factors, such as light source spread, spectrometer resolution, finite lifetime of the hole state, and solid-state effects. Here, for the first time, we set up…

Stretching dynamics of polymers in microfluidics is of particular interest for polymer scientists. As a charged polymer, a polyelectrolyte can be deformed from its coiled equilibrium configuration to an extended chain by applying uniform or…

Soft Condensed Matter · Physics 2014-11-18 Farnoush Farahpour , Fathollah Varnik , Mohammad Reza Ejtehadi

We develop a continuum theory for thermoelectric bodies following the framework of continuum mechanics and conforming to general principles of thermodynamics. For steady states, the governing equations for local fields are intrinsically…

Materials Science · Physics 2012-03-05 Liping Liu

A composite conductive material, which consists of fibers of a high conductivity in a matrix of low conductivity, is discussed. The effective conductivity of the system considered is calculated in Clausius-Mossotti approximation. Obtained…

Materials Science · Physics 2011-03-01 Yuri Kornyushin

We present a set of molecular dynamics (MD) simulations of strongly charged, flexible polyelectrolyte chains under poor solvent conditions in a salt free solution. Structural properties of the chains and of the solutions are reported. By…

Soft Condensed Matter · Physics 2007-05-23 Uwe Micka , Christian Holm , Kurt Kremer

We suppose and develop a simple quantitative model of polymer film conductivity. This model can be seen as a further development of the ideas of Vlasov, Apresyan et al. The main point of the model is that conducting islands exist, and the…

Soft Condensed Matter · Physics 2015-03-17 Andrey Dmitrievich Vlasov