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Related papers: Auger-induced charge migration

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Photons carry one unit of angular momentum associated with their spin~\cite{Beth1936}. Structured vortex beams carry additional orbital angular momentum which can also be transferred to matter~\cite{Allen1992}. This extra twist has been…

Charge acceleration during an intense light field application to solids attracts much attention as elementary processes in high-harmonic generation and photoelectron emission [1-7]. For manipulating such attosecond dynamics of charge,…

Strongly Correlated Electrons · Physics 2020-07-22 Y. Kawakami , T. Amano , H. Ohashi , H. Itoh , Y. Nakamura , H. Kishida , T. Sasaki , G. Kawaguchi , H. M. Yamamoto , K. Yamamoto , S. Ishihara , K. Yonemitsu , S. Iwai

Ultrashort electron pulses are crucial for time-resolved electron diffraction and microscopy of fundamental light-matter interaction. In this work, we study experimentally and theoretically the generation and characterization of attosecond…

Optics · Physics 2018-03-21 Yuya Morimoto , Peter Baum

Laser-plasma electron accelerators can be used to produce high-intensity X-rays, as electrons accelerated in wakefields emit radiation due to betatron oscillations.Such X-ray sources inherit the features of the electron beam;…

Plasma Physics · Physics 2021-04-07 Julien Ferri , Vojtech Horný , Tünde Fülöp

The treatment of the previous paper is extended to molecular wires. Specifically, the effect of electron-vibrational interactions on the electronic transport induced by femtosecond $\omega+2\omega$ laser fields along unbiased molecular…

Quantum Physics · Physics 2009-11-13 Ignacio Franco , Moshe Shapiro , Paul Brumer

Photoionization as a half-scattering process is not instantaneous. Usually, time delays in photoionization are of the order of few tens of attoseconds (1 as = 10$^{-18}$ s). While going from a single atom to a nano-object, one can expect…

The soft character of organic materials leads to strong coupling between molecular nuclear and electronic dynamics. This coupling opens the way to control charge transport in organic electronic devices by inducing molecular vibrational…

Recent progress in orbitronics reveals the possibility of using orbit current as an information carrier. The interconversion between orbit currents and charge currents is crucial for orbit information processing. Although orbit currents can…

Mesoscale and Nanoscale Physics · Physics 2023-03-10 Yong Xu , Fan Zhang , Yongshan Liu , Renyou Xu , Yuhao Jiang , Houyi Cheng , Albert Fert , Weisheng Zhao

This tutorial presents an introduction to the interaction of light and matter on the attosecond timescale. Our aim is to detail the theoretical description of ultra-short time-delays, and to relate these to the phase of extreme ultraviolet…

Atomic Physics · Physics 2012-07-20 J. M. Dahlström , A. L'Huillier , A. Maquet

Ultraintense pulses from X-ray free-electron lasers can drive, within femtoseconds, multiple processes in the inner shells of atoms and molecules in all phases of matter. The ensuing complex ionization pathways of outer-shell electrons from…

Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element…

Atomic Physics · Physics 2016-06-08 S. M. Teichmann , F. Silva , S. L. Cousin , M. Hemmer , J. Biegert

Achieving precise control of photoinduced molecular charge transfer reactions underpins key emerging technologies. As such, the use of hybrid light-matter molecular exciton-polariton states has been proposed as a scheme to directly modify…

The emission of an Auger electron is the predominant relaxation mechanism of core-vacant states in molecules composed of light nuclei. In this non-radiative decay process, one valence electron fills the core vacancy while a second valence…

Chemical Physics · Physics 2023-01-24 Florian Matz , Thomas-C. Jagau

The landscape of ultrafast structured light pulses has recently evolved driven by the capability of high-order harmonic generation (HHG) to up-convert orbital angular momentum (OAM) from the infrared to the extreme-ultraviolet (EUV)…

We describe numerically the ionization process induced by linearly and circularly polarized XUV attosecond laser pulses on an aligned atomic target, specifically, the excited state…

Atomic Physics · Physics 2021-05-26 Juan J. Omiste , Lars Bojer Madsen

We demonstrate the coherent transfer of the orbital angular momentum of a photon to an atom in quantized units of hbar, using a 2-photon stimulated Raman process with Laguerre-Gaussian beams to generate an atomic vortex state in a…

Quantum Physics · Physics 2009-11-13 M. F. Andersen , C. Ryu , Pierre Clade , V. Natarajan , A. Vaziri , K. Helmerson , W. D. Phillips

We explore the role of laser induced anti-alignment in enhancing molecular orientation. A field-free enhanced orientation via anti-alignment scheme is presented, which combines a linearly polarized femtosecond laser pulse with a half-cycle…

Optics · Physics 2009-11-11 E. Gershnabel , I. Sh. Averbukh , Robert J. Gordon

Intense attosecond magnetic field pulses are predicted to be produced by intense few cycle circularly polarized UV pulses. Numerical solutions of the time dependent Schr\"{o}dinger equation for H$_2^+$ are used to study the dynamical…

Optics · Physics 2013-07-24 Kai-Jun Yuan , Andre D. Bandrauk

We determine charge transfer statistics in a quantum conductor driven by a time-dependent voltage and identify the elementary transport processes. At zero temperature unidirectional and bidirectional single charge transfers occur. The…

Mesoscale and Nanoscale Physics · Physics 2008-12-10 Mihajlo Vanevic , Yuli V. Nazarov , Wolfgang Belzig

Atomic motion dynamics during structural changes or chemical reactions have been visualized by picosecond and femtosecond pulsed electron beams via ultrafast electron diffraction and microscopy. Imaging the even faster dynamics of electrons…

Optics · Physics 2019-05-15 Martin Kozák , Norbert Schönenberger , Peter Hommelhoff