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Interactions of electron spins with rotational degrees of freedom during collisions or with external fields are fundamental processes that limit the coherence time of spin gases. We experimentally study the decoherence of hot cesium spins…

Quantum Physics · Physics 2025-05-29 Mark Dikopoltsev , Avraham Berrebi , Uriel Levy , Or Katz

We propose a general protocol for on-demand generation of robust entangled states of nuclear and/or electron spins of ultracold $^1\Sigma$ and $^2\Sigma$ polar molecules using electric dipolar interactions. By encoding a spin-1/2 degree of…

Quantum Physics · Physics 2023-04-10 Timur V. Tscherbul , Jun Ye , Ana Maria Rey

Strongly interacting spins underlie many intriguing phenomena and applications ranging from magnetism to quantum information processing. Interacting spins combined with motion display exotic spin transport phenomena, such as superfluidity…

Ultra-cold atoms trapped in an optical dipole trap and prepared in a coherent superposition of their hyperfine ground states, decohere as they interact with their environment. We demonstrate than the loss in coherence in an "echo"…

Quantum Physics · Physics 2016-08-16 M. F. Andersen , A. Kaplan , T. Grünzweig , N. Davidson

We report on the enhancement of the spin coherence time (T2) by almost an order-of-magnitude in exciton-polariton condensates through driven spin precession resonance. Using a rotating optical trap formed by a bichromatic laser excitation,…

Quantum Gases · Physics 2026-05-14 Ivan Gnusov , Alexey Yulin , Stepan Baryshev , Sergey Alyatkin , Pavlos G. Lagoudakis

A detailed treatment of an electro-optical trap for polar molecules, realized by embedding an optical trap within a uniform electrostatic field, is presented and the trap's properties analyzed and discussed. The electro-optical trap offers…

Atomic Physics · Physics 2022-06-15 Bretislav Friedrich

We show that the electric dipole-dipole interaction between a pair of polar molecules undergoes an all-out transformation when superimposed by a far-off resonant optical field. The combined interaction potential becomes tunable by variation…

Atomic Physics · Physics 2015-05-30 Mikhail Lemeshko , Bretislav Friedrich

We examine the potential-energy curves and polarization of the dipole moments of two static polar molecules under the influence of an external dc electric field and their anisotropic dipole-dipole interaction. We model the molecules as…

Quantum Physics · Physics 2024-09-24 Felipe Isaule , Robert Bennett , Jörg B. Götte

We use state- and time-resolved coherent Raman spectroscopy to study the rotational dynamics of oxygen molecules in ultra-high rotational states. While it is possible to reach rotational quantum numbers up to $N \approx 50$ by increasing…

Chemical Physics · Physics 2015-06-19 Alexander A. Milner , Aleksey Korobenko , Valery Milner

Nuclear spins of noble gases can maintain coherence for hours at ambient conditions owing to their extraordinary isolation by the enclosing, complete electronic shells. This isolation, however, impedes the ability to manipulate and control…

Quantum Physics · Physics 2023-11-06 Roy Shaham , Or Katz , Ofer Firstenberg

We study the fully itinerant dynamics of ultracold but nondegenerate polar molecules with a spin-$1/2$ degree of freedom encoded into two of their electric field dressed rotational states. Center of mass molecular motion is constrained to…

Quantum Gases · Physics 2025-06-10 Reuben R. W. Wang , John L. Bohn

We report on the optical polarizability of microwave-shielded ultracold NaCs molecules in an optical dipole trap. While dressing a pair of rotational states with a microwave field, we observe a marked dependence of the optical…

Quantum Gases · Physics 2025-01-16 Siwei Zhang , Weijun Yuan , Niccolò Bigagli , Claire Warner , Ian Stevenson , Sebastian Will

We propose and analyze an electrostatic-optical nano-scale trap for cold diatomic polar molecules. The main ingredient of our proposal is an square-array of ferroelectric nano-rods {with alternating polarization}. We show that, in contrast…

Quantum Gases · Physics 2018-02-21 Omjyoti Dutta , Geza Giedke

Tightly focused optical dipole traps induce vector light shifts ("fictitious magnetic fields") which complicate their use for single-atom trapping and manipulation. The problem can be mitigated by adding a larger, real magnetic field, but…

Atomic Physics · Physics 2018-02-14 Sébastien Garcia , Jakob Reichel , Romain Long

Simultaneous two-dimensional trapping of neutral dipolar molecules in low- and high-field seeking states is analyzed. A trapping potential of the order of 20 mK can be produced for molecules like ND3 with time-dependent electric fields. The…

Chemical Physics · Physics 2009-11-10 T. Junglen , T. Rieger , S. A. Rangwala , P. W. H. Pinkse , G. Rempe

We investigate the properties of two interacting ultracold polar molecules described as distinguishable quantum rigid rotors, trapped in a one-dimensional harmonic potential. The molecules interact via a multichannel two-body contact…

Atomic Physics · Physics 2018-07-03 Anna Dawid , Maciej Lewenstein , Michał Tomza

This paper reviews recent advances in the study of strongly interacting systems of dipolar molecules. Heteronuclear molecules feature large and tunable electric dipole moments, which give rise to long-range and anisotropic dipole-dipole…

Quantum Gases · Physics 2016-07-14 Bryce Gadway , Bo Yan

Optical dipole-traps are used in various scientific fields, including classical optics, quantum optics and biophysics. Here, we propose and implement a dipole-trap for nanoparticles that is based on focusing from the full solid angle with a…

We investigate magic-wavelength trapping of ultracold bialkali molecules in the vicinity of weak optical transitions from the vibrational ground state of the X$^1\Sigma^+$ potential to low-lying rovibrational states of the b$^3\Pi_0$…

Quantum Physics · Physics 2021-04-14 Q. Guan , S. L. Cornish , S. Kotochigova

We investigate an optically trapped exciton-polariton condensate and observe temporal coherence beyond 1~ns duration. Due to the reduction of the spatial overlap with the thermal reservoir of excitons, the coherence time of the trapped…

Mesoscale and Nanoscale Physics · Physics 2021-06-28 K. Orfanakis , A. F. Tzortzakakis , D. Petrosyan , P. G. Savvidis , H. Ohadi